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We extensively investigated the critical behavior of mixtures of colloids and polymers via the two-component Asakura-Oosawa model and its reduction to a one-component colloidal fluid using accurate theoretical and simulation techniques. In…

Soft Condensed Matter · Physics 2009-11-11 F. Lo Verso , R. L. C. Vink , D. Pini , L. Reatto

We investigate the influence of confinement on phase separation in colloid-polymer mixtures. To describe the particle interactions, the colloid-polymer model of Asakura and Oosawa [J. Chem. Phys. 22, 1255 (1954)] is used. Grand canonical…

Soft Condensed Matter · Physics 2007-05-23 R. L. C. Vink , K. Binder , J. Horbach

An extension of the Asakura-Oosawa-Vrij model of hard sphere colloids and non-adsorbing polymers, that takes polymer non-ideality into account through a repulsive stepfunction pair potential between polymers, is studied with grand canonical…

Soft Condensed Matter · Physics 2007-05-23 R. L. C. Vink , M. Schmidt

Interfacial properties of colloid--polymer mixtures are examined within an effective one--component representation, where the polymer degrees of freedom are traced out, leaving a fluid of colloidal particles interacting via polymer--induced…

Soft Condensed Matter · Physics 2007-05-23 A. Moncho-Jorda' , J. Dzubiella , J. P. Hansen , A. A. Louis

The influence of confinement, due to flat parallel structureless walls, on phase separation in colloid-polymer mixtures, is investigated by means of grand-canonical Monte Carlo simulations. Ultra-thin films, with thicknesses between…

Soft Condensed Matter · Physics 2009-11-11 Richard L. C. Vink , Andres De Virgiliis , Juergen Horbach , Kurt Binder

We propose a new coarse-grained model for the description of liquid-vapor phase separation of colloid-polymer mixtures. The hard-sphere repulsion between colloids and between colloids and polymers, which is used in the well-known…

Soft Condensed Matter · Physics 2009-11-13 Jochen Zausch , Peter Virnau , Kurt Binder , Juergen Horbach , Richard L. Vink

The possibility to induce demixing in a colloidal mixture by adding small polymers, or other equivalent depletant agents, is theoretically investigated. By use of Mean Field Theory, suitably generalized to deal with short range effective…

Soft Condensed Matter · Physics 2015-10-28 Alberto Parola , Luciano Reatto

The equilibrium phase behavior of a binary mixture of charged colloids and neutral, non-adsorbing polymers is studied within free-volume theory. A model mixture of charged hard-sphere macroions and ideal, coarse-grained, effective-sphere…

Soft Condensed Matter · Physics 2009-11-11 Alan R. Denton , Matthias Schmidt

Colloidal suspensions with free polymer coils which are larger than the colloidal particles are considered. The polymer-colloid interaction is modeled by an extension of the Asakura-Oosawa model. Phase separation occurs into dilute and…

Soft Condensed Matter · Physics 2009-10-31 Richard P. Sear

The relevance of neglecting three- and four-body interactions in the coarse-grained version of the Asakura-Oosawa model is examined. A mapping between the first few virial coefficients of the binary nonadditive hard-sphere mixture…

Soft Condensed Matter · Physics 2016-08-08 Andrés Santos , Mariano López de Haro , Giacomo Fiumara , Franz Saija

We study numerically the critical behavior of a modified, active Asakura-Oosawa model for colloid-polymer mixtures. The colloids are modeled as self-propelled particles with Vicsek-like interactions. This system undergoes phase separation…

Soft Condensed Matter · Physics 2017-03-08 Benjamin Trefz , Jonathan Tammo Siebert , Thomas Speck , Kurt Binder , Peter Virnau

We use a microscopic density functional theory based on Wertheim's first order thermodynamic perturbation theory to study wetting behavior of athermal mixtures of colloids and excluded-volume polymers. In opposition to the wetting behavior…

Soft Condensed Matter · Physics 2007-05-23 Pawel Bryk

We present further evidence that gelation is an arrested phase separation in attractive colloid-polymer mixtures, based on a method combining confocal microscopy experiments with numerical simulations recently established in {\bf Nature…

Soft Condensed Matter · Physics 2009-11-13 Emanuela Zaccarelli , Peter J. Lu , Fabio Ciulla , David. A. Weitz , Francesco Sciortino

We investigate the structure of colloid-polymer mixtures by calculating the structure factors for the Asakura-Oosawa model in the PY approximation. We discuss the role of potential range, polymer concentration and polymer-polymer…

Soft Condensed Matter · Physics 2009-10-31 A. A. Louis , R. Finken , J-P. Hansen

The Asakura-Oosawa model for colloid-polymer mixtures is studied by Monte Carlo simulations at densities inside the two-phase coexistence region of fluid and solid. Choosing a geometry where the system is confined between two flat walls,…

Soft Condensed Matter · Physics 2015-06-04 Debabrata Deb , Alexander Winkler , Peter Virnau , Kurt Binder

The surface tension of interacting polymers in a good solvent is calculated theoretically and by computer simulations for a planar wall geometry and for the insertion of a single colloidal hard-sphere. This is achieved for the planar wall…

Soft Condensed Matter · Physics 2016-08-31 A. A. Louis , P. G. Bolhuis , E. J. Meijer , J. P. Hansen

As a generic model for liquid-vapour type transitions in random porous media, the Asakura-Oosawa model for colloid-polymer mixtures is studied in a matrix of quenched spheres using extensive Monte Carlo (MC) simulations. Since such systems…

Soft Condensed Matter · Physics 2009-11-13 R. L. C. Vink , K. Binder , H. Loewen

Phase separation of colloid-polymer mixtures, described by the Asakura-Oosawa (AO) model, confined in a thin slit pore is studied by grand-canonical Monte Carlo simulation. While one wall is a hard wall for both particles, at the other wall…

Soft Condensed Matter · Physics 2007-05-23 A. De Virgiliis , R. L. C. Vink , J. Horbach , K. Binder

As a model for a suspension of hard-sphere like colloidal particles where small nonadsorbing dissolved polymers create a depletion attraction, we introduce an effective colloid-colloid potential closely related to the Asakura-Oosawa model…

Soft Condensed Matter · Physics 2015-10-28 Antonia Statt , Peter Virnau , Kurt Binder

We study theoretically the equilibrium phase behaviour of a mixture of polydisperse hard-sphere colloids and monodisperse polymers, modelled using the Asakura-Oosawa model within the free volume approximation of Lekkerkerker et al. We…

Soft Condensed Matter · Physics 2009-11-10 M. Fasolo , P. Sollich
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