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The silicon-vacancy center in diamond offers attractive opportunities in quantum photonics due to its favorable optical properties and optically addressable electronic spin. Here, we combine both to achieve all-optical coherent control of…

Nanostructures based on platinum, such as small clusters or STM-tips, often exhibit an atomistic structure that relies upon one or very few strongly under-coordinated platinum atoms. Here, we analyze a paradigmatic example, an apex atom on…

Mesoscale and Nanoscale Physics · Physics 2015-06-15 Richard Korytar , Ferdinand Evers

Crystal defects can confine isolated electronic spins and are promising candidates for solid-state quantum information. Alongside research focusing on nitrogen vacancy centers in diamond, an alternative strategy seeks to identify new spin…

Spin impurities in diamond have emerged as a promising building block in a wide range of solid-state-based quantum technologies. The negatively charged silicon-vacancy centre combines the advantages of its high-quality photonic properties…

Diamond is studied by path integral molecular dynamics simulations of the atomic nuclei in combination with a tight-binding Hamiltonian to describe its electronic structure and total energy. This approach allows us to quantify the influence…

Materials Science · Physics 2009-11-11 Rafael Ramirez , Carlos P. Herrero , Eduardo R. Hernandez

We study the spin gap of the S=1/2 Heisenberg model on the distorted diamond chain, which is recently proposed to represent magnetic properties of Cu_3 Cl_6 (H_2 O)_2 2H_8 C_4 SO_2. This model is composed of stacked trimers and has three…

Strongly Correlated Electrons · Physics 2009-10-31 Kazuhiro Sano , Ken'ichi Takano

Coupled spin chains are promising candidates for 'wiring up' qubits in solid-state quantum computing (QC). In particular, two nitrogen-vacancy centers in diamond can be connected by a chain of implanted nitrogen impurities; when driven by a…

Quantum Physics · Physics 2013-03-07 Yuting Ping , Brendon W. Lovett , Simon C. Benjamin , Erik M. Gauger

We present a scheme of positioning a single electron spin with sub-nanometer resolution through multiple nitrogen-vacancy centers in diamond. With unwanted noise suppressed by dynamical decoupling, the spin coherence of each center develops…

Quantum Physics · Physics 2016-04-27 Wen-Long Ma , Shu-Shen Li , Geng-Yu Cao , Ren-Bao Liu

The novel aspect of the centre (NV-) in diamond is the high degree of spin polarisation achieved through optical illumination. In this paper it is shown that the spin polarisation occurs as a consequence of an electron-vibration interaction…

Materials Science · Physics 2010-11-15 Neil Manson , Lachlan Rogers , Marcus Doherty , Lloyd Hollenberg

Spin transport electronics - spintronics - focuses on utilizing electron spin as a state variable for quantum and classical information processing and storage. Some insulating materials, such as diamond, offer defect centers whose…

Mesoscale and Nanoscale Physics · Physics 2016-03-23 J. Cardellino , N. Scozzaro , M. R. Herman , A. J. Berger , C. Zhang , K. C. Fong , C. Jayaprakash , D. V. Pelekhov , P. C. Hammel

We report hyperpolarization of the electronic spins associated with substitutional nitrogen defects in bulk diamond crystal. Hyperpolarization is achieved by optical pumping of nitrogen vacancy centers followed by rapid cross relaxation at…

Mesoscale and Nanoscale Physics · Physics 2017-02-22 M. Loretz , H. Takahashi , T. F. Segawa , J. M. Boss , C. L. Degen

Initializing a set of qubits to a given quantum state is a basic prerequisite for the physical implementation of quantum-information protocols. Here, we discuss the polarization of the electronic and nuclear spin in a single nitrogen…

Quantum Physics · Physics 2017-07-26 Tanmoy Chakraborty , Jingfu Zhang , Dieter Suter

The search for long-lived quantum memories, which can be efficiently interfaced with flying qubits is longstanding. One possible solution is to use the electron spin of a color center in diamond to mediate interaction between a long-lived…

Mesoscale and Nanoscale Physics · Physics 2024-01-24 Marco Klotz , Richard Waltrich , Niklas Lettner , Viatcheslav Agafonov , Alexander Kubanek

Optically accessible solid state defect spins serve as a primary platform for quantum information processing, where precise control of the electron spin and ancillary nuclear spins is essential for operation. Using the nitrogen-vacancy (NV)…

Quantum Physics · Physics 2026-02-12 Gergő Thiering , Adam Gali

In recent years, nitrogen-vacancy (NV) color centers in diamond have become excellent solid-state quantum sensors due to their electronic spin properties. Especially for their easy optical initialization and detection, together with their…

We use single-spin resonant spectroscopy to study the spin structure in the orbital excited-state of a diamond nitrogen-vacancy center at room temperature. We find that the excited state spin levels have a zero-field splitting that is…

Quantum Physics · Physics 2009-11-13 G. D. Fuchs , V. V. Dobrovitski , R. Hanson , A. Batra , C. D. Weis , T. Schenkel , D. D. Awschalom

There has been rapidly growing interest in hybrid quantum devices involving a solid-state spin and a macroscopic mechanical oscillator. Such hybrid devices create exciting opportunities to mediate interactions between disparate qubits and…

Neutral silicon vacancy (SiV0) centers in diamond are promising candidates for quantum networks because of their excellent optical properties and long spin coherence times. However, spin-dependent fluorescence in such defects has been…

High fidelity quantum control over qubits is of crucial importance for realistic quantum computing, and it turns to be more challenging when there are inevitable interactions among qubits. By employing a bandselective shaped pulse, we…

The nitrogen-vacancy center in diamond is a promising candidate for realizing the spin qubits concept in quantum information. Even though this defect is known for a long time, its electronic structure and other properties have not yet been…

Other Condensed Matter · Physics 2008-06-24 Adam Gali , Maria Fyta , Efthimios Kaxiras