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We apply specular and off-specular neutron reflection at the hydrophobic silicon/water interface to check for evidence of nanoscopic air bubbles whose presence is claimed after an ad hoc procedure of solvent exchange. Nanobubbles and/or a…

Soft Condensed Matter · Physics 2017-10-13 Philipp Gutfreund , Marco Maccarini , Andrew Dennison , Max Wolff

Electrolysis of water is employed to produce surface nanobubbles on highly orientated pyrolytic graphite (HOPG) surfaces. Hydrogen (oxygen) nanobubbles are formed when the HOPG surface acts as negative (positive) electrode. Coverage and…

The growth of surface plasmonic microbubbles in binary water/ethanol solutions is experimentally studied. The microbubbles are generated by illuminating a gold nanoparticle array with a continuous wave laser. Plasmonic bubbles exhibit…

Water electrolysis in a microsystem is observed and analyzed on a short-time scale ~10 us. Very unusual properties of the process are stressed. An extremely high current density is observed because the process is not limited by the…

Soft Condensed Matter · Physics 2013-07-18 Vitaly B. Svetovoy , Remco G. P. Sanders , Miko C. Elwenspoek

The existence of surface nanobubbles has been previously suggested using various experimental techniques, including attenuated total reflection spectroscopy, quartz crystal microbalance, neutron reflectometry, and x-ray reflectivity, but…

Formation, evolution, and vanishing of bubbles are common phenomena in our nature, which can be easily observed in boiling or falling waters, carbonated drinks, gas-forming electrochemical reactions, etc. However, the morphology and the…

Spherical-cap-shaped interfacial nanobubbles (NBs) forming on hydrophobic surfaces in aqueous solutions have extensively been studied both from a fundamental point of view and due to their relevance for various practical applications. In…

Fluid Dynamics · Physics 2022-08-18 Yuliang Wang , Xiaolai Li , Shuai Ren , Hadush Tedros Alem , Lijun Yang , Detlef Lohse

The presence of nanobubbles on lubricant-infused surfaces (LIS) has so far been overlooked due to the difficulty in detecting them in such a complex system. We recently showed that anomalously large interfacial slip measured on LIS is…

Soft Condensed Matter · Physics 2021-11-05 Sam Peppou-Chapman , Christopher Vega-Sánchez , Chiara Neto

We use ultra-high-speed video imaging to look at the initial contact of a drop impacting onto a liquid layer. We observe experimentally the vortex street and the bubble-ring entrapments predicted numerically, for high impact velocities, by…

Fluid Dynamics · Physics 2013-05-01 M. -J. Thoraval , K. Takehara , T. G. Etoh , S. T. Thoroddsen

Nanobubbles in liquids are mysterious gaseous objects having exceptional stability. They promise a wide range of applications but their production is not well controlled and localized. Alternating polarity electrolysis of water is a tool…

Soft Condensed Matter · Physics 2017-12-27 Alexander V. Postnikov , Ilia V. Uvarov , Nikita V. Penkov , Vitaly B. Svetovoy

The widespread application of surface-attached nanobubbles and nanodroplets in biomedical engineering and nanotechnology is limited by numerous experimental challenges, in particular, the possibility of contamination in nucleation…

Soft Condensed Matter · Physics 2016-08-30 Hongjie An , Beng Hau Tan , Claus-Dieter Ohl

The bursting of bubbles at an air/liquid interface is a familiar occurrence important to foam stability, cell cultures in bioreactors and mass transfer between the sea and atmosphere. Here we document the hitherto unreported formation and…

Surface nanobubbles are stable gaseous phases in liquids that form on solid substrates. While their existence has been confirmed, there are many open questions related to their formation and dissolution processes along with their structures…

Fluid Dynamics · Physics 2022-04-20 Zhizhao Che , Panagiotis E. Theodorakis

The primary attribute of interest of surface nanobubbles is their unusual stability and a number of theories trying to explain this have been put forward. Interestingly, the dissolution of nanobubbles is a topic that did not receive a lot…

Recent research has revealed several different techniques for nanoscopic gas nucleation on submerged surfaces, with findings seemingly in contradiction with each other. In response to this, we have systematically investigated the occurrence…

We study surface nanobubbles using molecular dynamics simulation of ternary (gas, liquid, solid) systems of Lennard-Jones fluids. They form for sufficiently low gas solubility in the liquid, i.e., for large relative gas concentration. For…

Fluid Dynamics · Physics 2012-11-19 J. H. Weijs , J. H. Snoeijer , D. Lohse

Surface nanobubbles forming on hydrophobic surfaces in water present an exciting opportunity as potential agents of top-down, bottom-up nanopatterning. The formation and characteristics of surface nanobubbles are strongly influenced by the…

Chemical Physics · Physics 2023-09-26 Anayet Ullah Siddique , Rui Xie , Danielle Horlacher , Roseanne Warren

Solvent exchange is a process involving mixing between a good solvent with dissolved solute and a poor solvent. The process creates local oversaturation which causes the nucleation of minute solute droplets. Such ternary systems on a…

Fluid Dynamics · Physics 2022-06-07 You-An Lee , Chao Sun , Sander G. Huisman , Detlef Lohse

In this study, using direct digital and infrared imaging techniques, the freezing of up to three simultaneous THF hydrate droplets was investigated for the first time. Nucleation was initiated at the aqueous solution-air interface. Two…

Applied Physics · Physics 2023-02-24 Adam McElligott , André Guerra , Alexia Denoncourt , Alejandro D. Rey , Phillip Servio

Bubbles may form when imaging liquids with in situ liquid-cell electron microscopy. Fluid dynamics videos show beam-induced bubble nucleation and growth. By examining the bubble formation and growth process, we hope to gain a better…

Fluid Dynamics · Physics 2012-10-15 Joseph M. Grogan , Frances M. Ross , Haim H. Bau
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