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In this work, we present a computationally efficient methodology that utilizes a local real-space formulation of the projector augmented wave (PAW) method discretized with a finite-element (FE) basis to enable accurate and large-scale…

Computational Physics · Physics 2025-01-03 Kartick Ramakrishnan , Sambit Das , Phani Motamarri

We present an approach to calculate ballistic phonon transport that combines the atomistic Green's function (AGF) method with ab initio results. For the inter atomic potential we use the harmonic approach. The equilibrium positions of the…

Materials Science · Physics 2011-11-11 M. Bachmann , M. Czerner , S. Edaldati-Boostan , C. Heiliger

We develop nonequilibribrium Green's function based transport theory, which includes effects of nonadiabatic nuclear motion in the calculation of the electric current in molecular junctions. Our approach is based on the separation of slow…

Mesoscale and Nanoscale Physics · Physics 2017-12-20 Vincent F. Kershaw , Daniel S. Kosov

Since any realistic electronic device has some degree of disorder, predicting disorder effects in quantum transport is a critical problem. Here we report the theory of nonequilibrium coherent potential approximation (NECPA) for analyzing…

Mesoscale and Nanoscale Physics · Physics 2015-06-15 Yu Zhu , Lei Liu , Hong Guo

We consider optical spectroscopy of molecular junctions from the quantum transport perspective when radiation field is quantized and optical response of the system is simulated as photon flux. Using exact expressions for photon and…

Mesoscale and Nanoscale Physics · Physics 2016-05-09 Yi Gao , Michael Galperin

Due to their small size and unique properties, single-molecule electronics have long seen research interest from experimentalists and theoreticians alike. From a theoretical standpoint, modeling these systems using electronic structure…

Chemical Physics · Physics 2021-10-04 Andrew M. Sand , Justin T. Malme , Erik P. Hoy

We present an application of a new formalism to treat the quantum transport properties of fully interacting nanoscale junctions. We consider a model single-molecule nanojunction in the presence of two kinds of electron-vibron interactions.…

Mesoscale and Nanoscale Physics · Physics 2013-04-08 H. Ness , L. K. Dash

We report equilibrium and non-equilibrium conductance of terphenyl molecules with different anchoring groups including sulfur and nitrogen atom. The corresponding molecules are terphenyl-dithiols(TPDT) and diamino-terphenyl(DATP). The…

Materials Science · Physics 2015-10-15 Setianto , Th. Niehaus

Electron transport properties in nanostructures can be modeled, for example, by using the semiclassical Wigner formalism or the quantum mechanical Green's functions formalism. We compare the performance and the results of these methods in…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 Paula Havu , Noora Tuomisto , Riikka Vaananen , Martti J. Puska , Risto M. Nieminen

With recent developments in spintronics, it is now possible to envision spin-driven devices with magnets and interconnects that require a new class of transport models using generalized Fermi functions and currents, each with four…

Mesoscale and Nanoscale Physics · Physics 2019-08-27 Kerem Y. Camsari , Samiran Ganguly , Deepanjan Datta , Supriyo Datta

Non-equilibrium Green's functions (NEGF) formalism combined with extended Huckel (EHT) and charging model are used to study electrical conduction through single-molecule junctions. Analyzed molecular complex is composed of asymmetric…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 Kamil Walczak , Sergey Edward Lyshevski

The non-equilibrium Green's function (NEGF) method with B\"uttiker probe scattering self-energies is assessed by comparing its predictions for the thermal boundary resistance with molecular dynamics (MD) simulations. For simplicity, the…

A central open question in chiral-induced spin selectivity (CISS) is whether weak electron-phonon coupling in a helical molecular junction can generate a sizable spin polarization in two-terminal transport without invoking additional strong…

Mesoscale and Nanoscale Physics · Physics 2026-05-19 Vipul Upadhyay , Amikam Levy

We present an approach for self-consistent calculations of the many-body Green function in transition metals. The distinguishing feature of our approach is the use of the one-site approximation and the self-consistent quasiparticle wave…

Strongly Correlated Electrons · Physics 2009-11-07 N. E. Zein , V. P. Antropov

Comprehensive understanding of thermal transport in nanostructured materials needs large scale simulations bridging length scales dictated by different physics related to the wave versus particle nature of phonons. Yet, available…

Mesoscale and Nanoscale Physics · Physics 2020-04-10 Dhritiman Chakraborty , Hossein Karamitaheri , Laura de Sousa Oliveira , Neophytos Neophytou

We theoretically study the electronic transport in the monolayer of dithiolated phenylene vinylene oligomeres coupled to the (111) surfaces of gold electrodes. We use non-equilibrium Green functions (NEGF) and density functional theory(DFT)…

Materials Science · Physics 2009-11-10 Z. Crljen , A. Grigoriev , G. Wendin , K. Stokbro

An efficient and compact approach to the inclusion of dissipative effects in Non-Equilibrium Green's Function (NEGF) simulations of electronic systems is introduced. The algorithm is based on two well known methods in the literature,…

Mesoscale and Nanoscale Physics · Physics 2018-03-07 Jesse A. Vaitkus , Jared H. Cole

Stochastic and mixed stochastic-deterministic density functional theory (DFT) are promising new approaches for the calculation of the equation-of-state and transport properties in materials under extreme conditions. In the intermediate warm…

Computational Physics · Physics 2023-09-27 Vidushi Sharma , Lee A. Collins , Alexander J. White

The dynamics of strongly correlated fermions following an external excitation reveals extremely rich collective quantum effects. Examples are fermionic atoms in optical lattices, electrons in correlated materials, and dense quantum plasmas.…

Strongly Correlated Electrons · Physics 2020-02-26 Niclas Schluenzen , Jan-Philip Joost , Michael Bonitz

Development of experimental techniques at nanoscale resulted in ability to perform spectroscopic measurements on single-molecule current carrying junctions. These experiments are natural meeting point for research fields of optical…

Mesoscale and Nanoscale Physics · Physics 2025-02-20 Haoran Sun , Upendra Harbola , Shaul Mukamel , Michael Galperin