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We map the complex electric fields associated with the scattering of surface plasmon polaritons by single sub-wavelength holes of different sizes in thick gold films. We identify and quantify the different modes associated with this event,…

Mesoscale and Nanoscale Physics · Physics 2012-12-18 N. Rotenberg , M. Spasenovic , T. L. Krijger , B. le Feber , F. J. Garcıa de Abajo , L. Kuipers

The conventional explanation of plasmon-enhanced Raman scattering attributes the enhancement to the antenna effect focusing the electromagnetic field into sub-wavelength volumes. Here we introduce a new model that additionally accounts for…

Mesoscale and Nanoscale Physics · Physics 2016-02-10 Philippe Roelli , Christophe Galland , Nicolas Piro , Tobias J. Kippenberg

A consistent semiquantitative theoretical analysis of electronic Raman scattering from many-electron quantum dots under resonance excitation conditions has been performed. The theory is based on random-phase-approximation-like wave…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 Alain Delgado , Augusto Gonzalez , D. J. Lockwood

Raman-based technologies have enabled many ground-breaking scientific discoveries related to surface science, single molecule chemistry and biology. For example, researchers have identified surface bound molecules by their Raman vibrational…

Optics · Physics 2020-03-12 Xiaoqin Shen , Hyungwoo Choi , Dongyu Chen , Wei Zhao , Andrea M. Armani

Generalizing recent work, the Raman scattering intensity from a semi-infinite superconducting superlattice is calculated taking into account the surface contribution to the density response functions. Our work makes use of the formalism of…

Condensed Matter · Physics 2009-10-28 W. C. Wu , A. Griffin

Presented here are studies of the impact of excitation angle on surface enhanced Raman and luminescence spectroscopy of dye immobilised on a plasmon active nanocavity array support. Results show that both Raman and luminescence intensities…

Optics · Physics 2015-05-20 Frances Lordan , James H Rice , Bincy Jose , Robert J Forster , Tia E Keyes

The propagation of a surface plasmon-polariton along a stack of doped graphene sheets is considered. This auxiliary problem is used to discuss: (i) the scattering of such a mode at an interface between the stack and the vacuum; (ii) the…

Mesoscale and Nanoscale Physics · Physics 2016-06-29 Yu. V. Bludov , N. M. R. Peres , G. Smirnov , M. I. Vasilevskiy

We demonstrate importance of molecular multiple excitons and higher-order plasmons for both enhancement and quenching of resonance Raman and fluorescence of single dye molecule located at plasmonic hotspot under strong coupling regime. The…

Optics · Physics 2019-02-28 Tamitake Itoh , Yuko S. Yamamoto

Low-frequency Raman scattering experiments have been performed on thin films consisting of nickel-silver composite nanoparticles embedded in alumina matrix. It is observed that the Raman scattering by the quadrupolar modes, strongly…

Condensed Matter · Physics 2007-05-23 H. Portales , L. Saviot , E. Duval , M. Gaudry , E. Cottancin , M. Pellarin , J. Lerme , M. Broyer

Surface plasmon scattering by 1D indentations and protrusions is examined, mainly in the optical regime. The width of the defects is fixed, while its height is varied. Both individual and arrays of defects are considered. Protrusions mainly…

Mesoscale and Nanoscale Physics · Physics 2010-09-22 Giovanni Brucoli , Luis Martín Moreno

We present theoretical results concerning inelastic light (Raman) scattering from semiconductor quantum dots. The characteristics of each dot state (whether it is a collective or single-particle excitation, its multipolarity, and its spin)…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 Alain Delgado , Augusto Gonzalez , David J. Lockwood

The surface-enhanced Raman scattering in graphene deposited on AlxGa1-xN/GaN axial heterostructure nanowires was investigated. The intensity of graphene Raman spectra was found not to be correlated with aluminium content. Analysis of…

The low efficiency of Raman spectroscopy can be overcome by placing the active molecules in the vicinity of scatterers, typically rough surfaces or nanostructures with various shapes. This surface-enhanced Raman scattering (SERS) leads to…

Strong light-matter coupling gives rise to polaritons -- quasiparticles that combine both photonic and material characteristics. Here, we show that polar nanocrystals exhibit structure- and environment-dependent Raman scattering, enabled by…

We present a systematic theoretical study of the Raman scattering effect for a two-level atomic system in near proximity of an ultrathin dielectric film with an embedded parallel array of periodically aligned single-wall semiconducting…

Mesoscale and Nanoscale Physics · Physics 2026-04-21 SK Firoz Islam , Michael Dean Pugh , Igor V. Bondarev

We explored the surface enhanced Raman scattering (SERS) activity of the InN nanostructures, possessing surface electron accumulation (SEA), using the Rhodamine 6G (R6G) molecules. SERS enhancement is observed for the InN nanostructures…

Materials Science · Physics 2018-08-14 Kishore K. Madapu , Sandip Dhara

We have developed a theory of Raman scattering with single and double spin flips of localized resident electrons and holes as well as nonequilibrium localized excitons in semiconductor perovskite crystals under optical excitation in the…

Materials Science · Physics 2022-12-14 A. V. Rodina , E. L. Ivchenko

The Dipole-Quadrupole theory of Surface Enhanced Hyper Raman Scattering (SEHRS), created by the authors is expounded in details. Peculiarities of the behavior of electromagnetic field on rough metal surfaces are considered. It is…

Optics · Physics 2014-11-17 V. P. Chelibanov , A. M. Polubotko

Speckle patterns produced by disordered scattering systems exhibit a sensitivity to addition of individual particles which can be used for sensing applications. Using a coupled dipole model we investigate how multiple scattering can enhance…

Optics · Physics 2021-08-03 Joel Berk , Matthew R. Foreman

Surface plasmons are usually described as surface waves with either a complex wavevector or a complex frequency. When discussing their merits in terms of field confinment or enhancement of the local density of states, controversies…