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Quantum sensors based on individual spins provide unprecedented access to local magnetic fields in condensed matter, chemistry, and biology, with solid-state defect spins emerging as the leading platform. However, their molecular-sensing…

The nuclear spin, being much more isolated from the environment than its electronic counterpart, enables quantum experiments with prolonged coherence times and presents a gateway towards uncovering the intricate dynamics within an atom.…

Mesoscale and Nanoscale Physics · Physics 2023-09-08 Lukas M. Veldman , Evert W. Stolte , Mark P. Canavan , Rik Broekhoven , Philip Willke , Laëtitia Farinacci , Sander Otte

Spin injection and detection in silicon is a difficult problem, in part because the weak spin-orbit coupling and indirect gap preclude using standard optical techniques. We propose two ways to overcome this difficulty, and illustrate their…

Other Condensed Matter · Physics 2015-06-24 Igor Zutic , Jaroslav Fabian , Steven C. Erwin

The ability to manipulate electron spins with voltage-dependent electric fields is key to the operation of quantum spintronics devices, such as spin-based semiconductor qubits. A natural approach to electrical spin control exploits the…

A device enabling mechanically-controlled spin and electric transport in mesoscopic structures is proposed. It is based on the transfer of electrons through weak links formed by suspended nanowires, on which the charge carriers experience a…

Mesoscale and Nanoscale Physics · Physics 2014-07-09 R. I. Shekhter , O. Entin-Wohlman , A. Aharony

Carrier spins in semiconductor nanocrystals are promising candidates for quantum information processing. Using a combination of time-resolved Faraday rotation and photoluminescence spectroscopies, we demonstrate optical spin polarization…

Optically addressable spins are actively investigated in quantum communication, processing and sensing. Optical and spin coherence lifetimes, which determine quantum operation fidelity and storage time, are often limited by spin-spin…

Control over quantum systems is typically achieved by time-dependent electric or magnetic fields. Alternatively, electronic spins can be controlled by spin-polarized currents. Here we demonstrate coherent driving of a single spin by a…

Mesoscale and Nanoscale Physics · Physics 2024-06-26 Stepan Kovarik , Richard Schlitz , Aishwarya Vishwakarma , Dominic Ruckert , Pietro Gambardella , Sebastian Stepanow

This chapter describes the relationship between low frequency noise and coherence decay of localized spins in semiconductors. Section 2 establishes a direct relationship between an arbitrary noise spectral function and spin coherence as…

Mesoscale and Nanoscale Physics · Physics 2009-09-05 Rogerio de Sousa

We show that the accumulation of spin-polarized electrons at a forward-biased Schottky tunnel barrier between Fe and n-GaAs can be detected electrically. The spin accumulation leads to an additional voltage drop across the barrier that is…

Materials Science · Physics 2009-11-11 X. Lou , C. Adelmann , M. Furis , S. A. Crooker , C. J. Palmstrom , P. A. Crowell

We present a theory of the imprinting of the electron spin coherence and population in an n-doped semiconductor which forms a junction with a ferromagnet. The reflection of non-equilibrium semiconductor electrons at the interface provides a…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 C. Ciuti , J. P. McGuire , L. J. Sham

The tunability and spatial precision of paramagnetic molecules makes them attractive for quantum sensing. However, usual microwave-based detection methods have poor temporal and spatial resolution, and optical methods compatible with…

Quantum Physics · Physics 2024-07-30 Erica Sutcliffe , Nathanael P. Kazmierczak , Ryan G. Hadt

We investigate quantum coherence of electron spin transported through a semiconductor spintronic device, where spins are envisaged to be controlled by electrical means via spin-orbit interactions. To quantify the degree of spin coherence,…

Mesoscale and Nanoscale Physics · Physics 2017-08-23 Branislav K. Nikolic , Satofumi Souma

Spin is an intrinsically quantum property, characterized by angular momentum. A change in the spin state is equivalent to a change in the angular momentum or mechanical torque. This spin-induced torque has been invoked as the intrinsic…

Mesoscale and Nanoscale Physics · Physics 2009-09-30 Guiti Zolfagharkhani , Alexei Gaidarzhy , Pascal Degiovanni , Stefan Kettemann , Peter Fulde , Pritiraj Mohanty

Molecular spins are a versatile platform for quantum sensing. Not only are the spin-bearing molecules themselves widely tunable, they are also capable of being used as sensors as crystals, films and in solution. Using thin-films offers the…

Materials Science · Physics 2026-01-21 Adrian Mena , Nicholas P. Sloane , Max R. Bonengel , Dane R. McCamey

We find that detuning an optical pulse train from electronic transitions in quantum dots controls the direction of nuclear spin flips. The optical pulse train generates electron spins that precess about an applied magnetic field, with a…

Quantum Physics · Physics 2015-05-13 S. G. Carter , A. Shabaev , Sophia E. Economou , T. A. Kennedy , A. S. Bracker , T. L. Reinecke

The generation of an out-of-equilibrium population of spin-polarized carriers is a keystone process for quantum technologies and spintronics alike. It can be achieved through the so-called optical spin orientation by exciting the material…

The angular momentum of evanescent light fields has been studied in nano-optics and plasmonics, but not in the microwave regime. Here we predict non-contact pumping of electron spin currents in conductors by the evanescent stray fields of…

Mesoscale and Nanoscale Physics · Physics 2020-07-29 Tao Yu , Gerrit E. W. Bauer

Molecular nanomagnets show clear signatures of coherent behavior and have a wide variety of effective low-energy spin Hamiltonians suitable for encoding qubits and implementing spin-based quantum information processing. At the nanoscale,…

Mesoscale and Nanoscale Physics · Physics 2013-05-29 Mircea Trif , Filippo Troiani , Dimitrije Stepanenko , Daniel Loss

The photon spin is an important resource for quantum information processing as is the electron spin in spintronics. However, for subwavelength confined optical excitations, polarization as a global property of a mode cannot be defined.…

Optics · Physics 2018-12-11 Enno Krauss , Gary Razinskas , Dominik Köck , Swen Grossmann , Bert Hecht