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Related papers: Dynamics of end to end loop formation for an isola…

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We investigate theoretically the end-to-end looping time of a long chain polymer molecule immersed in a solvent. The dynamics of the end-to-end distance is governed by a Smoluchowski-like equation of a particle moving under the influence of…

Soft Condensed Matter · Physics 2018-03-20 Moumita Ganguly , Aniruddha Chakraborty

This study focuses on comparing the individual polymer chain dynamics in an entangled polymeric liquid under different shear and extension rates. Polymer chains under various shear rates and extension rates were simulated using a…

Chemical Physics · Physics 2021-01-15 Behrouz Behdani , Tong Mou , Cody Spratt , Slava Butcovich , Ryan Gettler , Joontaek Park

The dynamics of loop formation by linear polymer chains has been a topic of several theoretical/experimental studies. Formation of loops and their opening are key processes in many important biological processes. Loop formation in flexible…

Soft Condensed Matter · Physics 2015-05-14 K. P. Santo , K. L. Sebastian

Chemical reactions inside cells are typically subject to the effects both of the cell's confining surfaces and of the viscoelastic behavior of its contents. In this paper, we show how the outcome of one particular reaction of relevance to…

Soft Condensed Matter · Physics 2015-06-04 Pinaki Bhattacharyya , Rati Sharma , Binny J. Cherayil

We investigate the kinetics of loop formation in flexible ideal polymer chains (Rouse model), and polymers in good and poor solvents. We show for the Rouse model, using a modification of the theory of Szabo, Schulten, and Schulten, that the…

Soft Condensed Matter · Physics 2007-11-13 Ngo Minh Toan , Greg Morrison , Changbong Hyeon , D. Thirumalai

We study the dynamical response of a single semiflexible polymer chain based on the theory developed by Hallatschek et al. for the wormlike-chain model. The linear viscoelastic response under oscillatory forces acting at the two chain ends…

Soft Condensed Matter · Physics 2009-11-03 T. Hiraiwa , T. Ohta

We propose and analyze a simple model for the evolution of an immersed, inextensible filament which incorporates linear viscoelastic effects of the surrounding fluid. The model is a closed-form system of equations along the curve only which…

Analysis of PDEs · Mathematics 2024-05-21 Laurel Ohm

We investigate the conformational and dynamical properties of a partially active Rouse chain, where activity is localized within a specific segment, positioned at various locations along the chain and spanning any given length. Through…

Soft Condensed Matter · Physics 2024-12-06 Koushik Goswami , Norman Hsia , Cheng-Hung Chang , Hong-Yan Shih

A theory of diffusion-controlled intramolecular reactions of polymer chain in dilute solution is formulated. Our model is based on the widely used diffusion-reaction formalism of Wilemski and Fixman (J. Chem. Phys. 60, 866 (1974). Our model…

Soft Condensed Matter · Physics 2016-06-02 Aniruddha Chakraborty

We present a theoretical model for understanding the kinetics of a long polymer in solution. A Smoluchowski-like equation has been used to model the problem of polymer looping with a Dirac delta function sink of finite strength. The results…

Statistical Mechanics · Physics 2017-04-25 Moumita Ganguly , Anirudhha Chakraborty

In recent past, experiments and simulations have suggested that apart from the solvent friction, friction arising from the protein itself plays an important role in protein folding by affecting the intra-chain loop formation dynamics. This…

Soft Condensed Matter · Physics 2014-06-25 Nairhita Samanta , Jayanta Ghosh , Rajarshi Chakrabarti

The linear viscoelastic response of single semiflexible polymer chains in the infinite-dilution limit is studied using Brownian dynamics simulations of coarse-grained bead-spring chains. The springs obey the FENE-Fraenkel force law, a…

Soft Condensed Matter · Physics 2026-03-03 Amit Varakhedkar , P. Sunthar , J. Ravi Prakash

We present exact spatio-temporal correlation functions of a Rouse polymer chain submerged in a fluid having planar mixed flow, in the steady state. Using these correlators, determination of the time scale distribution functions associated…

Statistical Mechanics · Physics 2011-09-06 Dipjyoti Das , Sanjib Sabhapandit , Dibyendu Das

We study the dynamics of a polymer that is pulled by a constant force through a viscoelastic medium. This is a model for a polymer being pulled through a cell by an external force, or for an active biopolymer moving due to a self generated…

Soft Condensed Matter · Physics 2015-06-22 Hans Vandebroek , Carlo Vanderzande

The deformation and break-up of Newtonian/viscoelastic droplets are studied in confined shear flow. Our numerical approach is based on a combination of Lattice-Boltzmann models (LBM) and finite difference schemes, the former used to model…

Soft Condensed Matter · Physics 2016-11-15 A. Gupta , M. Sbragaglia

Loop formation between monomers in the interior of semiflexible chains describes elementary events in biomolecular folding and DNA bending. We calculate analytically the interior distance distribution function for semiflexible chains using…

Soft Condensed Matter · Physics 2009-11-11 Changbong Hyeon , D. Thirumalai

We present a Brownian dynamics theory with full hydrodynamics (Stokesian dynamics) for a Gaussian polymer chain embedded in a liquid membrane which is surrounded by bulk solvent and walls. The mobility tensors are derived in Fourier space…

Soft Condensed Matter · Physics 2011-04-04 Sanoop Ramachandran , Shigeyuki Komura , Kazuhiko Seki , Gerhard Gompper

We revisit the celebrated Wilemski-Fixman (WF) treatment for the looping time of a free-draining polymer. The WF theory introduces a sink term into the Fokker-Planck equation for the $3(N+1)$-dimensional Ornstein-Uhlenbeck process of the…

Soft Condensed Matter · Physics 2019-10-29 Felix X. -F. Ye , Panos Stinis , Hong Qian

Recently single molecule experiments have shown the importance of internal friction in biopolymer dynamics. Such studies also suggested that the internal friction although independent of solvent viscosity has strong dependence on denaturant…

Soft Condensed Matter · Physics 2015-06-02 Nairhita Samanta , Rajarshi Chakrabarti

Contrary to some expectations, an experimental finding for a polymer that the solution intrinsic viscosity $[\eta]$ or the melt viscosity is linear in the polymer molecular weight $M$ does not indicate that polymer dynamics are Rouselike.…

Soft Condensed Matter · Physics 2021-05-03 George D. J. Phillies
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