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We investigate how proximity to a metal nanostructure, particularly to a flat mirror or a cavity confined between two mirrors, affects the vibronic structure of Raman scattering signals. We find that such proximity, particularly for the…

Optics · Physics 2026-05-28 Zeyu Zhou , Maxim Sukharev , Abraham Nitzan , Joseph Eli Subotnik

Spectroscopic stimulated Raman scattering (SRS) imaging has become a useful tool finding a broad range of applications. Yet, wider adoption is hindered by the bulky and environmentally-sensitive solid-state optical parametric oscillator…

Optics · Physics 2021-08-20 Hongli Ni , Peng Lin , Yifan Zhu , Meng Zhang , Yuying Tan , Yuewei Zhan , Ji-Xin Cheng

We report on ultrafast optical experiments in which femtosecond mid-infrared radiation is used to excite the lattice of complex oxide heterostructures. By tuning the excitation energy to a vibrational mode of the substrate, a long-lived…

A seemingly anomalous enhancement of electron mobility in strained silicon inversion layers at high sheet densities has exposed a conspicuous gap between device physics theory and experiment in recent years. We show that the root of this…

Mesoscale and Nanoscale Physics · Physics 2015-06-04 Chris Bowen , Ryan Hatcher

We investigate nanoscale local anodic oxidation (LAO) on hydrogen-intercalated graphene grown by controlled sublimation of silicon carbide (SiC). Scanning probe microscopy (SPM) was used as a lithographic and characterization tool in order…

We report an experimental and numerical study of femtosecond multi-pulse laser-induced densification in vitreous silica (v-SiO2) and its signature in Raman spectra. We compare the experimental findings to recently developed molecular…

Disordered Systems and Neural Networks · Physics 2018-02-21 N. S. Shcheblanov , M. E. Povarnitsyn , K. N. Mishchik , A. Tanguy

Electroactive polymer thin films undergo repeated reversible structural change during operation in electrochemical applications. While synchrotron X-ray scattering is powerful for the characterization of stand-alone and ex-situ organic thin…

The evolution of the atomic structure of LaAlO3 grown on SrTiO3 was investigated using surface x-ray diffraction in conjunction with model-independent, phase-retrieval algorithms between two and five monolayers film thickness. A…

The two-loop temperature hysteresis of integrated intensity of Raman scattering of light is explained theoretically for a line of frequency 50 cm-1 in a superconducting oxide Ba1-xKxBiO3 single crystal.

Materials Science · Physics 2009-11-10 A. P. Saiko , S. A. Markevich

Accurate measurements of the dependence of low-frequency Raman scattering on the scattering angle were performed in two silica glasses. By a comparison of spectra measured at a large scattering angle (close to back scattering) and a small…

Soft Condensed Matter · Physics 2009-10-31 N. V. Surovtsev , J. Wiedersich , V. N. Novikov , E. R"ossler , E. Duval

Raman spectroscopy is a powerful technique to characterize materials. It probes non-destructively chemical composition, crystallinity, defects, strain and coupling phenomena. However, the Raman response of surfaces or thin films is often…

Under homogeneous uniaxial strains, the Raman 2D band of graphene involving two-phonon double-resonance scattering processes splits into two peaks and they altogether redshift strongly depending on the direction and magnitude of the strain.…

Mesoscale and Nanoscale Physics · Physics 2015-03-19 Duhee Yoon , Young-Woo Son , Hyeonsik Cheong

We have investigated the interlayer shear and breathing phonon modes in MoS$_{2}$ with pure 3R and 2H stacking order by using polarization-dependent ultralow-frequency Raman spectroscopy. We observe up to three shear branches and four…

Mesoscale and Nanoscale Physics · Physics 2019-02-01 Jeremiah van Baren , Gaihua Ye , Jia-An Yan , Zhipeng Ye , Pouyan Rezaie , Peng Yu , Zheng Liu , Rui He , Chun Hung Lui

To better understand the electronic and chemical properties of wide-gap oxide surfaces at the atomic scale, experimental work has focused on epitaxial films on metal substrates. Recent findings show that these films are considerably thinner…

Materials Science · Physics 2007-08-21 Christoph Freysoldt , Patrick Rinke , Matthias Scheffler

Raman scattering (RS) spectra and current-voltage characteristics at room temperature were measured in six series of small samples fabricated by means of electron-beam lithography on the surface of a large size (5x5 mm) industrial monolayer…

Mesoscale and Nanoscale Physics · Physics 2015-01-13 I. Shlimak , A. Haran , E. Zion , T. Havdala , Yu. Kaganovskii , A. V. Butenko , L. Wolfson , V. Richter , D. Naveh , A. Sharoni , E. Kogan , M. Kaveh

Raman spectroscopy is frequently used to identify composition, structure and layer thickness of 2D materials. Here, we describe an efficient first-principles workflow for calculating resonant first-order Raman spectra of solids within…

Materials Science · Physics 2020-07-15 A. Taghizadeh , U. Leffers , T. G. Pedersen , K. S. Thygesen

Epitaxial BiFeO3/SrRuO3 superlattices have been grown by pulsed laser deposition on a (001) oriented LaAlO3 substrate and probed by X-ray diffraction and Raman spectroscopy. To investigate the structural competition between rhombohedral…

Materials Science · Physics 2021-07-09 S. Yousfi , M. El Marssi , H. Bouyanfif

Polarized Raman scattering and infrared reflection spectra of hexagonal HoMnO$_3$ single crystals in the temperature range 10-300 K are reported. Group-theoretical analysis is performed and scattering selection rules for the second order…

Strongly Correlated Electrons · Physics 2009-11-10 A. P. Litvinchuk , M. N. Iliev , V. N. Popov , M. M. Gospodinov

Raman spectroscopy measurements have been performed on alpha-, beta-, gamma-NaxCoO2 phases differing in their stacking of CoO6 octahedra along the c-axis direction. The results demonstrate that, in general, there are five active phonons for…

Superconductivity · Physics 2009-11-11 H. X. Yang , Y. Xia , Y. G. Shi , H. F. Tian , R. J. Xiao , X. Liu , Y. L. Liu , J. Q. Li

The Raman effect -- inelastic scattering of light by lattice vibrations (phonons) -- produces an optical response closely tied to a material's crystal structure. Here we show that resonant optical excitation of IR and Raman phonons gives…

Materials Science · Physics 2021-07-07 Guru Khalsa , Nicole A. Benedek , Jeffrey Moses