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Polymer nanoparticle composites (PNC) with ultra high loading of nanoparticles (> 50%) have been shown to exhibit markedly improved strength, stiffness, and toughness simultaneously compared to the neat systems of their components. Recent…

Soft Condensed Matter · Physics 2020-07-01 Emily Y. Lin , Amalie L. Frischknecht , Robert A. Riggleman

We study the influence of spherical, triangular, and rod-like nanoparticles on the mechanical properties of a polymer nanocomposite (PNC), via coarse-grained molecular dynamics simulations. We focus on how the nanoparticle size, loading,…

Soft Condensed Matter · Physics 2012-12-19 Aki Kutvonen , Giulia Rossi , Sakari R. Puisto , Niko K. J. Rostedt , Tapio Ala-Nissila

This paper presents a study of the polymer-filler interfacial effects on filler dispersion and mechanical reinforcement in Polystyrene (PS) / silica nanocomposites by direct comparison of two model systems: un-grafted and PS-grafted silica…

Soft Condensed Matter · Physics 2011-07-12 Chloé Chevigny , Nicolas Jouault , Florent Dalmas , François Boué , Jacques Jestin

While recent efforts have shown how local structure plays an essential role in the dynamic heterogeneity of homogeneous glass-forming materials, systems containing interfaces such as thin films or composite materials remain poorly…

Soft Condensed Matter · Physics 2022-04-27 Entao Yang , James F. Pressly , Bharath Natarajan , Robert Colby , Karen I. Winey , Robert A. Riggleman

A large body of experimental work on the microstructure and dynamics of simplifiedindustrial nanocomposites made of disordered silica filler in a styrene-butadiene matrixby solid-phase mixing is regrouped and critically discussed in this…

Soft Condensed Matter · Physics 2018-11-21 Anne-Caroline Genix , Guilhem P. Baeza , Julian Oberdisse

Fundamental understanding of macroscopic properties of polymer nanocomposites (PNCs) remains difficult due to the complex interplay of microscopic dynamics and structure, namely interfacial layer relaxations and three-dimensional…

The recent development of nanoscale fillers, such as carbon nanotube, graphene, and nanocellulose, allows the functionality of polymer nanocomposites to be controlled and enhanced. However, conventional synthesis methods of polymer…

Short-fiber-reinforced polymer composites are increasingly used in engineering applications and industrial products owing to their unique combination of superior mechanical properties, and relatively easy and low cost manufacturing process.…

Applied Physics · Physics 2017-04-25 Behrouz Arash , Harold S. Park , Timon Rabczuk

Polymers at the interface exhibit frustrated chain conformation distinct from the bulk, impacting particle dispersion and properties of polymer nanocomposites (PNCs). Utilizing bimodal molecular weight (MW) PNCs, we observed unusual chain…

Soft Condensed Matter · Physics 2025-01-14 Tae Yeon Kong , So Youn Kim

Over the past two decades polymer nanocomposites have received tremendous interest from industry and academia due to their advanced properties comparative to polymer blends. Many computational studies have revealed that the macroscopic…

Materials Science · Physics 2015-04-07 Argyrios Karatrantos

Nanoparticles can greatly enhance the mechanical response of elastomeric polymers essential to a wide range of applications, yet their precise molecular mechanisms of high-strain reinforcement remain largely unresolved. Here we show, based…

Soft Condensed Matter · Physics 2025-01-15 Pierre Kawak , Harshad Bhapkar , David S. Simmons

We use molecular dynamics simulations to study a semidilute, unentangled polymer solution containing well dispersed, weakly attractive nanoparticles (NP) of size ($\sigma_N$) smaller than the polymer radius of gyration $R_g$. We find that…

Soft Condensed Matter · Physics 2018-09-18 Valerio Sorichetti , Virginie Hugouvieux , Walter Kob

Polymer composites were manufactured using biocarbon particles as a reinforcing filler to improve the mechanical and thermal properties. However, a detailed examination of dispersion and agglomeration of filler is essential to correlate the…

Applied Physics · Physics 2021-06-10 J. George , D. Bhattacharyya

A study of the reinforcement effect of a soft polymer matrix by hard nanometric filler particles is presented. In the main part of this article, the structure of the silica filler in the matrix is studied by Small Angle Neutron Scattering…

Soft Condensed Matter · Physics 2007-05-23 Julian Oberdisse , Abdeslam El Harrak , Geraldine Carrot , Jacques Jestin , Francois Boue

In this work, a coarse-grained (CG) model of carbon nanotube (CNT) reinforced polymer matrix composites is developed. A distinguishing feature of the CG model is the ability to capture interactions between polymer chains and nanotubes. The…

Applied Physics · Physics 2017-04-25 Behrouz Arash , Harold S. Park , Timon Rabczuk

Molecular dynamics simulation methods are used to study the folding of polymer chains into packed cubic states. The polymer model, based on a chain of linked sites moving in the continuum, includes both excluded volume and torsional…

Soft Condensed Matter · Physics 2009-11-10 D. C. Rapaport

This chapter deals with the fundamental properties of polymer nanocomposites (PNC) and their characteristics that play a significant role in deciding their capability for the advanced energy storage device. The various synthesization…

Materials Science · Physics 2018-07-11 Anil Arya , A. L. Sharma

The conformational and dynamical properties of active Brownian polymers embedded in a fluid depend on the nature of the driving mechanism, e.g., self-propulsion or external actuation of the monomers. Implementations of self-propelled and…

Soft Condensed Matter · Physics 2022-01-24 Judit Clopés Llahí , Aitor Martín-Gómez , Gerhard Gompper , Roland G. Winkler

Short fiber reinforced polymer composites have found extensive industrial and engineering applications owing to their unique combination of low cost, relatively easy processing and superior mechanical properties compared to their parent…

Computational Physics · Physics 2017-04-06 Atiyeh Alsadat Mousavi , Behrouz Arash , Xiaoying Zhuang , Timon Rabczuk

Thermal conduction in polymer nanocomposites depends on several parameters including the thermal conductivity and geometrical features of the nanoparticles, the particle loading, their degree of dispersion and formation of a percolating…

Applied Physics · Physics 2021-01-25 Alessandro di Pierro , Alberto Fina
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