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The complete magnetic and multiferroic phase diagram of Mn$_{1-x}$Co$_{x}$WO$_4$ single crystals is investigated by means of magnetic, heat capacity, and polarization experiments. We show that the ferroelectric polarization…

Strongly Correlated Electrons · Physics 2012-07-13 K. -C. Liang , Y. Q. Wang , Y. Y. Sun , B. Lorenz , F. Ye , J. A. Fernandez-Baca , H. A. Mook , C. W. Chu

Obtaining strong magnetoelectric couplings in bulk materials and heterostructures is an ongoing challenge. We demonstrate that manganite heterostructures of the form ${\rm (Insulator)/(LaMnO_3)_n/(CaMnO_3)_n/(Insulator)}$ show strong…

Strongly Correlated Electrons · Physics 2017-02-22 Sanjukta Paul , Ravindra Pankaj , Sudhakar Yarlagadda , Pinaki Majumdar , Peter B. Littlewood

Obtaining strong magnetoelectric couplings in bulk materials and heterostructures is an ongoing challenge. We demonstrate that manganite heterostructures of the form ${\rm (Insulator)/(LaMnO_3)_n/(CaMnO_3)_n/(Insulator)}$ show strong…

Strongly Correlated Electrons · Physics 2017-11-22 Sanjukta Paul , Ravindra Pankaj , Sudhakar Yarlagadda , Pinaki Majumdar , Peter B. Littlewood

A neutron scattering investigation of the magnetoelectric coupling in PbFe_{1/2}Nb_{1/2}O_{3} (PFN) has been undertaken. Ferroelectric order occurs below 400 K, as evidenced by the softening with temperature and subsequent recovery of the…

Materials Science · Physics 2018-07-20 C. Stock , S. R. Dunsiger , R. A. Mole , X. Li , H. Luo

An effective model is developed to explain the phase diagram and the mechanism of magnetoelectric coupling in multiferroics, $RMn_2O_5$. We show that the nature of magnetoelectric coupling in $RMn_2O_5$ is a coupling between two Ising-type…

Strongly Correlated Electrons · Physics 2009-11-13 Chen Fang , Jiangping Hu

Our results describe an unprecedented example of change in the mechanism of magnetically-induced electric polarization from spin current to spin-dependent p-d hybridization model. We have followed the evolution of the magnetic structures of…

By calculating the electronic, orbital, magnetic and lattice structure of half-doped manganites we establish the central role of oxygen buckling caused by the tilting of the MnO$_6$ octahedra -- in essence a steric effect. The buckling…

Strongly Correlated Electrons · Physics 2015-05-27 Paolo Barone , Silvia Picozzi , Jeroen van den Brink

Hexagonal YMnO_3 with space group P63cm is one of the rare examples of multiferroic materials that exhibit co-dependence of a robust ferroelectric phase along with antiferromagnetic ordering. This is primarily ascribed to tilting of the…

Strongly Correlated Electrons · Physics 2010-05-25 A. K. Singh , S. D. Kaushik , V. Siruguri , S. Patnaik

We present the microscopic theory of improper multiferroicity in BiMnO3, which can be summarized as follows: (1) the ferroelectric polarization is driven by the hidden antiferromagnetic order in the otherwise centrosymmetric C2/c structure;…

Materials Science · Physics 2010-11-01 I. V. Solovyev , Z. V. Pchelkina

This work reports an experimental investigation of the magneto-elastic coupling and polarization character of magnetic phases of the orthorhombic Eu1-xYxMnO3 system at low temperatures. The temperature dependence of the polarization…

Recent progress in the field of multiferroics led to the discovery of many new materials in which ferroelectricity is induced by cycloidal spiral orders. The direction of the electric polarization is typically constrained by spin…

We report the observation of a magnetic polarization of the O\,$2p$-states in YMn$_2$O$_5$ through the use of soft X-ray resonant scattering at the oxygen $K$-edge. Remarkably, we find that the temperature dependence of the integrated…

Strongly Correlated Electrons · Physics 2015-03-19 S. Partzsch , S. B. Wilkins , J. P. Hill , E. Schierle , E. Weschke , D. Souptel , B. Büchner , J. Geck

There has been tremendous research activity in the field of magneto-electric (ME) multiferroics after Kimura et al. [1] showed that antiferromagnetic and ferroelectric order coexist in orthorhom- bically distorted perovskite TbMnO3 and are…

A systematic microscopic theory of magnetically induced ferroelectricity and lattice modulation is presented for all electron configurations of Mott-insulating transition-metal oxides. Various mechanisms of polarization are identified in…

Strongly Correlated Electrons · Physics 2009-11-13 Chenglong Jia , Shigeki Onoda , Naoto Nagaosa , Jung Hoon Han

The origin of the spiral spin-order in perovskite multiferroic manganites $R$MnO$_{3}$ ($RE=$ Tb or Dy) is here investigated using a two $e_{\rm g}$-orbitals double-exchange model. Our main result is that the experimentally observed spiral…

Strongly Correlated Electrons · Physics 2008-10-22 Shuai Dong , Rong Yu , Seiji Yunoki , J. -M. Liu , Elbio Dagotto

Type-II multiferroics, in which the magnetic order breaks inversion symmetry, are appealing for both fundamental and applied research due their intrinsic coupling between magnetic and electrical orders. Using first-principles calculations…

Materials Science · Physics 2023-11-20 Urmimala Dey , Mark S. Senn , Nicholas C. Bristowe

The correlation between static magnetoelectric coupling and magnetic structure was investigated in $TbMn_{0.98}Fe_{0.02}O_{3}$ with magnetic field up to 8 T and down to 2 K. Single-crystal neutron diffraction experiments reveal a…

We present a first-principles study on the interface between perovskite ferroelectrics (PbTiO3) and conducting magnetic manganites La_{1-x}Sr_xMnO3. We show that by switching the ferroelectric polarization, additional carriers are…

Materials Science · Physics 2015-06-11 Hanghui Chen , Sohrab Ismail-Beigi

Magnetization, magnetoresistance, and magnetodielectric measurements have been carried out on the half doped charge ordered manganite, Pr_0.5Ca_0.5MnO_3. The low temperature state is found to be strongly dependent on the oxygen…

Strongly Correlated Electrons · Physics 2009-04-29 A. Karmakar , S. Majumdar , A. K. Singh , S. Patnaik , S. Giri

We have deployed density functional theory, Wannier function analysis and mean-field calculations to investigate the double-double perovskite compound CaMnCrSbO_{6}. The crystallographically non-equivalent Mn atoms in the unit cell have…

Materials Science · Physics 2022-06-14 Rakshanda Dhawan , Padmanabhan Balasubramanian , Tashi Nautiyal