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To support efforts on cooling and trapping of alkaline-earth atoms and designs of atomic clocks, we performed ab initio relativistic many-body calculations of electric-dipole transition amplitudes between low-lying states of Mg, Ca, and Sr.…

Atomic Physics · Physics 2009-11-07 S. G. Porsev , M. G. Kozlov , Yu. G. Rakhlina , A. Derevianko

We present electric dipole polarizabilities ($\alpha_d$) of the alkali-metal negative ions, from H$^-$ to Fr$^-$, by employing four-component relativistic many-body methods. Differences in the results are shown by considering Dirac-Coulomb…

Atomic Physics · Physics 2021-01-07 B. K. Sahoo

The development of numerical methods capable of simulating realistic materials with strongly correlated electrons, with controllable errors, is a central challenge in quantum many-body physics. Here we describe how a hybrid between…

Strongly Correlated Electrons · Physics 2015-04-23 Alexei A. Kananenka , Emanuel Gull , Dominika Zgid

The random-phase approximation with exchange (RPAE) is used with a $B$-spline basis to compute dynamic dipole polarizabilities of noble-gas atoms and several other closed-shell atoms (Be, Mg, Ca, Zn, Sr, Cd, and Ba). From these, values of…

Atomic Physics · Physics 2015-07-08 A. R. Swann , J. A. Ludlow , G. F. Gribakin

A QCD model with an infinite number of vector mesons suggested by one of the authors is used to derive the value of the correction $\delta\alpha_{hadr}$ for $\alpha(m_{Z}^{2})$ due to the strong interactions. The result is…

High Energy Physics - Phenomenology · Physics 2009-10-28 B. V. Geshkenbein , V. L. Morgunov

Treating water as a linearly responding dielectric continuum on molecular length scales allows very simple estimates of solvation structure and thermodynamics for charged and polar solutes. While this approach can successfully account for…

Statistical Mechanics · Physics 2021-07-07 Stephen J. Cox , Kranthi K. Mandadapu , Phillip L. Geissler

We review the determination of the QED coupling at the Z pole, which is a crucial parameter for electroweak theory. We include recent e+e- -> hadron data from Novosibirsk and Beijing to re-evaluate alpha (M_Z^2). We find 1/alpha (M_Z^2) =…

High Energy Physics - Phenomenology · Physics 2008-11-26 A. D. Martin , J. Outhwaite , M. G. Ryskin

Electronic structure methods built around double-electron excitations have a rich history in quantum chemistry. However, it seems to be the case that such methods are only suitable in particular situations and are not naturally equipped to…

Chemical Physics · Physics 2024-07-12 Zachary W. Windom , Ajith Perera , Rodney J. Bartlett

Calculating polarizabilities of large clusters with first-principles techniques is challenging because of the unfavorable scaling of computational cost with cluster size. To address this challenge, we demonstrate that polarizabilities of…

Materials Science · Physics 2021-08-26 Mario G. Zauchner , Stefano Dal Forno , Gábor Cśanyi , Andrew Horsfield , Johannes Lischner

We investigate the dynamic second-order hyperpolarizabilities {\gamma}(-3{\omega}; {\omega}, {\omega}, {\omega}) (indicated by {\gamma}THG) of the Si2C and Si3C clusters using the highly accurate coupled cluster singles-and-doubles (CCSD)…

Atomic and Molecular Clusters · Physics 2017-03-21 You-Zhao Lan , Yun-Long Feng

The quadrupole coupling constant $C_{\text{Q}}$ and the asymmetry parameter $\eta$ of the aluminium nuclei in two polymorphs of the complex aluminium hydride CsAlH4 are determined from both $^{27}$Al MAS NMR spectra and $^{27}$Al NMR…

Materials Science · Physics 2024-10-11 Bodo Zibrowius , Michael Fischer

In nanophotonics, multipole framework has become an indispensable theoretical tool for analyzing subwavelength meta-atoms and their radiation properties. This work presents higher-order exact dynamic polarizability (alpha) tensors, which…

Optics · Physics 2020-04-08 Jungho Mun , Sunae So , Jaehyuck Jang , Junsuk Rho

A new approach has been used to explain the experimental data for the $^{12}$C+$^{12}$C system over a wide energy range in the laboratory system from 32.0 MeV to 126.7 MeV. This new coupled-channels based approach involves replacing the…

Nuclear Theory · Physics 2009-11-07 I. Boztosun , W. D. M. Rae

A relativistic version of the coupled-cluster single-double (CCSD) method is developed for atoms with a single valence electron. In earlier work, a linearized version of the CCSD method (with extensions to include a dominant class of triple…

Atomic Physics · Physics 2009-11-13 Rupsi Pal , M. S. Safronova , W. R. Johnson , Andrei Derevianko , Sergey G. Porsev

By inferring the dynamic permittivity of different material media from the observations and calculating dynamic electric dipole polarizabilties of the Li through Cs alkali atoms, precise values of $C_3$ coefficients were estimated in Phys.…

Atomic Physics · Physics 2023-10-02 Harpreet Kaur , Vipul Badhan , Bindiya Arora , B. K. Sahoo

Being a determination at low energies, the analysis of hadronic tau decay data provides a rather precise determination of the strong coupling alpha_s after evolving the result to M_Z. At such a level of precision, even small…

High Energy Physics - Phenomenology · Physics 2015-06-03 D. Boito , O. Cata , M. Golterman , M. Jamin , K. Maltman , J. Osborne , S. Peris

The results of a recent next-to-leading order QCD analysis of the world data on polarized deep inelastic scattering are reported. New parameterizations are derived for the quark and gluon distributions and the value of $\alpha_s(M_z^2)$ is…

High Energy Physics - Phenomenology · Physics 2010-11-19 Johannes Blümlein , Helmut Böttcher

In the $GW$ approximation, the screened interaction $W$ is a non-local and dynamical potential that usually has a complex frequency dependence. A full description of such dependence is possible but often computationally demanding. For this…

The status of the experimental and theoretical investigations on the polarizabilities of the nucleon is presented. This includes a confirmation of the validity of the previously introduced recommended values of the polarizabilities [1,2].…

High Energy Physics - Phenomenology · Physics 2019-11-15 Martin Schumacher

Methods of the explicitly correlated F12 approach are applied to the problem of calculating the uncoupled second-order dispersion energy in symmetry-adapted perturbation theory. The accuracy of the new method is tested for noncovalently…

Chemical Physics · Physics 2018-05-15 Michal Przybytek