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The temperature-dependent electron spin relaxation of positively charged excitons in a single InAs quantum dot (QD) was measured by time-resolved photoluminescence spectroscopy at zero applied magnetic fields. The experimental results show…

Mesoscale and Nanoscale Physics · Physics 2015-06-03 X. M. Dou , B. Q. Sun , D. S. Jiang , H. Q. Ni , Z. C. Niu

We study theoretically the electron spin noise in quantum dots under non-equilibrium conditions caused by the pumping by a train of circularly polarized optical pulses. In such a situation, the nuclear spins are known to adjust in such a…

Mesoscale and Nanoscale Physics · Physics 2018-08-01 Natalie Jäschke , Frithjof B. Anders , Mikhail M. Glazov

Current-induced electron spin polarization is shown to produce nuclear hyperpolarization through dynamic nuclear polarization. Saturated fields of several millitesla are generated upon the application of electric field over a timescale of a…

Mesoscale and Nanoscale Physics · Physics 2014-10-31 C. J. Trowbridge , B. M. Norman , Y. K. Kato , D. D. Awschalom , V. Sih

We propose a new, more efficient, and potentially cost effective, solid-state nuclear spin hyperpolarization method combining the Cross Effect mechanism and electron spin optical hyperpolarization in rotating solids. We first demonstrate…

Quantum Physics · Physics 2022-01-25 Frederic Mentink-Vigier , Vinayak Rane , Thierry Dubroca , Krishnendu Kundu

We show that by illuminating an InGaAs/GaAs self-assembled quantum dot with circularly polarized light, the nuclei of atoms constituting the dot can be driven into a bistable regime, in which either a threshold-like enhancement or reduction…

We demonstrate dynamical nuclear spin polarization in the absence of an external magnetic field, by resonant circularly polarized optical excitation of a single electron or hole charged quantum dot. Optical pumping of the electron spin…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 C. W. Lai , P. Maletinsky , A. Badolato , A. Imamoglu

The control of nuclear spins in quantum dots is essential to explore their many-body dynamics and exploit their prospects for quantum information processing. We present a unique combination of dynamic nuclear spin polarization and…

Mesoscale and Nanoscale Physics · Physics 2015-12-16 Florian Forster , Max Mühlbacher , Dieter Schuh , Werner Wegscheider , Geza Giedke , Stefan Ludwig

The available theoretical approaches aiming at describing Dynamic Nuclear spin Polarization (DNP) in solutions containing molecules of biomedical interest and paramagnetic centers are not able to model the behaviour observed upon varying…

Statistical Mechanics · Physics 2014-06-06 Sonia Colombo Serra , Marta Filibian , Pietro Carretta , Alberto Rosso , Fabio Tedoldi

Optically addressable molecular triplet spins provide a chemically tunable platform for quantum application, but their coherence is often limited by interactions with surrounding spin baths. Here we demonstrate controlled suppression of…

We have investigated the spin preparation efficiency by optical pumping of individual Mn atoms embedded in CdTe/ZnTe quantum dots. Monitoring the time dependence of the intensity of the fluorescence during the resonant optical pumping…

Mesoscale and Nanoscale Physics · Physics 2012-06-18 C. Le Gall , R. S. Kolodka , C. Cao , H. Boukari , H. Mariette , J. Fernández-Rossier , L. Besombes

The magnetic interactions between the spin of an unpaired electron and the surrounding nuclear spins can be exploited to gain structural information, to reduce nuclear relaxation times as well as to create nuclear hyperpolarization via…

Two electrons in a quantum dot (QD) can form triplet states. We analyze the exchange coupling of the triplet states of the negatively charged exciton in a QD (X$^-$, two electrons and one hole) with the spin of a magnetic atom (Mn). Two…

Mesoscale and Nanoscale Physics · Physics 2023-07-12 L. Besombes , S. Ando , S. Kuroda , H. Boukari

We achieve direct detection of electron hyperfine shifts in individual CdTe/ZnTe quantum dots. For the previously inaccessible regime of strong magnetic fields $B_z\gtrsim0.1$ T, we demonstrate robust polarization of a few-hundred-particle…

Mesoscale and Nanoscale Physics · Physics 2019-03-11 G. Ragunathan , J. Kobak , G. Gillard , W. Pacuski , K. Sobczak , J. Borysiuk , M. S. Skolnick , E. A. Chekhovich

Nuclear quadrupole interaction extends the limits imposed by hyperfine interaction on the spin coherence of the electron and nuclei in a quantum dot. The strain-induced nuclear quadrupole interaction suppresses the nuclear spin flip and…

Mesoscale and Nanoscale Physics · Physics 2008-04-01 R. I. Dzhioev , V. L. Korenev

For applications of solid state quantum computing and quantum simulations, high fidelity initialisation of thermally mixed electronic and nuclear spin qubits is essential. Whereas electronic spins can readily be initialised optically to…

Quantum Physics · Physics 2024-04-12 O. T. Whaites , T. S. Monteiro

The dynamic polarization of nuclear spins by photoexcited electrons is studied in a high quality GaAs/AlGaAs quantum well. We find a surprisingly high efficiency of the spin transfer from the electrons to the nuclei as reflected by a…

Mesoscale and Nanoscale Physics · Physics 2017-11-15 R. W. Mocek , V. L. Korenev , M. Bayer , M. Kotur , R. I. Dzhioev , D. O. Tolmachev , G. Cascio , K. V. Kavokin , D. Suter

We demonstrate a new method of measuring the exciton spin relaxation time in semiconductor nanostructures by continuous-wave photoluminescence. We find that for self-assembled CdTe quantum dots the degree of circular polarization of…

Materials Science · Physics 2009-11-10 S. Mackowski , T. A. Nguyen , H. E. Jackson , L. M. Smith , J. Kossut , G. Karczewski

We study experimentally the dependence of dynamic nuclear spin polarization on the power of non-resonant optical excitation in two types of individual neutral semiconductor quantum dots: InGaAs/GaAs and GaAs/AlGaAs. We show that the…

Mesoscale and Nanoscale Physics · Physics 2013-07-10 J. Puebla , E. A. Chekhovich , M. Hopkinson , P. Senellart , A. Lemaitre , M. S. Skolnick , A. I. Tartakovskii

Tunnel-coupled optically active quantum dot molecules (QDMs), have the potential to operate as spin-photon-interfaces with coupled spins that interact with two different photon frequencies at the same time. A prerequisite is to…

We report polarized photoluminescence excitation spectroscopy of the negative trion in single charge tunable InAs/GaAs quantum dots. The spectrum exhibits a p-shell resonance with polarized fine structure arising from the direct excitation…

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