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We report theoretical calculations of high-order harmonic generation (HHG) of Xe with the inclusion of multi-electron effects and macroscopic propagation of the fundamental and harmonic fields in an ionizing medium. By using the…

Atomic Physics · Physics 2011-10-11 Cheng Jin , Anh-Thu Le , Carlos A. Trallero-Herrero , C. D. Lin

The irradiation of atoms by a strong IR laser field of frequency $\omega$ results in the emission of odd-harmonics of $\omega$ ("IR harmonics") up to some maximal cut-off frequency. The addition of an XUV field of frequency…

Atomic Physics · Physics 2008-02-04 Avner Fleischer , Nimrod Moiseyev

High-harmonic generation (HHG) is a highly nonlinear optical process that typically requires an intense laser to trigger emissions at integer multiples of the driving field frequency. However, the strong fields required for conventional HHG…

Optics · Physics 2025-12-05 Lu Wang , Andrew M. Parks , Adam Thorpe , Graeme Bart , Giulio Vampa , Thomas Brabec

High-harmonic generation (HHG) from solid state offers promising potential for attosecond optics with enhanced efficiency and compact configurations. However, Current implementations face critical limitations imposed by material damage…

Optics · Physics 2025-08-19 Qing-Guo Fan , Kang Lai , Wen-hao Liu , Lin-Wang Wang , Jun-Wei Luo , Zhi Wang

In the past two decades high-harmonic generation (HHG) has become a key process in ultra-fast science due to the extremely short time-structure of the underlying electron dynamics being imprinted in the emitted harmonic light bursts. After…

Atomic Physics · Physics 2012-01-25 Markus C. Kohler , Thomas Pfeifer , Karen Z. Hatsagortsyan , Christoph H. Keitel

The underlying physics behind the molecular harmonic emission in relatively long sin$^2$-like laser pulses is investigated. We numerically solved the full-dimensional electronic time-dependent Schr\"{o}dinger equation beyond the…

Atomic Physics · Physics 2016-09-21 H. Ahmadi , M. Vafaee , A. Maghari

High-harmonic generation (HHG) provides short-wavelength light that is useful for precision spectroscopy and probing ultrafast dynamics. We report efficient, phase-coherent harmonic generation up to 9th-order (333 nm) in chirped…

Here, we study the possibility of selective high-harmonic generation (HHG) based on the concept of charge transfer plasmons (CTP) in bridged nanoparticle assemblies. By choosing plasmonic dimer nanoantenna, as a fundamental member of…

Optics · Physics 2018-01-16 Burak Gerislioglu , Arash Ahmadivand , Nezih Pala

The interaction of a helium atom with intense short 800 nm laser pulse is studied theoretically beyond the single-active-electron approximation. For this purpose, the time-dependent Schr\"odinger equation for the two-electron wave packet…

Atomic and Molecular Clusters · Physics 2017-03-08 Anton N. Artemyev , Lorenz S. Cederbaum , Philipp V. Demekhin

We study intraband high-harmonic generation (HHG) in a crystal driven by quantum light. Previous theoretical studies have developed a framework based on coherent state expansions in terms of P distributions to consider nonclassical driving…

Quantum Physics · Physics 2026-05-08 Rasmus Vesterager Gothelf , Christian Saugbjerg Lange , Lars Bojer Madsen

Characterizing and controlling electronic properties of quantum materials require direct measurements of non-equilibrium electronic band structures over large regions of momentum space. Here, we demonstrate an experimental apparatus for…

We theoretically investigate high-order harmonic generation (HHG) and its ellipticity in gapped graphene, driven by a femtosecond short-pulse laser at various orientation angles, employing the two-band density-matrix equations within the…

Atomic Physics · Physics 2025-05-21 Xinru Song , Xiaoyu Bu , Xiaohui Zhao , Rongxiang Zhang , Shang Wang , Fulong Dong

High-order harmonic generation (HHG) in aligned linear molecules can offer valuable information about strong-field interactions in lower-lying molecular orbitals, but extracting this information is difficult for three-dimensional molecular…

Time- and angle-resolved photoemission spectroscopy has played an important role in revealing the non-equilibrium electronic structures of solid-state materials. The implementation of high harmonic generation to obtain a higher photon…

Strongly Correlated Electrons · Physics 2022-06-29 Takeshi Suzuki , Shik Shin , Kozo Okazaki

We observe a new regime of coherent XUV radiation generation in noble gases induced by femtosecond pulses at very high intensities. This XUV emission has both a reduced divergence and spectral width as compared to high-order harmonic…

We perform a detailed analysis of how high-order harmonic generation (HHG) and above-threshold ionization (ATI) can be controlled by a time-delayed attosecond-pulse train superposed to a strong, near-infrared laser field. In particular we…

Atomic Physics · Physics 2009-11-11 C. Figueira de Morisson Faria , P. Salieres , P. Villain , M. Lewenstein

We perform a Bohmian-trajectory analysis of high-order harmonic generation (HHG), focusing on the fact that typical HHG spectra are best reproduced by the Bohmian trajectory starting at the innermost part of the core [Phys. Rev. A…

Atomic Physics · Physics 2013-12-30 J. Wu , B. B. Augstein , C. Figueira de Morisson Faria

High-harmonic generation (HHG), an extreme nonlinear effect, introduces an unprecedented paradigm to detect emergent quantum phases and electron dynamics inconceivable in the framework of linear and low-order nonlinear processes. As an…

High harmonic generation is a convenient way to obtain extreme ultraviolet light from table-top laser systems and the experimental tools to exploit this simple and powerful light source for time-resolved spectroscopy are being developed by…

Atomic and Molecular Clusters · Physics 2013-12-20 Jakob Grilj , Emily Sistrunk , Markus Koch , Markus Gühr

We studied the high-order harmonic generation (HHG) from 2D solid materials in circularly and bichromatic circularly polarized laser fields numerically by simulating the dynamics of single-active-electron processes in 2D periodic…