English
Related papers

Related papers: Ordered Array of Single Adatoms with Remarkable Th…

200 papers

Density functional molecular dynamics simulations have been carried out to understand the finite temperature behavior of Au$_{19}$ and Au$_{20}$ clusters. Au$_{20}$ has been reported to be a unique molecule having tetrahedral geometry, a…

Statistical Mechanics · Physics 2016-09-28 Sailaja Krishnamurty , Ghazal Shafai , D. G. Kanhere , B. Soulé de Bas , M. J. Ford

Sodium, magnesium and aluminum adatoms, which, respectively, possess one, two and three valence electrons in terms of 3s, $3s^2$, and ($3s^2$, 3p) orbitals, are very suitable for helping us understand the adsorption-induced diverse…

Materials Science · Physics 2020-03-06 Ngoc Thanh Thuy Tran , Godfrey Gumbs , Duy Khanh Nguyen , Ming-Fa Lin

We report the magnetization, ac susceptibility, and specific heat of optically float-zoned single crystals of CePdAl$_{3}$. In comparison to the properties of polycrystalline CePdAl$_{3}$ reported in the literature, which displays a…

Using ab initio thermodynamics we compile a phase diagram for the surface of Fe3O4(001) as a function of temperature and oxygen pressures. A hitherto ignored polar termination with octahedral iron and oxygen forming a wave-like structure…

Materials Science · Physics 2009-11-11 R. Pentcheva , F. Wendler , H. L. Meyerheim , W. Moritz , N. Jedrecy , M. Scheffler

This work reports the successful formation of Ag and Au nanoparticles in $\beta$-Ga$_2$O$_3$ single-crystals by ion implantation and annealing at 550 {\deg}C. X-ray diffraction measurements revealed that nanoparticles were formed after the…

Low energy electron diffraction (LEED), scanning tunneling microscopy (STM), and photoelectron spectroscopy have been used to study an ordered structure formed by Ge atoms deposited onto the Au(111) surface. Based on a careful analysis of…

Materials Science · Physics 2018-01-03 W. Wang , R. I. G. Uhrberg

The adsorption of atomic oxygen and its inclusion into subsurface sites on Ag(210) and Ag(410) surfaces have been investigated using density functional theory. We find that--in the absence of adatoms on the first metal layer--subsurface…

Condensed Matter · Physics 2009-11-10 A. Kokalj , N. Bonini , A. Dal Corso , S. de Gironcoli , S. Baroni

Measurements of electrical resistivity ($\rho$), DC magnetization ($M$) and specific heat ($C$) have been performed on layered oxide Li$_x$CoO$_2$ (0.25$\leq$$x$$\leq$0.99) using single crystal specimens. The $\rho$ versus temperature ($T$)…

Strongly Correlated Electrons · Physics 2015-05-19 K. Miyoshi , C. Iwai , H. Kondo , M. Miura , S. Nishigori , J. Takeuchi

Unique electronic properties of self-organized Au atom chains on Ge(001) in novel c(8x2) long-range order are revealed by scanning tunneling microscopy. Along the nanowires an exceptionally narrow conduction path exists which is virtually…

Strongly Correlated Electrons · Physics 2009-11-13 J. Schaefer , C. Blumenstein , S. Meyer , M. Wisniewski , R. Claessen

Extensive first principles calculations are carried out to investigate gold-promoted TiO2(110) surfaces in terms of structure optimizations, electronic structure analyses, ab initio thermodynamics calculations of surface phase diagrams, and…

Materials Science · Physics 2015-05-28 Matteo Farnesi Camellone , Piotr M. Kowalski , Dominik Marx

The stability, electronic and magnetic properties of Fe atoms adsorbed on the self-assembled Bi-dimer lines nanostructure on the H/Si(001) surface are addressed by spin-density functional calculations. Our results show that Fe adatoms are…

Materials Science · Physics 2007-05-23 W. Orellana , R. H. Miwa

Gold-silica hybrids are appealing in different fields of applications like catalysis, sensors, drug delivery, and biotechnology. In most cases, the morphology and distribution of the hetero-units play significant roles in their functional…

Materials Science · Physics 2015-03-04 Paromita Kundu , Hamed Heidari , Sara Bals , N. Ravishankar , Gustaaf Van Tendeloo

Iron oxides (FeOx) are among the most common support materials utilized in single atom catalysis. The support is nominally Fe2O3, but strongly reductive treatments are usually applied to activate the as-synthesized catalyst prior to use.…

We present a density-functional theory study addressing the energetics and electronic structure properties of isolated oxygen adatoms at the SrTiO3(001) surface. Together with a surface lattice oxygen atom, the adsorbate is found to form a…

Materials Science · Physics 2015-05-13 Hannes Guhl , Wolfram Miller , Karten Reuter

The one-dimensional reconstruction of Au/Ge(001) was investigated by means of autocorrelation functions from surface x-ray diffraction (SXRD) and scanning tunneling microscopy (STM). Interatomic distances found in the SXRD-Patterson map are…

Strongly Correlated Electrons · Physics 2013-05-30 S. Meyer , T. Umbach , C. Blumenstein , J. Schäfer , R. Claessen , S. Sauer , S. J. Leake , P. R. Willmott , M. Fiedler , F. Bechstedt

We use density functional theory calculations to characterize the early stages of fluorination of silver's (100) and (110) surfaces. In the Ag(100) surface, the hollow site is the most favorable for F adatoms. In the Ag(110) surface, three…

The Earth's crust is known to be depleted of gold, among other slightly heavy noble metals transported by magma from the Earth's mantle to the crust. The bulk silicate Earth (BSE) model also suggests significant depletion of Au in the…

In this manuscript we report helium atom scattering (HAS) measurements of the structure of the first H2O layer on Au(111). The interaction between H2O and Au(111) is believed to be particularly weak and conflicting evidence from several…

The crystalline structure, magnetism, and magnetocaloric effect of a GdCrO$_3$ single crystal grown with the laser-diode-heated floating-zone technique have been studied. The GdCrO$_3$ single crystal crystallizes into an orthorhombic…

Strongly Correlated Electrons · Physics 2020-10-27 Yinghao Zhu , Pengfei Zhou , Tao Li , Junchao Xia , Si Wu , Ying Fu , Kaitong Sun , Qian Zhao , Zhen Li , Zikang Tang , Yinguo Xiao , Zhenqiang Chen , Hai-Feng Li

The adsorption of rare gases on metal surfaces serve as the paradigm of weak adsorption where it is typically assumed that the adsorbate occupies maximally coordinated hollow sites. Density-functional theory calculations using the…

Materials Science · Physics 2009-11-07 Juarez L. F. Da Silva , Catherine Stampfl , Matthias Scheffler