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We performed molecular dynamics simulations to study equilibrium and flow properties of a liquid in a nano-channel with confining surfaces coated with a layer of grafted semiflexible polymers. The coverage spans a wide range of grafting…

Computational Physics · Physics 2015-09-30 Kevin Speyer , Claudio Pastorino

The non-equilibrium structural and dynamical properties of a flexible polymer tethered to a reflecting wall and subject to oscillatory linear flow are studied by numerical simulations. Polymer is confined in two dimensions and is modeled as…

Soft Condensed Matter · Physics 2024-07-30 A. Lamura

Frictional properties of interfaces with dynamic chemical bonds have been the subject of intensive experimental investigation and modeling, as it provides important insights into the molecular origin of the empirical rate and state laws,…

Mesoscale and Nanoscale Physics · Physics 2020-01-24 Wengen Ouyang , Yao Cheng , Ming Ma , Michael Urbakh

There is ample evidence that polymer brushes reduce friction between surfaces. Several industrial applications take advantage of this fact, such as those in plastic bag production, where the brushes act as slip agents; however, the complex…

We formulate a theoretical model of the shear failure of a thin film tethered to a rigid substrate. The interface between film and substrate is modeled as a cohesive layer with randomly fluctuating shear strength/fracture energy. We…

Materials Science · Physics 2009-11-13 Michael Zaiser , Paolo Moretti , Avraam Konstantinidis , Elias C Aifantis

We report on the multi-contact frictional dynamics of model elastomer surfaces rubbed against bare glass slides. The surfaces consist of layers patterned with thousands spherical caps (radius of curvature 100 $\mu$m) distributed both…

Soft Condensed Matter · Physics 2015-06-17 V. Romero , E. Wandersman , G. Debrégeas , A. Prevost

Self-mated hydrogel contacts show extremely small friction coefficients at low loads but a distinct velocity dependence. Here we combine mesoscopic simulations and experiments to test the polymer-relaxation hypothesis for this velocity…

Soft Condensed Matter · Physics 2023-05-30 Jan Mees , Rok Simič , Thomas C. O'Connor , Nicholas D. Spencer , Lars Pastewka

\textbf{Background} Hydrogels are crosslinked polymer networks that can absorb and retain a large fraction of liquid. Near a critical sliding velocity, hydrogels pressed against smooth surfaces exhibit time-dependent frictional behavior…

Soft Condensed Matter · Physics 2021-01-13 Brady Wu , Joshua Méndez Harper , Justin C. Burton

We constrast the dynamics in model unentangled polymer melts of chains of three different stiffnesses: flexible, intermediate, and rodlike. Flexible and rodlike chains, which readily solidify into close-packed crystals (respectively with…

Soft Condensed Matter · Physics 2016-11-23 Hong T. Nguyen , Robert S. Hoy

We present a modified model based on shear rate and aging time dependent static friction between a soft solid such as gelatin hydrogel and a hard surface for instance glass surface. Earlier the model for static friction (Juvekar and Singh,…

Soft Condensed Matter · Physics 2021-01-26 Arun K. Singh , Vinay A. Juvekar

Frictional properties of contacts between a smooth viscoelastic rubber and rigid surfaces are investigated using a torsional contact configuration where a glass lens is continuously rotated on the rubber surface. From the inversion of the…

Soft Condensed Matter · Physics 2017-02-01 M. Trejo , C. Frétigny , A. Chateauminois

We review the present state of understanding of solid friction at low velocities and for systems with negligibly small wear effects. We first analyze in detail the behavior of friction at interfaces between wacroscopic hard rough solids,…

Soft Condensed Matter · Physics 2015-06-25 Tristan Baumberger , Christiane Caroli

We propose a simple friction model for isolated polymer chains on a solid substrate. The chains are pulled at constant velocity by one end, the other end can be trapped on the solid substrate on localised sites. We focus on the energy…

Soft Condensed Matter · Physics 2009-10-31 T. Charitat , J. F. Joanny

We present molecular dynamics friction calculations for confined hydrocarbon solids with molecular lengths from 20 to 1400 carbon atoms. Two cases are considered: (a) polymer sliding against a hard substrate, and (b) polymer sliding on…

Soft Condensed Matter · Physics 2009-11-19 I. M. Sivebaek , V. N. Samoilov , B. N. J. Persson

We study the deformations of elastic filaments confined within slowly-shrinking circular boundaries, under contact forces with friction. We perform computations with a spring-lattice model that deforms like a thin inextensible filament of…

Soft Condensed Matter · Physics 2022-02-23 Silas Alben

We measure the displacement response of a frictional multicontact interface between identical polymer glasses to a biased shear force oscillation. We evidence the existence, for maximum forces close below the nominal static threshold, of a…

Materials Science · Physics 2009-11-07 L. Bureau , T. Baumberger , C. Caroli

An exact solution of coarse-grained polymer models with fluctuating internal friction and hydrodynamic interactions has not been proposed so far due to a one-to-all coupling between the connector vector velocities that precludes the…

Soft Condensed Matter · Physics 2024-06-19 R. Kailasham , Rajarshi Chakrabarti , J. Ravi Prakash

We study the possibility for a semi-infinite block of linear viscoelastic material, in homogeneous frictional contact with a non-deformable one, to slide under shear via a periodic set of ``self-healing pulses'', i.e. a set of drifting slip…

Materials Science · Physics 2009-10-31 C. Caroli

We consider directed semiflexible polymers embedded in a fluctuating surface which is governed by either surface tension or bending rigidity. The attractive interactions induced by the fluctuations of the surface reduce the rigidity of the…

Condensed Matter · Physics 2009-10-28 Ramin Golestanian

Thin liquid films on surfaces are part of our everyday life, they serve e.g. as coatings or lubricants. The stability of a thin layer is governed by interfacial forces, described by the effective interface potential, and has been subject of…

Soft Condensed Matter · Physics 2015-06-04 Oliver Bäumchen , Renate Fetzer , Mischa Klos , Matthias Lessel , Ludovic Marquant , Hendrik Hähl , Karin Jacobs