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The response of gold nanoparticle dimers is studied theoretically near and beyond the limit where the particles are touching. As the particles approach each other, a dominant dipole feature is observed that is pushed into the infrared due…

Other Condensed Matter · Physics 2009-11-13 I. Romero , J. Aizpurua , G. W. Bryant , F. J. Garcia de Abajo

We consider the effect of electromagnetic coupling between localized surface plasmons in a metallic nanoparticle (NP) and excitons or weakly interacting electron-hole pairs in a semiconductor matrix where the NP is embedded. An expression…

Mesoscale and Nanoscale Physics · Physics 2018-10-08 Rui M. S. Pereira , Joel Borges , Georgui V. Smirnov , Filipe Vaz , Mikhail I. Vasilevskiy

Steady-state plasmonic lasing is studied theoretically for a system consisting of many dye molecules arranged regularly around a gold nano-sphere. A three-level model with realistic molecular dissipation is employed to analyze the…

Optics · Physics 2018-01-31 Yuan Zhang , Klaus Mølmer

Strong coupling (SC) between light and matter excitations such as excitons and molecular vibrations bear intriguing potential for controlling chemical reactivity, conductivity or photoluminescence. So far, SC has been typically achieved…

An optical nanoantenna and adjacent atomic systems are strongly coupled when an excitation is repeatedly exchanged between these subsystems prior to its eventual dissipation into the environment. It remains challenging to reach the strong…

Mesoscale and Nanoscale Physics · Physics 2013-11-15 Karolina Słowik , Robert Filter , Jakob Straubel , Falk Lederer , Carsten Rockstuhl

Surface polaritons display short wavelengths compared to propagating light, thus enabling large spatial concentration and enhancement of electromagnetic energy. However, this wavelength mismatch is generally accompanied by poor…

Optics · Physics 2021-04-13 Eduardo J. C. Dias , F. Javier García de Abajo

Strong coupling of molecules to vacuum fields has been widely reported to lead to modified chemical properties such as reaction rates. However, some recent attempts to reproduce infrared strong coupling results have not been successful,…

Mesoscale and Nanoscale Physics · Physics 2024-01-03 Philip A. Thomas , Wai Jue Tan , Vasyl G. Kravets , Alexander N. Grigorenko , William L. Barnes

The energetic positions of molecular electronic states at molecule/electrode interfaces are crucial factors for determining the transport and optoelectronic properties of molecular junctions. Strong light--matter coupling offers a potential…

Mesoscale and Nanoscale Physics · Physics 2023-05-10 Kuniyuki Miwa , Souichi Sakamoto , Akihito Ishizaki

Crystals of plasmonic metal nanoparticles have intriguing optical properties. They reach the regimes of ultrastrong and deep strong light-matter coupling, where the photonic states need to be included in the simulation of material…

An emitter in the vicinity of a metal nanostructure is quenched by its decay through non-radiative channels, leading to the belief in a zone of inactivity for emitters placed within $<$10nm of a plasmonic nanostructure. Here we demonstrate…

We reveal new aspects of the interaction between plasmons and phonons in 2D materials that go beyond a mere shift and increase in plasmon width due to coupling to either intrinsic vibrational modes of the material or phonons in a supporting…

The nonlinear optical dynamics of nano-materials comprised of plasmons interacting with quantum emitters is investigated by a self-consistent model based on the coupled Maxwell-Liouville-von Neumann equations. It is shown that ultra-short…

Mesoscale and Nanoscale Physics · Physics 2013-12-04 Maxim Sukharev , Tamar Seideman , Robert J. Gordon , Adi Salomon , Yehiam Prior

We have studied theoretically the exciton-plasmon coupling effects on the third-order optical nonlinearity of a coherently coupled hybrid system of a metal nanoparticle and a semiconductor quantum dot in the presence of a strong control…

Optics · Physics 2013-07-23 Nam-Chol Kim , Myong-Chol Ko , Song-Jin Im , Zhong-Hua Hao

Surface plasmon polaritons (plasmons) have the potential to interface electronic and optical devices. They could prove extremely useful for integrated quantum information processing. Here we demonstrate on-chip electrical detection of…

Mesoscale and Nanoscale Physics · Physics 2010-01-18 Reinier W. Heeres , Sander N. Dorenbos , Benny Koene , Glenn S. Solomon , Leo P. Kouwenhoven , Valery Zwiller

Plasmon hybridization between closely spaced nanoparticles yields new hybrid modes not found in individual constituents, allowing for the engineering of resonance properties and field enhancement capabilities of metallic nanostructure.…

Optics · Physics 2016-10-13 Jingjing Zhang , Zhen Liao , Yu Luo , Xiaopeng Shen , Stefan A. Maier , Tie Jun Cui

We present a quantum theoretical treatment of light-matter coupling in the system consisting of a quantum dot and a spherical core-shell metal-dielectric multilayer nanoparticle. It is shown that both weak and strong coupling regimes can be…

Optics · Physics 2015-12-18 Mehedi Hasan , Ivan Iorsh , Pavel Belov

Plasmonic nanocavities enable access to the quantum properties of matter, but are often simplified to single mode models despite their complex multimode structure. Here, we show that off-resonant plasmonic modes in fact play a crucial role…

Quantum Physics · Physics 2024-11-13 Angus Crookes , Ben Yuen , Angela Demetriadou

Molecular polaritons are hybrid states of photonic and molecular character that form when molecules strongly interact with light. Strong coupling tunes energy levels and importantly, can modify molecular properties (e.g. photoreaction…

Chemical Physics · Physics 2023-02-14 Francesca Fassioli , Kyu Hyung Park , Sarah E. Bard , Gregory D. Scholes

We study the strong-coupling (SC) interaction between two like-charged membranes of finite thickness embedded in a medium of higher dielectric constant. A generalized SC theory is applied along with extensive Monte-Carlo simulations to…

Soft Condensed Matter · Physics 2009-05-26 Y. S. Jho , M. Kanduc , A. Naji , R. Podgornik , M. W. Kim , P. A. Pincus

Effects of coupling between an molecular exciton and a surface plasmon (exciton-plasmon coupling) on the luminescence properties of the molecule and the surface plasmons are investigated using nonequilibrium Green's function method.…

Materials Science · Physics 2013-11-12 Kuniyuki Miwa , Mamoru Sakaue , Hideaki Kasai
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