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We present a first-principles scheme for computing the magnetoelectric response of multiferroics. We apply our method to BiFeO3 (BFO) and related compounds in which Fe is substituted by other magnetic species. We show that under certain…

Materials Science · Physics 2012-04-17 Jacek C. Wojdel , Jorge Iniguez

We use a Green's function method with Random Phase Approximation to show how magnetic correlations may affect electric polarization in multiferroic materials with magnetic-exchange-type magnetoelectric coupling. We use a model spin 1/2…

Materials Science · Physics 2010-02-17 K. L. Livesey , R. L. Stamps

The development of new computing technologies has given a new stimulus in the study of multiferroics. The use of multiferroics allows the realization of competitive energy efficient scalable logic and storage devices. The low-power…

Materials Science · Physics 2023-10-10 Z. V. Gareeva , N. V. Shulga , A. K. Zvezdin

Materials that exhibit ferroaxial order hold potential for novel multiferroic applications. However, in pure ferroaxials, domains are not directly coupled to stress or static electric field due to their symmetry, limiting the ability to…

Materials Science · Physics 2024-05-16 Zhiren He , Guru Khalsa

We show that for Ni$_3$V$_2$O$_8$ long-range ferroelectric and incommensurate magnetic order appear simultaneously in a single phase transition. The temperature and magnetic field dependence of the spontaneous polarization show a strong…

The olivine compound Mn2GeO4 is shown to feature both a ferroelectric polarization and a ferromagnetic magnetization that are directly coupled and point along the same direction. We show that a spin spiral generates ferroelectricity (FE),…

Materials Science · Physics 2012-08-07 J. S. White , T. Honda , K. Kimura , T. Kimura , Ch. Niedermayer , O. Zaharko , A. Poole , B. Roessli , M. Kenzelmann

For the past decades, the low-temperature phase of Ca$_3$Ru$_2$O$_7$ below the 48K first-order phase transition remains a puzzle with controversial suggestions involving metallic ferroelectric, orbital or magnetic ordering. Through analysis…

Strongly Correlated Electrons · Physics 2018-09-13 Zheting Jin , Wei Ku

LuFe2O4 often is considered as a prototypical multiferroic with polar order arising from the electronic degrees of freedom only ("electronic ferroelectricity"). In the present work, we check the intrinsic nature of the dielectric response…

Strongly Correlated Electrons · Physics 2012-08-31 A. Ruff , S. Krohns , F. Schrettle , V. Tsurkan , P. Lunkenheimer , A. Loidl

Using a joint approach of density functional theory and model calculations, we demonstrate that a prototypical charge ordered half-doped manganite, La$_{1/2}$Ca$_{1/2}$MnO$_3$ is multiferroic. The combination of a peculiar charge-orbital…

Materials Science · Physics 2010-07-15 Gianluca Giovannetti , Sanjeev Kumar , Jeroen van den Brink , Silvia Picozzi

Ferroic transition metal oxides, which exhibit spontaneous elastic, electrical, magnetic or toroidal order, exhibit functional properties that find use in ultrastable solid-state memories to sensors and medical imaging technologies. To…

Materials Science · Physics 2015-03-20 Andrew T. Mulder , Nicole A. Benedek , James M. Rondinelli , Craig J. Fennie

It has been recently demonstrated that the magnetic state of FeRh can be controlled by electric fields in FeRh/BaTiO$_{\text{3}}$ heterostructures [R.O. Cherifi et al. Nature Mater. 13, 345 (2014)]. Voltage-controlled changes in the…

Multiferroic materials combine multiple ferroic orders that may enable cross-functionalities, e.g. control of one ferroic order by the field conjugate to the other one. BaCoSiO$_4$, a recently proposed multiferroic combines multiple unit…

Materials Science · Physics 2024-07-04 Aditya Putatunda , Sergey Artyukhin

The interplay of light and magnetism has been a topic of interest since the original observations of Faraday and Kerr where magnetic materials affect the light polarization. While these effects have historically been exploited to use light…

Recently, oxide multiferroics have attracted much attention due to their large magnetoelectric effect which allows the tuning of magnetic properties with electric field and vice versa and open new venues for future spintronic applications…

Strongly Correlated Electrons · Physics 2010-10-12 M. Cazayous , Y. Gallais , A. Sacuto , R. De Sousa , D. Lebeugle , D. Colson

Magnetoelectric multiferroic materials, particularly type-II multiferroics where ferroelectric polarizations arise from magnetic order, offer significant potential for the simultaneous control of magnetic and electric properties. However,…

Strongly Correlated Electrons · Physics 2025-03-04 Blake S. Dastrup , Zhuquan Zhang , Peter R. Miedaner , Yu-Che Chien , Young Sun , Yan Wu , Huibo Cao , Edoardo Baldini , Keith A. Nelson

We present a simple two-dimensional model in which the lattice degrees of freedom mediate the interactions between magnetic moments and electric dipoles. This model reproduces basic features, such as a sudden electric polarization…

Strongly Correlated Electrons · Physics 2022-04-06 L. Pili , R. A. Borzi , D. C. Cabra , S. A. Grigera

Electronic structure and dielectric property in an electronic ferroelectricty, where electric polarization is driven by an electronic charge order without inversion symmetry, are studied. Motivated from layered iron oxides, roles of quantum…

Strongly Correlated Electrons · Physics 2015-05-19 Tsutomu Watanabe , Sumio Ishihara

We propose the phenomenological description of ferroelectric disordering in ferroelectric-semiconductors caused by charged impurities with the charge density random fluctuations. The material improper conductivity is proportional to the…

Materials Science · Physics 2007-05-23 Anna N. Morozovska , Eugeny A. Eliseev

The coupling between localized spins and phonons can lead to shifts in the dielectric constant of insulating materials at magnetic ordering transitions. Studies on isostructural SeCuO3 (ferromagnetic) and TeCuO3 (antiferromagnetic)…

Materials Science · Physics 2009-04-14 G. Lawes , T. Kimura , C. M. Varma , M. A. Subramanian , R. J. Cava , A. P. Ramirez

Multiferroics are singular materials that can display simultaneously electric and magnetic orders. Some of them can be ferroelectric and ferromagnetic and, for example, provide the unique opportunity of encoding information independently in…