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The conductance of single molecule junctions is calculated using a Landauer approach combined to many-body perturbation theory MBPT) to account for electron correlation. The mere correction of the density-functional theory eigenvalues,…

Mesoscale and Nanoscale Physics · Physics 2015-05-27 T. Rangel , A. Ferretti , P. E. Trevisanutto , V. Olevano , G. -M. Rignanese

The ability to control the conductance of single molecules will have a major impact in nanoscale electronics. Azobenzene, a molecule that changes conformation as a result of a trans/cis transition when exposed to radiation, could form the…

Mesoscale and Nanoscale Physics · Physics 2008-11-26 Miriam del Valle , Rafael Gutierrez , Carlos Tejedor , Gianaurelio Cuniberti

We study the low-energy electronic properties of a junction made of two crossed metallic carbon nanotubes of general chiralities. We derive a tight binding tunneling matrix element that couples low-energy states on the two tubes, which…

Mesoscale and Nanoscale Physics · Physics 2013-10-29 A. A. Maarouf , E. J. Mele

Electromigrated nanoscale junctions have proven very useful for studying electronic transport at the single-molecule scale. However, confirming that conduction is through precisely the molecule of interest and not some contaminant or metal…

Mesoscale and Nanoscale Physics · Physics 2008-09-04 D. R. Ward , G. D. Scott , Z. K. Keane , N. J. Halas , D. Natelson

We report detailed atomistic simulations combined with high-fidelity conductance calculations to probe the structural origins of conductance fluctuations in thermally evolving Au-benzene-1,4-dithiolate-Au junctions. We compare the behavior…

Mesoscale and Nanoscale Physics · Physics 2013-03-07 William R. French , Christopher R. Iacovella , Ivan Rungger , Amaury Melo Souza , Stefano Sanvito , Peter T. Cummings

The process of creating an atomically defined and robust metallic tip is described and quantified using measurements of contact conductance between gold electrodes and numerical simulations. Our experiments show how the same conductance…

Materials Science · Physics 2012-05-30 C. Sabater , C. Untiedt , J. J. Palacios , M. J. Caturla

A quantum dot is a sub-micron-scale conducting device containing up to several thousand electrons. Transport through a quantum dot at low temperatures is a quantum-coherent process. This review focuses on dots in which the electron's…

Mesoscale and Nanoscale Physics · Physics 2008-11-26 Y. Alhassid

We present a comprehensive study of the properties of the off-resonant conductance spectrum in oligomer nanojunctions between graphitic electrodes. By employing first-principle-based methods and the Landauer approach of quantum transport,…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Giorgos Fagas , Agapi Kambili

We create two molecular devices with superconducting junctions, using nickelocene molecules, single Fe atoms, and Pb electrodes at low temperature. We find contrasting behavior based on the coordination of the Fe atom: one device shows…

Using an atomic force microscope we have created nanotube junctions such as buckles and crossings within individual single-wall metallic carbon nanotubes connected to metallic electrodes. The electronic transport properties of these…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 Henk W. Ch. Postma , Mark de Jonge , Zhen Yao , Cees Dekker

We present a theoretical study of the conductance and thermopower of single-molecule junctions based on C60 and C60-terminated molecules. We first analyze the transport properties of gold-C60-gold junctions and show that these junctions can…

Mesoscale and Nanoscale Physics · Physics 2012-06-08 S. Bilan , L. A. Zotti , F. Pauly , J. C. Cuevas

The transport properties of a conduction junction model characterized by two mutually coupled channels that strongly differ in their couplings to the leads are investigated. Models of this type describe molecular redox junctions (where a…

Mesoscale and Nanoscale Physics · Physics 2015-06-16 Alexander J. White , Agostino Migliore , Michael Galperin , Abraham Nitzan

Based on the non-equilibrium Green's function (NEGF) technique and the Landauer-B\"{u}ttiker theory, the possibility of a molecular spin-electronic device, which consists of a single C$_{60}$ molecule attached to two ferromagnetic…

Mesoscale and Nanoscale Physics · Physics 2008-12-31 Alireza Saffarzadeh

One of the major industrial challenges is to profit from some fascinating physical features present at the nanoscale. The production of dissipationless nanoswitches (or nanocontacts) is one of such attractive applications. Nevertheless, the…

Interfaces play a crucial role in energy transport at the nanoscale. However, direct experimental observations of interfacial thermal conductance across molecular junctions have remained challenging due to the high spatiotemporal resolution…

Chemical Physics · Physics 2025-12-23 Md. Shahriar Hossain Shuvo , Xing He , Mithun Ghosh , Ding-Shyue Yang

We collect evidences on existence of microscopic solitons, and their determining role in electronic processes of quasi-1D conductors. The ferroelectric charge ordering gives access to several types of solitons in conductivity and…

Strongly Correlated Electrons · Physics 2009-11-13 S. Brazovskii

We show that individual dopant atoms dominate the transport characteristics of nanometer sized devices, by investigating metal semiconductor diodes down to 15 nm diameter. Room temperature measurements reveal a strongly increasing scatter…

Condensed Matter · Physics 2009-11-10 G. D. J. Smit , S. Rogge , J. Caro , T. M. Klapwijk

Atomic quantum point contacts accommodate a small number of conduction channels. Their number N and transmission coefficients {T_n} can be determined by analyzing the subgap structure due to multiple Andreev reflections in the…

Superconductivity · Physics 2009-10-31 E. Scheer , J. C. Cuevas , A. Levy Yeyati , A. Martin-Rodero , P. Joyez , M. H. Devoret , D. Esteve , C. Urbina

By carrying out density functional theory (DFT) analysis within the Keldysh non-equilibrium Green's function (NEGF) framework, we investigate the quantum transport properties of Au-C60-Au molecular junctions from the first principles. We…

Materials Science · Physics 2007-05-23 N. Sergueev , D. Roubtsov , H. Guo

We analyze the effect of a gate on the conductance of molecules by separately evaluating the gate-induced polarization and the potential shift of the molecule relative to the leads. The calculations use ab initio density functional theory…

Materials Science · Physics 2007-05-23 San-Huang Ke , Harold U. Baranger , Weitao Yang