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We propose a possible route to achieve high thermoelectric efficiency in molecular junctions by combining a local chemical tuning of the molecular electronic states with the use of semiconducting electrodes. The former allows to control the…

Materials Science · Physics 2009-08-05 D. Nozaki , H. Sevinçli , W. Li , R. Gutierrez , G. Cuniberti

Multi-heme cytochromes (MHC) are fascinating proteins used by bacterial organisms to shuttle electrons within and between their cells. When placed in a solid state electronic junction, they support temperature-independent currents over…

Quantum transport in mesoscopic conductors is essentially governed by the laws of quantum mechanics. One of the major open questions of quantum mechanics is what happens if non-commuting observables are measured simultaneously. Since…

Mesoscale and Nanoscale Physics · Physics 2010-03-15 Adam Bednorz , Wolfgang Belzig

We investigate the possibility of optical current control through single molecules which are weakly coupled to leads. A master equation approach for the transport through a molecule is combined with a Floquet theory for the time-dependent…

Chemical Physics · Physics 2016-09-08 Jörg Lehmann , Sébastien Camalet , Sigmund Kohler , Peter Hänggi

The dynamical control of tunneling processes of single particles plays a major role in science ranging from Shapiro steps in Josephson junctions to the control of chemical reactions via light in molecules. Here we show how such control can…

The semiconductor diode, which acts as an electrical rectifier and allows unidirectional electronic transports, is the key to information processing in integrated circuits. Analogously, an optical rectifier (or diode) working at specific…

Quantum Physics · Physics 2014-09-05 H. Z. Shen , Y. H. Zhou , X. X. Yi

Ultrafast photocurrent experiments are performed on semiconducting, single-walled carbon nanotubes under a resonant optical excitation of their subbands. The photogenerated excitons are dissociated at large electric fields and the resulting…

Mesoscale and Nanoscale Physics · Physics 2017-04-19 Christoph Karnetzky , Lukas Sponfeldner , Max Engl , Alexander W. Holleitner

We analyze long-range transport through an ac driven triple quantum dot with one single electron. An effective model is proposed for the analysis of photoassisted cotunnel in order to account for the virtual processes which dominate the…

Mesoscale and Nanoscale Physics · Physics 2015-04-07 Fernando Gallego-Marcos , Rafael Sánchez , Gloria Platero

Using a model comprising a 2-level bridge connecting free electron reservoirs we show that coupling of a molecular bridge to electron-hole excitations in the leads can markedly effect the source-drain current through a molecular junction.In…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Michael Galperin , Abraham Nitzan , Mark A. Ratner

Coherent one photon ($2 \omega$) and two photon ($ \omega$) electronic excitations are studied for graphene sheets and for carbon nanotubes using a long wavelength theory for the low energy electronic states. For graphene sheets we find…

Materials Science · Physics 2016-08-31 E. J. Mele , P. Kral , D. Tomanek

Among the most exciting recent advances in the field of superconducting quantum circuits is the ability to coherently couple microwave photons in low-loss cavities to quantum electronic conductors (e.g.~semiconductor quantum dots or carbon…

Mesoscale and Nanoscale Physics · Physics 2014-12-09 J. -R. Souquet , M. J. Woolley , Julien Gabelli , Pascal Simon , Aashish A. Clerk

Conical intersections (CI) between molecular potential energy surfaces with non-vanishing non-adiabatic couplings generally occur in any molecule consisting of at least three atoms. They play a fundamental role in describing the molecular…

We study transport through one or two ultrasmall quantum dots with discrete energy levels to which a time-dependent field is applied (e.g., microwaves). The AC field causes photon-assisted tunneling and also transitions between discrete…

Mesoscale and Nanoscale Physics · Physics 2009-10-30 Ph. Brune , C. Bruder , H. Schoeller

The Coulomb drag phenomenon in a Coulomb-coupled double quantum dot system is revisited with a simple model that highlights the importance of simultaneous tunneling of electrons. Previously, cotunneling effects on the drag current in…

Mesoscale and Nanoscale Physics · Physics 2018-02-16 Jong Soo Lim , Rosa Lopez , David Sanchez

This paper contains a detailed derivation of the photoinduced current density at third order in the coupling between a semiconductor and a multifrequency photon field, starting from its standard textbook expression as a third order time…

Mesoscale and Nanoscale Physics · Physics 2008-10-29 M. Combescot , O. Betbeder-Matibet

The coherent optical injection and temporal decay of spin and charge currents in semiconductor heterostructures is described microscopically, including excitonic effects, carrier LO-phonon and carrier-carrier scattering, as well as…

Other Condensed Matter · Physics 2007-05-23 Huynh Thanh Duc , T. Meier , S. W. Koch

We derive a formula for the current through an interacting quantum dot coupled to two supercouducting leads, using the non-equilibrium Green's function formalism. It is shown that the formula takes an especially simple form, when the…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 Kicheon Kang

We theoretically investigate the effect of inter-molecular Coulomb interactions on transport through molecular monolayers (or other devices based on a large number of nanoscale conductors connected in parallel). Due to the interactions, the…

Mesoscale and Nanoscale Physics · Physics 2013-04-09 Martin Leijnse

The time-of-flight method is a fundamental approach for characterizing the transport properties of semiconductors. Recently, the transient photocurrent and optical absorption kinetics have been simultaneously measured for thin films;…

Chemical Physics · Physics 2023-03-21 Kazuhiko Seki , Naoya Muramatsu , Tomoaki Miura , Tadaaki Ikoma

Understanding the carrier excitation and transport processes at the single-charge level plays a key role in quantum-dot-based solar cells and photodetectors. Here, we report on Coulomb-induced giant photocurrent enhancement of positive…

Mesoscale and Nanoscale Physics · Physics 2019-02-13 Kai Peng , Shiyao Wu , Xin Xie , Jingnan Yang , Chenjiang Qian , Feilong Song , Sibai Sun , Jianchen Dang , Yang Yu , Shushu Shi , Jiongji He , Xiulai Xu
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