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Related papers: Laser induced electron diffraction: a tool for mol…

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Intense light with frequencies above typical atomic or molecular ionization potentials as provided by free-electron lasers couples many photons into extended targets such as clusters and biomolecules. This implies, in contrast to…

Atomic and Molecular Clusters · Physics 2011-05-25 Christian Gnodtke , Ulf Saalmann , Jan-Michael Rost

We investigate the ionization dynamics of atoms irradiated by an intense laser field using a semiclassical model that includes magnetic Lorentz force in the rescattering process. We find that, the electrons tunneled with different initial…

Atomic Physics · Physics 2017-01-25 J. F. Tao , Q. Z. Xia , J. Cai , L. B. Fu , J. Liu

The tomographic imaging of arbitrary molecular orbitals via high-order harmonic generation requires that electrons recollide from one direction only. Within a semi-classical model, we show that extremely short phase-stabilized laser pulses…

Atomic Physics · Physics 2009-11-13 Elmar V. van der Zwan , Manfred Lein

A photoelectron forced to pass through two atomic energy levels before receding from the residual ion shows interference fringes in its angular distribution as manifestation of a two-slit-type interference experiment in wave-vector space.…

Quantum Physics · Physics 2019-07-16 Jonas Wätzel , Andrew James Murray , Jamal Berakdar

Using a three-dimensional quasiclassical technique we explore the double ionization pathways of a diatomic molecule driven by an intense infrared (800nm) ultrashort laser pulse. For intensities corresponding to the tunneling regime, we find…

Atomic Physics · Physics 2009-02-26 Agapi Emmanouilidou

We consider tunnel ionization of an atom or molecule in a strong field within an analytical treatment of the R-matrix method, in which an imaginary boundary is set up inside the classically forbidden region that acts as a source of ionized…

Quantum Physics · Physics 2016-11-26 Emilio Pisanty

D$_2$ molecules, excited by linearly cross-polarized femtosecond extreme ultraviolet (XUV) and near-infrared (NIR) light pulses, reveal highly structured D$^+$ ion fragment momenta and angular distributions that originate from two different…

Large polyatomic molecules typically exhibit low ionization potentials, Ip, leading to over-the-barrier ionization (OBI) already at relatively low intensities (~1013 W/cm2). We revisit laser-induced electron diffraction (LIED) in the…

Atomic Physics · Physics 2024-11-07 B. Belsa , K. M. Ziems , A. Sanchez , K. Chirvi , X. Liu , S. Grfe , J. Biegert

We study the dynamics of initial nucleation processes of photoinduced structural change of molecular crystals. In order to describe the nonadiabatic transition in each molecule, we employ a model of localized electrons coupled with a fully…

Materials Science · Physics 2009-11-13 Kunio Ishida , Keiichiro Nasu

We investigate electron correlation effects in internuclear-distance-dependent enhanced ionization of $\mathrm{H}_2$, $\mathrm{LiH}$, and $\mathrm{HF}$ molecules by intense near-infrared laser pulses using a 3D description of the systems…

Atomic Physics · Physics 2019-02-27 Siddhartha Chattopadhyay , Lars Bojer Madsen

The ionization of H2 in intense laser pulses is studied by numerical integration of the time-dependent Schr\"odinger equation for a single-active-electron model including the vibrational motion. The electron kinetic-energy spectra in…

Atomic Physics · Physics 2009-11-13 Stefan Pieper , Manfred Lein

When polarized electrons traverse a region where the laser light is focused their polarization varies even if their energy and direction of motion are not changed. This effect is due to interference of the incoming electron wave and an…

High Energy Physics - Phenomenology · Physics 2009-10-30 G. L. Kotkin , H. Perlt , V. G. Serbo

We investigate laser-induced nonsequential double ionization by a polarization-gated laser pulse, constructed employing two counter-rotating circularly polarized few cycle pulses with a time delay $T_{d}$. We address the problem within a…

Atomic Physics · Physics 2015-05-13 W. Quan , X. Liu , C. Figueira de Morisson Faria

Electron transfer within and between molecules is crucial in chemistry, biochemistry, and energy science. This study describes a quantum simulation method that explores the influence of light polarization on the electron transfer between…

We study single-photon ionization of aligned H$_2^+$ in a high-frequency low-intensity laser field. We focus on the case where the laser frequency is not far larger than the ionization potential of the target. The calculated photoelectron…

Atomic Physics · Physics 2022-12-02 F. B. Zhang , J. Y. Che , W. Y. Li , C. Chen , Y. J. Chen

The creation of well-thermalized, hot and dense plasmas is attractive for warm dense matter studies. We investigate collisionally induced energy absorption of an ultraintense and ultrashort laser pulse in a solid copper target using…

Plasma Physics · Physics 2020-04-29 Andréas Sundström , Laurent Gremillet , Evangelos Siminos , István Pusztai

The influence has been studied of the ionization laser polarization on the effective temperature of an ultracold electron source, which is based on near-threshold photoionization. This source is capable of producing both high-intensity and…

Atomic Physics · Physics 2013-12-24 W. J. Engelen , D. J. Bakker , O. J. Luiten , E. J. D. Vredenbregt

We simulate the femtosecond laser induced desorption dynamics of a diatomic molecule from a metal surface by including the effect of the electron and phonon excitations created by the laser pulse. Following previous models, the laser…

Materials Science · Physics 2016-01-14 Ivor Lončarić , M. Alducin , P. Saalfrank , J. I. Juaristi

We investigate the quantum interference shifts between energetically close states, where the state structure is observed by laser spectroscopy. We report a compact and analytical expression that models the quantum interference induced shift…

With a semiclassical quasi-static model we achieve an insight into the complex dynamics of two correlated electrons under the combined influence of a two-center Coulomb potential and an intense laser field. The model calculation is able to…

Atomic and Molecular Clusters · Physics 2009-11-13 J. Liu , D. F. Ye , J. Chen , X. liu