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We study the spin and orbital dynamics of single nitrogen-vacancy (NV) centers in diamond between room temperature and 700 K. We find that the ability to optically address and coherently control single spins above room temperature is…

Mesoscale and Nanoscale Physics · Physics 2012-07-18 D. M. Toyli , D. J. Christle , A. Alkauskas , B. B. Buckley , C. G. Van de Walle , D. D. Awschalom

The nitrogen-vacancy (NV) centre, as a promising candidate solid state system of quantum information processing, its electron spin coherence is influenced by the magnetic field fluctuations due to the local environment. In pure diamonds,…

Mesoscale and Nanoscale Physics · Physics 2011-04-08 Nan Zhao , Jian-Liang Hu , Sai-Wah Ho , Tsz-Kai Wen , R. B. Liu

We present a protocol that detects molecular conformational changes with two nitroxide electron-spin labels and a nitrogen-vacancy (NV) center in diamond. More specifically, we demonstrate that the NV can detect energy shifts induced by the…

Quantum Physics · Physics 2022-12-21 C. Munuera-Javaloy , R. Puebla , B. D'Anjou , M. B. Plenio , J. Casanova

Due to interest in both solid state based quantum computing architectures and the application of quantum mechanical systems to nanomagnetometry, there has been considerable recent attention focused on understanding the microscopic dynamics…

Mesoscale and Nanoscale Physics · Physics 2013-09-30 Liam T. Hall , Jared H. Cole , Lloyd C. L. Hollenberg

Magnetic resonance techniques provide a powerful tool for controlling spin systems, with applications ranging from quantum information processing to medical imaging. Nevertheless, the behavior of a spin system under strong excitation…

Quantum Physics · Physics 2015-05-19 Lilian Childress , Jean McIntyre

We present measurements of spin relaxation times (T_1, T_1,rho, T_2) on very shallow (<5 nm) nitrogen-vacancy (NV) centers in high-purity diamond single crystals. We find a reduction of spin relaxation times up to 30x compared to bulk…

Mesoscale and Nanoscale Physics · Physics 2014-05-15 T. Rosskopf , A. Dussaux , K. Ohashi , M. Loretz , R. Schirhagl , H. Watanabe , S. Shikata , K. M. Itoh , C. L. Degen

Nitrogen-vacancy (NV) center in diamond is an ideal candidate for quantum sensors because of its excellent optical and coherence property. However, previous studies are usually conducted at low or room temperature. The lack of full…

We report an experimental study of the longitudinal relaxation time ($T_1$) of the electron spin associated with single nitrogen-vacancy (NV) defects hosted in nanodiamonds (ND). We first show that $T_1$ decreases over three orders of…

Mesoscale and Nanoscale Physics · Physics 2015-06-15 J. -P. Tetienne , T. Hingant , L. Rondin , A. Cavailles , L. Mayer , G. Dantelle , T. Gacoin , J. Wrachtrup , J. -F. Roch , V. Jacques

A broad effort is underway to understand and harness the interaction between superconductors and spin-active color centers with an eye on the realization of hybrid quantum devices and novel imaging modalities of superconducting materials.…

We characterize single nitrogen-vacancy (NV) centers created by 10-keV N+ ion implantation into diamond via thin SiO$_2$ layers working as screening masks. Despite the relatively high acceleration energy compared with standard ones (< 5…

Quantum Physics · Physics 2020-06-26 Shuntaro Ishizu , Kento Sasaki , Daiki Misonou , Tokuyuki Teraji , Kohei M. Itoh , Eisuke Abe

Dynamical polarization of nuclear spin ensembles is of central importance for magnetic resonance studies, precision sensing and for applications in quantum information theory. Here we propose a scheme to generate long-lived singlet pairs in…

Quantum Physics · Physics 2017-04-06 Johannes N. Greiner , D. D. Bhaktavatsala Rao , Jörg Wrachtrup

Understanding the limits to the spin-coherence of the nitrogen-vacancy (NV) center in diamond is vital to realizing the full potential of this quantum system. We show that relaxation on the $|m_{s}=-1\rangle \leftrightarrow…

Mesoscale and Nanoscale Physics · Physics 2021-02-17 M. C. Cambria , A. Gardill , Y. Li , A. Norambuena , J. R. Maze , S. Kolkowitz

Spin impurities in diamond have emerged as a promising building block in a wide range of solid-state-based quantum technologies. The negatively charged silicon-vacancy centre combines the advantages of its high-quality photonic properties…

Inhomogeneous dephasing from uncontrolled environmental noise can limit the coherence of a quantum sensor or qubit. For solid state spin qubits such as the nitrogen-vacancy (NV) center in diamond, a dominant source of environmental noise is…

Quantum Physics · Physics 2015-12-23 E. R. MacQuarrie , T. A. Gosavi , S. A. Bhave , G. D. Fuchs

The excellent sensitivities of quantum sensors are a double-edged sword: minuscule quantities can be observed, but any undesired signal acts as noise. This is challenging when detecting quantities that are obscured by such noise. Decoupling…

The nitrogen-vacancy (NV) center in diamond is supposed to be a building block for quantum computing and nanometer scale metrology at ambient conditions. Therefore, precise knowledge of its quantum states is crucial. Here, we experimentally…

Quantum Physics · Physics 2013-05-29 G. Waldherr , J. Beck , M. Steiner , P. Neumann , A. Gali , Th. Frauenheim , F. Jelezko , J. Wrachtrup

The most direct approach for characterizing the quantum dynamics of a strongly-interacting system is to measure the time-evolution of its full many-body state. Despite the conceptual simplicity of this approach, it quickly becomes…

Ultimate sensitivity for quantum magnetometry using nitrogen-vacancy (NV) centers in diamond is limited by number of NV centers and coherence time. Microwave irradiation with a high and homogeneous power density for a large detection volume…

A neutral nitrogen-vacancy center (NV$^0$) is promising for realizing strong coupling with a single microwave photon due to its large electric field sensitivity, although it is susceptible to environmental phonon noise at 5 K. Decreasing…

We present an experimental method to perform dual-channel lock-in magnetometry of time-dependent magnetic fields using a single spin associated with a nitrogen-vacancy (NV) color center in diamond. We incorporate multi-pulse quantum sensing…

Quantum Physics · Physics 2014-07-03 N. M. Nusran , M. V. Gurudev Dutt