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We present an efficient particle-particle random phase approximation (ppRPA) approach that predicts accurate excitation energies of point defects, including the nitrogen-vacancy (NV$^-$) and the silicon-vacancy (SiV$^0$) centers in diamond…

Chemical Physics · Physics 2024-03-13 Jiachen Li , Yu Jin , Jincheng Yu , Weitao Yang , Tianyu Zhu

In the superconducting state, the presence of a finite gap in the excitation spectrum implies that the number of excitations (quasiparticles) is exponentially small at temperatures well below the critical one. Conversely, minute…

Superconductivity · Physics 2023-05-31 P. B. Fischer , G. Catelani

We present a real-space formulation and higher-order finite-difference implementation of periodic Orbital-free Density Functional Theory (OF-DFT). Specifically, utilizing a local reformulation of the electrostatic and kernel terms, we…

Computational Physics · Physics 2015-12-23 Swarnava Ghosh , Phanish Suryanarayana

Implicit and explicit density functionals for the exchange energy in finite two-dimensional systems are developed following the approach of Becke and Roussel [Phys. Rev. A 39, 3761 (1989)]. Excellent agreement for the exchange-hole…

Strongly Correlated Electrons · Physics 2008-05-08 S. Pittalis , E. Rasanen , N. Helbig , E. K. U. Gross

We extend our recently developed sparse-stochastic fragmented exchange formalism for ground-state hybrid DFT (ngH-DFT) to calculate absorption spectra within linear-response time-dependent Generalized Kohn-Sham DFT (LR-GKS-TDDFT), for…

Chemical Physics · Physics 2025-03-11 Mykola Sereda , Tucker Allen , Nadine C. Bradbury , Khaled Z. Ibrahim , Daniel Neuhauser

We present a framework for obtaining reliable solid-state charge and optical excitations and spectra from optimally-tuned range-separated hybrid density functional theory. The approach, which is fully couched within the formal framework of…

Materials Science · Physics 2015-09-30 Sivan Refaely-Abramson , Manish Jain , Sahar Sharifzadeh , Jeffrey B. Neaton , Leeor Kronik

Quasiparticle spectra of potentially half-metallic Co2MnSi and Co2FeSi Heusler compounds have been calculated within the one-shot GW approximation in an all-electron framework without adjustable parameters. For Co2FeSi the many-body…

Materials Science · Physics 2013-01-04 Markus Meinert , Christoph Friedrich , Günter Reiss , Stefan Blügel

The quasiparticle excitation spectrum of an isolated vortex in a clean layered d-wave superconductor is calculated, using both the Bogoliubov--de Gennes and the quasiclassical Eilenberger equations. Analytical solutions are obtained within…

Superconductivity · Physics 2015-06-25 Irena Knezevic , Zoran Radovic

The energy levels of the ground states of the three-particle and four-particle bound states of leptons in quantum electrodynamics are calculated. For the calculation, the variational method with Gaussian basis functions is used. The…

High Energy Physics - Phenomenology · Physics 2026-03-09 A. V. Eskin , A. P. Martynenko , F. A. Martynenko , D. K. Pometko

We study the statistics of quasiparticle and quasihole levels in small interacting disordered systems within the Hartree-Fock approximation. The distribution of the inverse compressibility, given according to Koopmans' theorem by the…

Mesoscale and Nanoscale Physics · Physics 2008-12-18 Shimon Levit , Dror Orgad

Recent progress in the applications of covariant density functional theory (CDFT) to the description of the spectroscopy of the heaviest nuclei is reviewed. The analysis of quasiparticle spectra in actinides and the heaviest A ~ 250 nuclei…

Nuclear Theory · Physics 2011-09-30 A. V. Afanasjev , H. Abusara , E. Litvinova , P. Ring

The $GW$-Bethe-Salpeter Equation (BSE) method is promising for calculating the low-lying excited states of molecular systems. So far, it has only been applied to rather small molecules, and in the commonly implemented diagonal…

Chemical Physics · Physics 2022-08-10 Arno Förster , Lucas Visscher

We develop a second order correction to commonly used density functional approximations (DFA) to eliminate the systematic delocalization error. The method, based on the previously developed global scaling correction (GSC), is an exact…

Chemical Physics · Physics 2021-07-22 Yuncai Mei , Zehua Chen , Weitao Yang

We formulate a time-dependent density functional theory (TDDFT) in terms of the density matrix to study ultrafast phenomena in semiconductor structures. A system of equations for the density matrix components, which is equivalent to the…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 V. Turkowski , C. A. Ullrich

A theory is developed for the evolution of the non-equilibrium distribution of quasiparticles when the scattering rate decreases due to particle collisions. We propose a "modified one-collision approximation" which is most effective for…

Disordered Systems and Neural Networks · Physics 2009-11-10 R. N. Gurzhi , A. I. Kopeliovich , A. N. Kalinenko , A. V. Yanovsky , E. N. Bogachek , Uzi Landman , H. Buhmann , L. W. Molenkamp

Following a nonperturbative formulation of strong-field QED developed in our earlier works, and using the Dirac model of the graphene, we construct a reduced QED_{3,2} to describe one species of the Dirac fermions in the graphene…

Mesoscale and Nanoscale Physics · Physics 2023-02-24 S. P. Gavrilov , D. M. Gitman

We propose a hybrid approach which employs the dynamical mean-field theory (DMFT) self-energy for the correlated, typically rather localized orbitals and a conventional density functional theory (DFT) exchange-correlation potential for the…

Strongly Correlated Electrons · Physics 2021-06-16 Sumanta Bhandary , Karsten Held

Recent progress in the field of (time-independent) ensemble density-functional theory (DFT) for excited states are reviewed. Both Gross-Oliveira-Kohn (GOK) and $N$-centered ensemble formalisms, which are mathematically very similar and…

Chemical Physics · Physics 2021-11-29 Filip Cernatic , Bruno Senjean , Vincent Robert , Emmanuel Fromager

A stochastic cumulant GW method is presented, allowing us to map the evolution of photoemission spectra, quasiparticle energies, lifetimes and emergence of collective excitations from molecules to bulk-like systems with up to thousands of…

Mesoscale and Nanoscale Physics · Physics 2018-03-21 Vojtech Vlcek , Eran Rabani , Daniel Neuhauser

The widely used thermal Hartree-Fock (HF) theory is generalized to include the effect of electron correlation while maintaining its quasi-independent-particle framework. An electron-correlated internal energy (or grand potential) is…

Statistical Mechanics · Physics 2024-08-22 So Hirata
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