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Upon reduction of the film thickness we observe a metal-insulator transition in epitaxially stabilized, spin-orbit coupled SrIrO$_3$ ultrathin films. By comparison of the experimental electronic dispersions with density functional theory at…

Strongly Correlated Electrons · Physics 2017-12-27 P. Schütz , D. Di Sante , L. Dudy , J. Gabel , M. Stübinger , M. Kamp , Y. Huang , M. Capone , M. -A. Husanu , V. Strocov , G. Sangiovanni , M. Sing , R. Claessen

We study the resistive switching triggered by an applied electrical bias in antiferromagnetic Mott insulator Sr(3)Ir(2)O(7). The switching was previously associated with an electric-field driven structural transition. Here we use…

Materials Science · Physics 2018-05-02 Morgan Williamson , Shida Shen , Gang Cao , Jianshi Zhou , John B. Goodenough , Maxim Tsoi

The insulating ground state of the 5d transition metal oxide CaIrO3 has been classified as a Mott-type insulator. Based on a systematic density functional theory (DFT) study with local, semilocal, and hybrid exchange-correlation…

Strongly Correlated Electrons · Physics 2015-09-04 Sun-Woo Kim , Chen Liu , Hyun-Jung Kim , Jun-Ho Lee , Yongxin Yao , Kai-Ming Ho , Jun-Hyung Cho

The presence of spin-orbit coupling drives the anomalous magnetotransport at oxide interfaces and forms the basis for numerous intriguing properties of these 2D electron systems, such as topologically protected phases or anti-localization.…

Strongly Correlated Electrons · Physics 2018-02-28 Patrick Seiler , Jone Zabaleta , Robin Wanke , Jochen Mannhart , Thilo Kopp , Daniel Braak

Spin-orbit entangled magnetic dipoles, often referred to as pseudospins, provide a new avenue to explore novel magnetism inconceivable in the weak spin-orbit coupling limit, but the nature of their low-energy interactions remains to be…

Time-of-flight inelastic neutron scattering measurements on Sr2IrO4 single crystals were performed to access the spin Hamiltonian in this canonical Jeff=1/2 spin-orbital Mott insulator. The momentum of magnetic scattering at all inelastic…

Strongly Correlated Electrons · Physics 2018-12-12 S. Calder , D. M. Pajerowski , M. B. Stone , A. F. May

The alloy Ca$_{2-x}$Sr$_x$RuO$_4$ exhibits a complex phase diagram with peculiar magnetic metallic phases. In this paper some aspects of this alloy are discussed based on a mean field theory for an effective Kugel-Khomskii model of…

Strongly Correlated Electrons · Physics 2007-05-23 Manfred Sigrist , Matthias Troyer

We report a La2CuO4-like interlayer antiferromagnetic order in Sr2IrO4 films with large orthorhombic distortion (> 1.5%). The biaxial lattice strain in epitaxial heterostructures of Sr2IrO4/Ca3Ru2O7 lowers the crystal symmetry of Sr2IrO4…

Strongly Correlated Electrons · Physics 2022-03-23 S. Shrestha , M. Krautloher , M. Zhu , J. Kim , J. Hwang , J. Kim , J. -W. Kim , B. Keimer , A. Seo

Bilayer CrI$_3$ attracted much attention owing to peculiar switching between the layered ferromagnetic and antiferromagnetic order upon stacking alternation. This finding pointed out the importance of the apparently small interlayer…

Materials Science · Physics 2024-06-19 Srdjan Stavrić , Paolo Barone , Silvia Picozzi

The temperature dependence and anisotropy of optical spectral weights associated with different multiplet transitions is determined by the spin and orbital correlations. To provide a systematic basis to exploit this close relationship…

Strongly Correlated Electrons · Physics 2007-05-23 Andrzej M. Oles , Giniyat Khaliullin , Peter Horsch , Louis Felix Feiner

We report on the longitudinal magnetoresistance (MR) in thin metal films on an Ising-type antiferromagnetic insulator, Na5Co15.5Te6O36 (NCTO). Steep changes in the MR spectra with hysteresis were observed at spin-flip transitions driven by…

Strongly Correlated Electrons · Physics 2026-05-04 Hirotsugu Tagami , Takuya Kawada , Yuki Shiomi

In quantum magnetism spin dimers are typically associated with spin-singlet states. To date, $triplet$ $dimerization$ has not been observed in any 3D or quasi-2D material. With this in mind we here discuss the electronic structure of the…

Antiferromagnetic spintronics actively introduces new principles of magnetic memory, in which the most fundamental spin-dependent phenomena, i.e. anisotropic magnetoresistance effects, are governed by an antiferromagnet instead of a…

Materials Science · Physics 2018-05-08 Chengliang Lu , Bin Gao , Haowen Wang , Wei Wang , Songliu Yuan , Shuai Dong , Jun-Ming Liu

The nature of insulating phase in 5$d$ based Sr$_2$IrO$_4$ is quite debated as the theoretical as well as experimental investigations have put forward evidences in favor of both magnetically driven Slater-type and interaction driven…

Strongly Correlated Electrons · Physics 2017-02-08 Imtiaz Noor Bhatti , A. K. Pramanik

One way to induce insulator to metal transitions in the spin-orbit Mott insulator Sr2IrO4 is to substitute iridium with transition metals (Ru, Rh). However, this creates intriguing inhomogeneous metallic states, which cannot be described by…

Strongly Correlated Electrons · Physics 2021-09-08 Véronique Brouet , Paul Foulquier , Alex Louat , François Bertran , Patrick Le Fèvre , Julien E. Rault , Dorothée Colson

We discuss the notions of spin-orbital polarization and ordering in paramagnetic materials, and address their consequences in transition metal oxides. Extending the combined density functional and dynamical mean field theory scheme to the…

Strongly Correlated Electrons · Physics 2014-12-16 Cyril Martins , Markus Aichhorn , Loig Vaugier , Silke Biermann

Nanoscale superlattices with uniaxial ferromagnetic layers antiferromagnetically coupled through non-magnetic spacers are recently used as components of magnetoresistive and recording devices. In the last years intensive experimental…

Materials Science · Physics 2015-06-24 U. K. Roessler , A. N. Bogdanov

Sr2IrO4 exhibits a novel insulating state assisted by spin-orbit interactions. A series of polycrystalline samples of Sr2-xIrO4 have been synthesized. It is found that deep Sr-vacancies of Sr2-xIrO4 greatly reduce the rotation of IrO6…

Strongly Correlated Electrons · Physics 2016-11-01 Xuanyong Sun , S. L. Liu , Haiyun Wang , Bin Li , Jie Cheng , Z. H. Wang

Spin spirals form inside the magnetic layers of antiferromagnetic and noncollinearly-coupled magnetic multilayers in the presence of an external magnetic field. This spin structure can be modeled to extract the direct exchange stiffness of…

Mesoscale and Nanoscale Physics · Physics 2024-09-04 Elliot Wadge , Afan Terko , George Lertzman-Lepofsky , Paul Omelchenko , Bret Heinrich , Manuel Rojas , Erol Girt

We report point-contact measurements of anisotropic magnetoresistance (AMR) in a single crystal of antiferromagnetic (AFM) Mott insulator Sr2IrO4. The point-contact technique is used here as a local probe of magnetotransport properties on…

Mesoscale and Nanoscale Physics · Physics 2014-12-03 Cheng Wang , Heidi Seinige , Gang Cao , Jian-Shi Zhou , John B. Goodenough , Maxim Tsoi