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Related papers: Kapellasite: a kagome quantum spin liquid

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Motivated by recent experiments on the Heisenberg S=1/2 quantum spin liquid candidate material kapellasite, we classify all possible chiral (time-reversal symmetry breaking) spin liquids with fermionic spinons on the kagome lattice. We…

Strongly Correlated Electrons · Physics 2016-02-05 Samuel Bieri , Laura Messio , Bernard Bernu , Claire Lhuillier

We report $^{35}$Cl NMR, ESR, $\mu$SR and specific heat measurements on the $S=1/2$ frustrated kagom\'e magnet kapellasite, $\alpha-$Cu$_3$Zn(OH)$_6$Cl$_2$, where a gapless spin liquid phase is stabilized by a set of competing exchange…

Frustrated magnetism on the kagome lattice has been a fertile ground for rich and fascinating physics, ranging from experimental evidence of a spin liquid to theoretical predictions of exotic superconductivity. Among experimentally realized…

Strongly Correlated Electrons · Physics 2015-12-16 Yasir Iqbal , Harald O. Jeschke , Johannes Reuther , Roser Valentí , I. I. Mazin , Martin Greiter , Ronny Thomale

The recently discovered natural minerals Cu3Zn(OH)6Cl2 and Cu3Mg(OH)6Cl2 are spin 1/2 systems with an ideal kagome geometry. Based on electronic structure calculations, we develop a realistic model which includes couplings across the kagome…

Strongly Correlated Electrons · Physics 2008-09-05 O. Janson , J. Richter , H. Rosner

Geometric frustration of magnetic ions can lead to a quantum spin liquid ground state where long range magnetic order is avoided despite strong exchange interactions. The physical realization of quantum spin liquids comprises a major…

Strongly Correlated Electrons · Physics 2023-06-07 Alex Hallett , Catalina Avarvarei , John W. Harter

A quantum spin liquid (QSL) is an exotic quantum state of matter characterized by fluctuating spins which may exhibit long-range entanglement. Among the possible host candidates for a QSL ground state, the $S$=1/2 kagome lattice…

Based on experimental data and our theoretical analysis, we provide a strategy for unambiguous establishing of gapless quantum spin liquid state (QSL) in herbertsmithite and other materials. To clarify the nature of QSL, we recommend…

Quantum spin liquids form a novel class of matter where, despite the existence of strong exchange interactions, spins do not order down to the lowest measured temperature. Typically, these occur in lattices that act to frustrate the…

Strongly Correlated Electrons · Physics 2016-12-05 M. R. Norman

The study of quantum spin-liquid states (QSL) with lattice dimension $>1$ has proven an enduring problem in solid state physics. Key candidate materials are the $S=\frac{1}{2}$ kagome magnets due to their ability to host quantum…

Materials Science · Physics 2016-10-04 E Connolly , P Reeves , D Boldrin , A S Wills

Low energy inelastic neutron scattering on single crystals of the kagome spin liquid compound ZnCu3(OD)6Cl2 (Herbertsmithite) reveals antiferromagnetic correlations between impurity spins for energy transfers E < 0.8 meV (~J/20). The…

Strongly Correlated Electrons · Physics 2016-08-24 Tian-Heng Han , M. R. Norman , J. -J. Wen , Jose A. Rodriguez-Rivera , Joel S. Helton , Collin Broholm , Young S. Lee

Herbertsmithite, ZnCu3(OH)6Cl2, is the prototype candidate for a spin liquid behavior on a geometrically perfect kagome lattice. Its discovery and the absence of any evidence for spin-freezing down to the lowest probed temperature to-date…

Strongly Correlated Electrons · Physics 2015-05-28 P. Mendels , F. Bert

Recent experiments suggest a quantum spin liquid ground state in the material PbCuTe$_2$O$_6$, where $S=1/2$ moments are coupled by antiferromagnetic Heisenberg interactions into a three dimensional structure of corner sharing triangles…

Strongly Correlated Electrons · Physics 2021-09-15 Li Ern Chern , Yong Baek Kim

The quantum spin liquid (QSL) is a highly entangled magnetic state characterized by the absence of static magnetism in its ground state. Instead, the spins fluctuate in a highly correlated way down to the lowest temperatures. The QSL is…

Motivated by the recent experiments on the new spin half Kagome compound ZnCu3(OH)6Cl2, we study a phenomenological model of a frustrated quantum magnet. The model has a spin liquid groundstate and is constructed so as to mimic the…

Strongly Correlated Electrons · Physics 2009-11-13 R. Chitra , M. J. Rozenberg

The kapellasite family $A$Cu$_3$(OH)$_{6+x}$(Cl,Br)$_{3-x}$ forms a series of compounds, wherein the chemical pressure realized by the $A-$site cation tunes the spin exchange in the frustrated distorted kagome lattice. Via hydrothermal…

Strongly Correlated Electrons · Physics 2025-08-12 Jonas Andreas Krieger , Thomas James Hicken , Hubertus Luetkens , Reinhard K. Kremer , Pascal Puphal

We report muSR experiments on Mg{x}Cu{4-x}(OH)6Cl2 with x \sim 1, a new material isostructural to Herbertsmithite exhibiting regular kagome planes of spin 1/2 (Cu^{2+}), and therefore a candidate for a spin liquid ground state. We evidence…

Strongly Correlated Electrons · Physics 2014-10-06 E. Kermarrec , P. Mendels , F. Bert , R. H. Colman , A. S. Wills , P. Strobel , P. Bonville , A. Hillier , A. Amato

Y-kapellasite (Y$_3$Cu$_9$(OH)$_{19}$Cl$_8$), which hosts an original anisotropic kagome sublattice, is a promising candidate for studying elusive and complex correlated physics. It exhibits a theoretically predicted in-plane $(1/3, 1/3)$…

We report magnetization, electron spin resonance (ESR), and muon spin relaxation ($\mu $SR) measurements on single crystals of the $S=1/2$ (Cu$% ^{+2}$) kagom\'{e} compound Cu(1,3-benzendicarboxylate). The $\mu $SR is carried to…

Strongly Correlated Electrons · Physics 2015-06-18 Oren Ofer , Lital Marcipar , V. Ravi Chandra , Snir Gazit , Daniel Podolsky , Daniel P. Arovas , Amit Keren

The emergent behavior of spin liquids that are born out of geometrical frustration makes them an intriguing state of matter. We show that in the quantum kagome antiferromagnet ZnCu$_3$(OH)$_6$SO$_4$ several different correlated, yet…

Strongly Correlated Electrons · Physics 2016-03-02 M. Gomilsek , M. Klanjsek , M. Pregelj , F. C. Coomer , H. Luetkens , O. Zaharko , T. Fennell , Y. Li , Q. M. Zhang , A. Zorko

A novel cuprate Volborthite, Cu3V2O7(OH)2-2H2O, containing an S-1/2 (Cu 2+ spin) kagome-like lattice is studied by magnetic susceptibility, specific heat, and 51 V NMR measurements. Signs for neither long-range order nor spin-gapped singlet…

Strongly Correlated Electrons · Physics 2009-11-07 Z. Hiroi , M. Hanawa , N. Kobayashi , M. Nohara , H. Takagi , Y. Kato , M. Takigawa
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