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Dynamic nuclear polarisation, which transfers the spin polarisation of electrons to nuclei, is routinely applied to enhance the sensitivity of nuclear magnetic resonance; it is also critical in spintronics, particularly when spin…

We simulate the dynamics of varying density quasi-two-dimensional spin ensembles in solid-state systems, focusing on the nitrogen-vacancy centers in diamond. We consider the effects of various control sequences on the averaged dynamics of…

Quantum Physics · Physics 2018-09-25 D. Farfurnik , Y. Horowicz , N. Bar-Gill

The sensing capability of a single optically bright electronic spin in diamond can be enhanced by making use of proximal dark nuclei as ancillary spins. Such systems, so far only realized in bulk diamond, provide orders of magnitude higher…

Quantum Physics · Physics 2017-10-04 Helena S. Knowles , Dhiren M. Kara , Mete Atatüre

We investigate the coherence properties of individual nuclear spin quantum bits in diamond [Dutt et al., Science, 316, 1312 (2007)] when a proximal electronic spin associated with a nitrogen-vacancy (NV) center is being interrogated by…

The use of the nuclear spins surrounding electron spin qubits as quantum registers and long-lived memories opens the way to new applications in quantum information and biological sensing. Hence, there is a need for generic and robust forms…

Quantum Physics · Physics 2021-07-06 O. T. Whaites , J. Randall , T. H. Taminiau , T. S. Monteiro

We study a mechanism by which nuclear hyperpolarization due to the polarization transfer from a microwave-pulse-controlled electron spin is suppressed. From analytical and numerical calculations of the unitary dynamics of multiple nuclear…

Quantum Physics · Physics 2024-03-12 Kento Sasaki , Eisuke Abe

Nuclear spins are highly coherent quantum objects. In large ensembles, their control and detection via magnetic resonance is widely exploited, e.g. in chemistry, medicine, materials science and mining. Nuclear spins also featured in early…

Coherent control and optical readout of the electron spin of the $^{29}$SiV$^{-}$ center in diamond has been demonstrated in literature, with exciting prospects for implementations as memory nodes and spin qubits. Nuclear spins may be even…

Quantum Physics · Physics 2022-06-15 Hyma H. Vallabhapurapu , Chris Adambukulam , Andre Saraiva , Arne Laucht

We consider an electronic spin, such as a nitrogen-vacancy (NV) center in diamond, weakly coupled to a large number (bath) of nuclear spins, and subjected to the Rabi driving with a periodically alternating phase (multiple rotary echo). We…

Mesoscale and Nanoscale Physics · Physics 2015-03-25 V. V. Mkhitaryan , F. Jelezko , V. V. Dobrovitski

Recently, magnetic field sensors based on an electron spin of a nitrogen vacancy (NV) center in diamond have been studied both from an experimental and theoretical point of view. This system provides a nanoscale magnetometer, and it is…

Dynamical polarization of nuclear spin ensembles is of central importance for magnetic resonance studies, precision sensing and for applications in quantum information theory. Here we propose a scheme to generate long-lived singlet pairs in…

Quantum Physics · Physics 2017-04-06 Johannes N. Greiner , D. D. Bhaktavatsala Rao , Jörg Wrachtrup

Single electron spins coupled to multiple nuclear spins provide promising multi-qubit registers for quantum sensing and quantum networks. The obtainable level of control is determined by how well the electron spin can be selectively coupled…

Quantum networks will rely on photons entangled to robust, local quantum registers for computation and error correction. We demonstrate control of and entanglement in a fully connected three-qubit $^{13}\mathrm{C}$ nuclear spin register in…

Quantum Physics · Physics 2025-08-08 Marco Klotz , Andreas Tangemann , David Opferkuch , Alexander Kubanek

We propose a scheme to achieve nuclear-nuclear indirect interactions mediated by a mechanically driven nitrogen-vacancy (NV) center in diamond. Here we demonstrate two-qubit entangling gates and quantum-state transfer between two carbon…

Quantum Physics · Physics 2022-11-18 Wan-Jun Su , Guang-Zheng Ye , Ya-Dong Wu , Zhen-Biao Yang , Barry C. Sanders

Electron and nuclear spins associated with point defects in insulators are promising systems for solid state quantum technology. While the electron spin usually is used for readout and addressing, nuclear spins are exquisite quantum bits…

The nuclear spin is a prime candidate for quantum information applications due to its weak coupling to the environment and inherently long coherence times. However, this weak coupling also challenges the addressability of the nuclear spin.…

Quantum Physics · Physics 2025-12-15 Hester G. Vennema , Cristina Mier , Evert W. Stolte , Leonard Edens , Jinwon Lee , Sander Otte

An interacting spin system is an excellent testbed for fundamental quantum physics and applications in quantum sensing and quantum simulation. For these investigations, detailed information of the interactions, e.g., the number of spins and…

Quantum Physics · Physics 2024-11-12 Yuhang Ren , Susumu Takahashi

We demonstrate a novel method for coherent optical manipulation of individual nuclear spins in the solid state, mediated by the electronic states of a proximal quantum emitter. Specifically, using the nitrogen-vacancy (NV) color center in…

Quantum Physics · Physics 2020-04-22 M. L. Goldman , T. L. Patti , D. Levonian , S. F. Yelin , M. D. Lukin

We perform sensitive nuclear magnetic resonance (NMR) with spin ensembles which are polarized by nitrogen vacancy centers (NV centers) in diamond at room-temperature. With a near shot-noise-limited photoluminescence detection and a highly…

Rare-earth related electron spins in crystalline hosts are unique material systems, as they can potentially provide a direct interface between telecom band photons and long-lived spin quantum bits. Specifically, their optically accessible…

Quantum Physics · Physics 2020-05-06 Thomas Kornher , Da-Wu Xiao , Kangwei Xia , Fiammetta Sardi , Nan Zhao , Roman Kolesov , Jörg Wrachtrup