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We show that a dimer made of two gold nanospheres exhibits a remarkable efficiency for second-harmonic generation under femtosecond optical excitation. The detectable nonlinear emission for the given particle size and excitation wavelength…

Mesoscale and Nanoscale Physics · Physics 2015-05-30 A. Slablab , L. Le Xuan , M. Zielinski , Y. de Wilde , V. Jacques , D. Chauvat , J. -F. Roch

We develop a quantitative mathematical theory that offers new perspectives on nonlinear harmonic generation in plasmonic structures arising from symmetry breaking. Focusing on second harmonic generation--the most fundamental process and the…

Analysis of PDEs · Mathematics 2026-05-04 Hongyu Liu , Zhi-Qiang Miao , Jingfeng Yao , Chengxun Yuan , Guang-Hui Zheng

Time-varying metamaterials rely on large and fast changes of the linear permittivity. Beyond the linear terms, however, the effect of a non-perturbative modulation of the medium on harmonic generation and the associated nonlinear…

We design and analyze photo-metamaterials with each meta-atom containing both photodiode and light-emitting diode. Illumination of the photodiode by the light-emitting diode gives rise to an additional optical feedback within each unit…

Structuring optical materials on a nanometer scale can lead to artificial effective media, or metamaterials, with strongly altered optical behavior. Metamaterials can provide a wide range of linear optical properties such as negative…

Nonlinear optical frequency conversion, where optical fields interact with a nonlinear medium to generate new frequencies, is a key phenomenon in modern photonic systems. However, a major challenge with these techniques lies in the…

Materials Science · Physics 2024-12-05 Simone Grillo , Elena Cannuccia , Maurizia Palummo , Olivia Pulci , Claudio Attaccalite

Scattering has usually be considered as detrimental for optical focusing or imaging. Recently, more and more research has shown that strongly scattering materials can be utilized to focus coherent light by controlling or shaping the…

Optics · Physics 2017-05-24 Yanqi Qiao , Xianfeng Chen , Yajun Peng , Yuanlin Zheng

We study the properties of a tunable nonlinear metamaterial operating at microwave frequencies. We fabricate the nonlinear metamaterial composed of double split-ring resonators and wires where a varactor diode is introduced into each…

Non-perturbative high-harmonic generation (HHG) has recently been observed in the liquid phase, where it was demonstrated to have a different physical mechanism compared to gas and solid phases of matter. The currently best physical picture…

Monolayer transition metal dichalcogenides, coupled to metal plasmonic nanocavities, have recently emerged as new platforms for strong light-matter interactions. These systems are expected to have nonlinear optical properties that will…

We employ structured light for the second-harmonic generation from subwavelength AlGaAs nanoparticles that support both electric and magnetic multipolar Mie resonances. The vectorial structure of the pump beam allows addressing selectively…

In this Letter, we provide experimental evidence of nonlinear wave propagation in a triangular lattice of repulsive magnets supported by an elastic foundation of thin pillars and we interpret all the individual features of the nonlinear…

Pattern Formation and Solitons · Physics 2021-03-22 Weijian Jiao , Stefano Gonella

We experimentally study the optical second harmonic generation (SHG) from deep subwavelength gold-silver heterodimer and silver-silver and gold-gold homodimers. Our results show that the SHG from the heterodimer is about an order of…

The second-harmonic generation of 150 nm spherical gold nanoparticles is investigated both experimentally and theoretically. We demonstrate that the interference effects between dipolar and octupolar plasmons can be used as a fingerprint to…

A comparative experimental investigation of the dependence of second harmonic generation (SHG) on applied external voltage between the standard nematic liquid crystalline material and an analogue ferromagnetic nematic liquid crystalline…

Soft Condensed Matter · Physics 2019-09-30 Jure Brence , Luka Cmok , Nerea Sebastian , Alenka Mertelj , Darja Lisjak , Irena Drevensek-Olenik

The search for miniaturized components for nonlinear optical processes needs a way to overcome the efficiency loss due to the effective size reduction of the active medium. We investigate here a combination of a nanosized nonlinear…

We apply a rigorous eigenmode analysis to study the electromagnetic properties of linear and weakly nonlinear metamaterials. The nonlinear response can be totally described by the linear eigenmodes when weak nonlinearities are attributed to…

Optics · Physics 2015-06-03 Y. Zeng , D. A. R. Dalvit , J. O'Hara , S. A. Trugman

We show that second harmonic generation can be enhanced by Fano resonant coupling of asymmetric plasmonic metal nanostructures. We develop a theoretical model examining the effects of electromagnetic interaction between two metal…

Second harmonic generation is enhanced at the surface lattice resonance in plasmonic nanoparticle arrays. We carried out a parametric investigation on two-dimensional lattices composed of gold nanobars where the centrosymmetry is broken at…

We use ultrafast laser pulses to experimentally demonstrate that the second-order optical response of bulk single crystals of the topological insulator Bi$_2$Se$_3$ is sensitive to its surface electrons. By performing surface doping…

Materials Science · Physics 2011-02-02 D. Hsieh , J. W. McIver , D. H. Torchinsky , D. R. Gardner , Y. S. Lee , N. Gedik