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Basis set extrapolations are typically rationalized either from analytical arguments involving the partial-wave or principal expansions of the correlation energy in helium-like systems, or from fitting extrapolation parameters to reference…

Chemical Physics · Physics 2024-09-09 Vladimir Fishman , Emmanouil Semidalas , Jan M. L. Martin

The use of finite harmonic oscillator spaces in many-body calculations introduces both infrared (IR) and ultraviolet (UV) errors. The IR effects are well approximated by imposing a hard-wall boundary condition at a properly identified…

Nuclear Theory · Physics 2014-12-30 S. König , S. K. Bogner , R. J. Furnstahl , S. N. More , T. Papenbrock

An appropriate iterative scheme for the minimization of the energy, based on the variational Monte Carlo (VMC) technique, is introduced and compared with existing stochastic schemes. We test the various methods for the 1D Heisenberg ring…

Strongly Correlated Electrons · Physics 2009-11-11 Sandro Sorella

Electron-molecule collisions play a central role in both natural processes and modern technological applications, particularly in plasma processing. Conventional computational strategies such as the R-matrix method have been widely adopted…

Quantum Physics · Physics 2026-05-13 Dario Picozzi , Jonathan Tennyson , Vincent Graves , Jimena D. Gorfinkiel

Numerical simulations of merging black hole binaries produce the most accurate gravitational waveforms. The availability of hundreds of these numerical relativity (NR) waveforms, often containing many higher spherical harmonic modes, allows…

General Relativity and Quantum Cosmology · Physics 2016-11-24 Chad R. Galley , Patricia Schmidt

In the Projector Augmented Wave (PAW) method, a local potential, basis functions, and projector functions form an All-Electron (AE) basis for valence wave functions in the application of Density Functional Theory (DFT). The construction of…

Materials Science · Physics 2010-08-05 R. J. Snow , A. F. Wright , C. Y. Fong

The Variation Evolving Method (VEM) that originates from the continuous-time dynamics stability theory seeks the optimal solutions with variation evolution principle. After establishing the first and the second evolution equations within…

Systems and Control · Computer Science 2025-01-28 Sheng Zhang , Fei Liao , Kai-Feng He

An eikonal expansion is used to provide systematic corrections to the eikonal approximation through order $1/k^2$, where $k$ is the wave number. Electron wave functions are obtained for the Dirac equation with a Coulomb potential. They are…

Nuclear Theory · Physics 2015-05-13 J. A. Tjon , S. J. Wallace

The Empirical Valence Bond (EVB) method offers a suitable framework to obtain reactive potentials through the coupling of non-reactive force fields. However, most of the implemented functional forms for the coupling terms depend on complex…

Chemical Physics · Physics 2021-01-27 Ivan Scivetti , Kakali Sen , Alin M. Elena , Ilian Todorov

It is proven that the exact excited-state wave function and energy may be obtained by minimizing the energy expectation value of trial wave functions that are constrained only to have the correct nodes of the state of interest. This…

Quantum Physics · Physics 2018-08-24 Federico Zahariev , Mark S. Gordon , Mel Levy

Buildings rarely perform as designed/simulated and and there are numerous tangible benefits if this gap is reconciled. A new scientific yet pragmatic methodology - called Enhanced Parameter Estimation (EPE) - is proposed that allows…

Systems and Control · Electrical Eng. & Systems 2021-03-15 Kris Subbarao , Srijan Didwania , T. Agami Reddy , Marlin Addison

In most nuclear many-body methods, observables are calculated using many-body wave functions explicitly. The variational two-particle reduced density matrix method is one of the few exceptions to the rule. Ground-state energies of both…

Nuclear Theory · Physics 2021-07-07 J. G. Li , N. Michel , W. Zuo , F. R. Xu

Our recent formulation of the analytic and variational Slater-Roothaan (SR) method, which uses Gaussian basis sets to variationally express the molecular orbitals, electron density and the one body effective potential of density functional…

Other Condensed Matter · Physics 2016-08-31 Rajendra R. Zope , Brett I. Dunlap

We propose a high-order spacetime wavelet method for the solution of nonlinear partial differential equations with a user-prescribed accuracy. The technique utilizes wavelet theory with a priori error estimates to discretize the problem in…

Numerical Analysis · Mathematics 2025-01-14 Cody D. Cochran , Karel Matous

This paper deals with the weak error estimates of the exponential Euler method for semi-linear stochastic partial differential equations (SPDEs). A weak error representation formula is first derived for the exponential integrator scheme in…

Numerical Analysis · Mathematics 2015-06-23 Xiaojie Wang

We perform an extrapolative analysis of "fast-growth" free-energy-difference (DF) estimates of a computer-modeled, fully-solvated ethane<->methanol transformation. The results suggest that extrapolation can greatly reduce the systematic…

Chemical Physics · Physics 2007-05-23 Daniel M. Zuckerman , Thomas B. Woolf

While there have been many developments in computational probes of both strongly-correlated molecular systems and machine-learning accelerated molecular dynamics, there remains a significant gap in capabilities in simulating accurate…

Chemical Physics · Physics 2025-04-04 Yannic Rath , George H. Booth

We have performed shell-model calculations starting from the CD-Bonn free nucleon-nucleon NN potential and making use of a new approach for the calculation of the effective interaction. This consists in deriving from the NN potential a…

Nuclear Theory · Physics 2007-05-23 A. Covello , L. Coraggio , A. Gargano , N. Itaco , T. T. S. Kuo

The efficiency of the variational perturbation theory [Phys. Rev. C {\bf 62}, 045503 (2000)] formulated recently for many-particle systems is examined by calculating the ground state correlation energy of the 3D electron gas with the…

Strongly Correlated Electrons · Physics 2009-11-07 Sang Koo You , Noboru Fukushima

We present an improved formalism for quantum Monte Carlo calculations of energy derivatives and properties (e.g. the interatomic forces), with a multideterminant Jastrow-Slater function. As a function of the number $N_e$ of Slater…

Chemical Physics · Physics 2017-06-26 Roland Assaraf , Saverio Moroni , Claudia Filippi