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Related papers: Projected Hartree-Fock Theory

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The localized Hartree-Fock potential has proven to be a computationally efficient alternative to the optimized effective potential, preserving the numerical accuracy of the latter and respecting the exact properties of being…

Quantum Physics · Physics 2015-08-18 V. U. Nazarov , G. Vignale

We use different types of determinantal Hartree-Fock (HF) wave functions to calculate variational bounds for the ground state energy of spin-half fermions in volume V_0, with mass m, electric charge zero, and magnetic moment mu, which are…

Strongly Correlated Electrons · Physics 2008-11-26 Sudhanshu S. Jha , S. D. Mahanti

Variation after particle-number restoration is incorporated for the first time into the Hartree-Fock-Bogoliubov framework employing the Skyrme energy density functional with zero-range pairing. The resulting projected HFB equations can be…

Nuclear Theory · Physics 2008-11-26 M. V. Stoitsov , J. Dobaczewski , R. Kirchner , W. Nazarewicz , J. Terasaki

Time-dependent Hartree--Fock (TDHF) method has been applied to various low-energy nuclear reactions, such as fusion, fission, and multinucleon transfer reactions. In this Mini Review, we summarize recent attempts to bridge a microscopic…

Nuclear Theory · Physics 2020-03-16 Kouhei Washiyama , Kazuyuki Sekizawa

A uniform derivation is presented of the self-consistent field equations in a finite basis set. Both restricted and unrestricted Hartree-Fock (HF) theory as well as various density functional (DF) approximations are considered. The unitary…

Computational Physics · Physics 2020-03-10 Susi Lehtola , Frank Blockhuys , Christian Van Alsenoy

Within the constrained Hartree-Fock (CHF) theory, an analytic condition is derived to estimate whether a concept of the self-consistent mean field is realized or not in level repulsive region. The derived condition states that an iterative…

Nuclear Theory · Physics 2009-11-10 Lu Guo , Fumihiko Sakata , Enguang Zhao

In the low-energy region far below the chiral symmetry breaking scale (which is of the order of 1 GeV) chiral perturbation theory provides a model-independent approach for quantitative description of nuclear processes. In the two- and…

High Energy Physics - Lattice · Physics 2016-08-14 Hermann Krebs , Bugra Borasoy , Evgeny Epelbaum , Dean Lee , Ulf-G. Meißner

We derive a multiconfigurational time-dependent Hartree theory for systems with particle conversion. In such systems particles of one kind can convert to another kind and the total number of particles varies in time. The theory thus extends…

Quantum Physics · Physics 2009-02-07 Ofir E. Alon , Alexej I. Streltsov , Lorenz S. Cederbaum

We prove the existence of solutions of the reduced Hartree-Fock equations at finite temperature for a periodic crystal with a small defect, and show total screening of the defect charge by the electrons. We also show the convergence of the…

Mathematical Physics · Physics 2020-07-28 Antoine Levitt

The Hartree-Fock equation is a fundamental equation in many-electron problems. It is of practical importance in quantum chemistry to find solutions to the Hartree-Fock equation. The self-consistent field (SCF) method is a standard numerical…

Analysis of PDEs · Mathematics 2023-11-17 Sohei Ashida

A new approach, motivated by Fock space localization, for constructing a reduced many-particle Hilbert space is proposed and tested. The self-consistent Hartree-Fock (SCHF) approach is used to obtain a single-electron basis from which the…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 Richard Berkovits

A practical electronic structure method in which a two-body functional is the fundamental variable is constructed. The basic formalism of our method is equivalent to Hartree-Fock density matrix functional theory [M. Levy in {\it Density…

Other Condensed Matter · Physics 2008-04-23 Balazs Hetenyi , Andreas W. Hauser

Extending density functional theory (DFT) to an {\it ab initio} orbital functional theory (OFT) requires new methodology for nonlocal exchange and correlation potentials. This paper describes such modifications to a standard Dirac-Slater…

Condensed Matter · Physics 2007-05-23 R. K. Nesbet

The crucial step in density-corrected Hartree-Fock density functional theory (DC(HF)-DFT) is to decide whether the density produced by the density functional for a specific calculation is erroneous and hence should be replaced by, in this…

Chemical Physics · Physics 2023-09-20 Daniel Graf , Alex J. W. Thom

Fractional-spin errors are inherent in all current approximate density functionals, including Hartree-Fock theory, and their origin has been related to strong static correlation effects. The conventional way to encode fractional-spin…

The use of an approximate reference state wave function |Phi_r> in electronic many-body methods can break the spin symmetry of Born-Oppenheimer spin-independent Hamiltonians. This can result in significant errors, especially when bonds are…

Computational Physics · Physics 2008-03-19 Wirawan Purwanto , W. A. Al-Saidi , Henry Krakauer , Shiwei Zhang

In this paper, we study the mixing of one-particle-one-hole projected states with the variation after projection (VAP) wave functions in attempt to improve the approximation of this method. It turns out that when minimizing only the lowest…

Nuclear Theory · Physics 2023-06-07 Xiao Lu , Zhan-Jiang Lian , Zao-Chun Gao

The few determinant (FED) methodology, introduced in our previous works for 1D lattices, is here adapted for the repulsive two-dimensional Hubbard model at half-filling and with finite doping fractions. Within this configuration mixing…

Strongly Correlated Electrons · Physics 2015-06-22 R. Rodríguez-Guzmán , Carlos A. Jiménez-Hoyos , Gustavo E. Scuseria

Slater determinants have underpinned quantum chemistry for nearly a century, yet their full potential has remained challenging to exploit. In this work, we show that a variational wavefunction composed of a few hundred optimized…

Chemical Physics · Physics 2026-04-17 Clemens Giuliani , Jannes Nys , Rocco Martinazzo , Giuseppe Carleo , Riccardo Rossi

In electronic structure theory, restricted single-reference coupled cluster (CC) captures weak correlation but fails catastrophically under strong correlation. Spin-projected unrestricted Hartree-Fock (SUHF), on the other hand, misses weak…

Chemical Physics · Physics 2017-11-22 John A. Gomez , Thomas M. Henderson , Gustavo E. Scuseria
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