Related papers: Molecular vibrations-induced quantum beats in two-…
Reconstruction of attosecond beating by interference of two-photon transitions (RABBITT) is a powerful photoelectron spectroscopy, offering direct access to internal dynamics of the target. It is being increasingly applied to molecular…
Techniques for coherent multidimensional optical spectroscopy have been developed and utilised to understand many different processes, including energy transfer in photosynthesis and many-body effects in semiconductor nanostructures.…
Spectroscopy is an indispensable tool in understanding the structures and dynamics of molecular systems. However computational modelling of spectroscopy is challenging due to the exponential scaling of computational complexity with system…
The dynamics of a wide range of technologically important quantum systems are dominated by their interaction with just a few environmental modes. Such highly structured environments give rise to long-lived bath correlations that induce…
We consider nonlinear spectroscopic effects - interaction-enhanced double resonance and spectrum instability - that appear in ultracold quantum gases owing to collisional frequency shift of atomic transitions and, consequently, due to the…
We briefly review the oscillator and spin bath models of quantum environments, which can be used to describe the low-energy dynamics of open quantum systems. We then use them to discuss both the mechanisms causing decoherence at low $T$,…
We study the influence of the phonon environment on the electron dynamics in a doped quantum dot molecule. A non-perturbative quantum kinetic theory based on correlation expansion is used in order to describe both diagonal and off-diagonal…
The quantum dynamics of mesoscopic or macroscopic systems is always complicated by their coupling to many "environmental" modes.At low T these environmental effects are dominated by localised modes, such as nuclear and paramagnetic spins,…
We identify an intriguing feature of the electron-vibrational dynamics of molecular systems via a computational examination of \emph{trans}-polyacetylene oligomers. Here, via the vibronic interactions, the decay of an electron in the…
A double quantum dot device is a tunable two-level system for electronic energy states. A dc electron current directly measures the rates for elastic and inelastic transitions between the two levels. For inelastic transitions energy is…
We report an anomalous decoherence phenomenon of a quantum dissipative system in the framework of a stochastic decoupling scheme along with a hierarchical equations-of-motion formalism without the usual Born-Markov or weak coupling…
We analyze excited-state quantum phase transitions (ESQPTs) in three schematic (integrable and nonintegrable) models describing a single-mode bosonic field coupled to a collection of atoms. It is shown that the presence of the ESQPT in…
The behavior of polyatomic molecules around their equilibrium positions can be regarded as quantum coupled anharmonic oscillators. Solving the corresponding Schr\"odinger equations can interpret or predict experimental spectra of molecules.…
Transition metal complexes for photochemical applications often feature a high density of electron-vibrational states characterized by nonadiabatic and spin-orbit couplings. Overall, the dynamics after photoexcitation is shaped by rapid…
We analytically tackle opto-vibronic interactions in molecular systems driven by either classical or quantum light fields. In particular, we examine a simple model of molecules with two relevant electronic levels, characterized by potential…
A time-dependent theory for the interactions between spatially separated lossy cavities in a homogeneous background medium using quantized quasinormal modes (QNMs) is presented. The cavities interact via a bath of traveling photons,…
The ultrafast quantum dynamics of photophysical processes in complex molecules is an extremely challenging computational problem with a wide variety of fascinating applications in quantum chemistry and biology. Inspired by recent…
The idea that excitonic state (electronic) coherences are of fundamental importance to natural photosynthesis gained popularity when, a decade ago, slowly dephasing quantum beats were observed in the two-dimensional electronic spectra of…
We introduce multi-pulse quantum noise spectroscopy protocols for spectral estimation of the noise affecting multiple qubits coupled to Gaussian dephasing environments including both classical and quantum sources. Our protocols are capable…
In this paper we give a general introduction to quantum critical phenomena, which we practically illustrate by a detailed study of the low energy properties of the spin boson model (SBM), describing the dynamics of a spin 1/2 impurity (or…