Related papers: Decelerating molecules with microwave fields
We demonstrate feedback control optimization for the Stark deceleration and trapping of neutral polar molecules using evolutionary strategies. In a Stark-decelerator beamline pulsed electric fields are used to decelerate OH radicals and…
A continuously operated electrostatic trap for polar molecules is demonstrated. The trap has a volume of ~0.6 cm^3 and holds molecules with a positive Stark shift. With deuterated ammonia from a quadrupole velocity filter, a trap density of…
Using frequency-chirped radiation pressure slowing, we precisely control the velocity of a pulsed CaF molecular beam down to a few m/s, compressing its velocity spread by a factor of 10 while retaining high intensity: at a velocity of…
We demonstrate slowing and longitudinal cooling of a supersonic beam of CaF molecules using counter-propagating laser light resonant with a closed rotational and almost closed vibrational transition. A group of molecules are decelerated by…
Stark deceleration enables the production of cold and dense molecular beams with applications in trapping, collisional studies, and precision measurement. Improving the efficiency of Stark deceleration, and hence the achievable molecular…
We present experimental results that demonstrate - for the first time - the Zeeman deceleration of helium atoms in the metastable 2^3S_1state. A more than 40% decrease of the kinetic energy of the beam is achieved for deceleration from 490…
We show that a magnetically levitated microsphere in high vacuum can be used as an accelerometer by comparing its response to that of a commercially available geophone. This system shows great promise for ultrahigh acceleration…
We present an opto-electrical cooling scheme for polar molecules based on a Sisyphus-type cooling cycle in suitably tailored electric trapping fields. Dissipation is provided by spontaneous vibrational decay in a closed level scheme found…
We present a robust, continuous molecular decelerator that employs high magnetic fields and few optical pumping steps. CaOH molecules are slowed, accumulating at low velocities in a range sufficient for loading both magnetic and…
Using calculations and mathematical modeling, we demonstrate the feasibility of constructing a synchrotron storage ring for neutral polar molecules. The lattice is a racetrack type 3.6 m in circumference consisting of two of 180-degree…
We propose a modified Stark-chirped rapid adiabatic passage technique for a robust rovibrational population transfer in the gas phase molecules in the presence of certain inhomogeneous electric fields. As an example application, the new…
Polar molecules are desirable systems for quantum simulations and cold chemistry. Molecular ions are easily trapped, but a bias electric field applied to polarize them tends to accelerate them out of the trap. We present a general solution…
A general scheme for rotational cooling of diatomic heteronuclear molecules is proposed. It uses a superconducting microwave cavity to enhance the spontaneous decay via Purcell effect. Rotational cooling can be induced by sequentially…
Cold, continuous, high flux beams of benzonitrile, fluorobenzine, and anisole have been created. Buffer-gas cooling with a cryogenic gas provides the cooling and slow forward beam velocities. The beam of benzonitrile was measured to have a…
We measure the response and thermal motion of a high-Q nanomechanical oscillator coupled to a superconducting microwave cavity in the resolved-sideband regime where the oscillator's resonance frequency exceeds the cavity's linewidth. The…
Devices for nano- and molecular size electronics are currently a focus of research aimed at an efficient current rectification and switching. Current switching due to conformational changes in the molecules is slow, on the order of a few…
Intense beams of cold and slow molecules are produced by supersonic expansion out of a rapidly rotating nozzle, as first demonstrated by Gupta and Herschbach. An improved setup is presented that allows to accelerate or decelerate cold…
Internal states of polar molecules can be controlled by microwave-frequency electric dipole transitions. If the applied microwave electric field has a spatial gradient, these transitions also affect the motion of these dipolar particles.…
We present a novel slowing scheme for beams of laser-coolable diatomic molecules reminiscent of Zeeman slowing of atomic beams. The scheme results in efficient compression of the 1-dimensional velocity distribution to velocities trappable…
Polar molecules in selected quantum states can be guided, decelerated, and trapped using electric fields created by microstructured electrodes on a chip. Here we explore how transitions between two of these quantum states can be induced…