Related papers: Sub-natural linewidths in excited-state spectrosco…
We present ultrafast transient absorption spectra of two oligofluorene derivatives in dilute solution. These spectra display clear vibronic structure, which we analyze rigorously using a time-dependent formalism of absorption to extract the…
We report measurements of absolute transition frequencies and hyperfine coupling constants for the 8S_{1/2}, 9S_{1/2}, 7D_{3/2}, and 7D_{5/2} states in ^{133}Cs vapor. The stepwise excitation through either the 6P_{1/2} or 6P_{3/2}…
Doppler broadening presents a major limitation for high-resolution spectroscopy and nonlinear optics in room-temperature atomic vapors. Here, we demonstrate the suppression of Doppler broadening accompanied by pronounced absorption on the…
We have measured the 6s - 7p_{1/2,3/2} transition probabilities in atomic cesium using a direct absorption technique. We use our result plus other previously measured transition rates to derive an accurate value of the vector transition…
We have completed a measurement of the Stark shift within the $^{115}$In $6s_{1/2} \rightarrow 6p_{1/2}$ excited-state transition using two-step laser spectroscopy in an indium atomic beam. Combining this measurement with recent…
We experimentally study the absorption spectroscopy from a collection of gaseous $^87 Rb$ atoms at room temperature irradiated with three fields. Two of these fields are in a pump probe saturation absorption configuration. The third field…
We have studied electromagnetically induced transparency (EIT) in diatomic cesium molecules in a vapor cell by using tunable diode lasers. We have observed a sub-natural Lambda-resonance in an absorption molecular band at different cesium…
We optically probe the spectrum of ground and excited state transitions of an individual, electrically tunable self-assembled quantum dot molecule. Photocurrent absorption measurements show that the spatially direct neutral exciton…
The 5S$\to$6P transition in Rubidium (Rb) at 420 nm offers the advantage of a narrower linewidth and diverse applications in quantum technologies. However, the direct spectroscopy at this transition is challenging due to its weak transition…
The $6S_{1/2}-5D_{5/2}$ electric quadrupole transition is investigated in Cesium vapor at room temperature via nonlinear Doppler-free 6P-6S-5D three-level spectroscopy. Frequency-resolved studies of individual E2 hyperfine lines allow one…
In this paper, we present a theoretical simulation of 87Rb absorption spectrum in a thermal cm-cell which is adaptive to the experimental observation. In experiment, the coupling and probe beams are configured to copropagate but…
Using the inherent timing stability of pulses from a mode-locked laser, we have precisely measured the cesium $6P_{3/2}$ excited state lifetime. An initial pump pulse excites cesium atoms in two counter-propagating atomic beams to the…
We present a detailed study of the absolute Doppler-broadened absorption of a probe beam scanned across the potassium D lines in a thermal vapour. Spectra using a weak probe were measured on the 4S $\rightarrow$ 4P transition and compared…
The resistive transition width of a recently discovered room temperature near-ambient-pressure superconductor [1] changes by more than three orders of magnitude between different samples, with the transition temperature nearly unchanged.…
Spectroscopy has played the key role in revealing, and thereby understanding, the structure of atoms and molecules. A central drive in this field is the pursuit of higher precision and accuracy so that ever more subtle effects might be…
A tunable diode laser spectrometer has been employed to examine the overtone absorption lines of $^{12}$CH$_4$ in the region around 12780 cm$^{-1}$ (780 nm) at room temperature. The spectrometer sources are commercially available tunable…
We demonstrate a method for precision spectroscopy on trapped ions in the limit of unresolved motional sidebands. By sympathetic cooling of a chain of crystallized ions we suppress adverse temperature variations induced by the spectroscopy…
Quantum mechanical calculations are performed of the emission and absorption profiles of the lithium 2s-2p resonance line under the influence of a helium perturbing gas. We use carefully constructed potential energy surfaces and transition…
Pump-probe saturation spectroscopy in the sub-terahertz region was performed in the rotational transition (J, K) = (16, 0) <- (15, 0) for gas-phase acetonitrile molecules in the counter-propagating configuration. We observed Lamb-dips at…
We present the observation of three semi-forbidden transitions in singly-ionized ytterbium from the metastable $^{2}\mathrm{F}^o_{7/2}$ state. Owing to the long lifetimes of both the upper and lower states involved, these transitions are…