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We have investigated Rb adsorption on the Si(100) surface for 0.5 and 1 monolayer coverages using the total energy method with norm-conserving pseudopotentials. For 2$\times$1 reconstruction at 1 ML coverage symmetrized dimers are found to…

Strongly Correlated Electrons · Physics 2007-05-23 E. Mete , R. Shaltaf , Ş. Ellialtıoğlu

Density-functional calculations on the polar TiX(111) (X = C, N) surfaces show (i) for clean surfaces, strong Ti3d-derived surface resonances (SR's) at the Fermi level and X2p-derived SR's deep in the upper valence band and (ii) for adatoms…

Materials Science · Physics 2009-11-11 Carlo Ruberto , Aleksandra Vojvodic , Bengt I. Lundqvist

First-principles calculations reveal that the adsorption of representative first-row atoms with different electronegativity, such as lithium (Li), carbon (C) and fluorine (F), on zigzag single-walled boron nitride nanotubes (BNNTs) exhibits…

Materials Science · Physics 2007-05-23 Jia Li , Gang Zhou , Haitao Liu , Wenhui Duan

Density-functional-theory calculations for the adsorption of molecular nitrogen on ruthenium surface are reported. It is found that nitrogen molecule is adsorbed while standing perpendicular to the triangular surface of ruthenium. The…

Chemisorption of CO on the stepped Cu(211) surface is studied within ab-initio density functional theory (DFT) and scanning tunneling microscopy (STM) imaging as well as manipulation experiments. Theoretically we focus on the experimentally…

Materials Science · Physics 2009-11-10 Marek Gajdos , Andreas Eichler , Jurgen Hafner , Gerhard Meyer , Karl-Heinz Rieder

Equilibrium atomic configurations and electron energy structure of ethanol adsorbed on the Si (111) surface are studied by the first-principles density functional theory. Geometry optimization is performed by the total energy minimization…

Computational Physics · Physics 2008-02-11 A. V. Gavrilenko , C. E. Bonner , V. I. Gavrilenko

First principles density functional calculations are used to study the early oxidation stages of the Mg(0001) surface for oxygen coverages 1/16 <= Theta <= 3 monolayers. It is found that at very low coverages O is incorporated below the…

Materials Science · Physics 2015-06-24 Elsebeth Schroder , Roman Fasel , Adam Kiejna

The adsorption of benzene on the Si(100) surface is studied theoretically using the self-consistent van der Waals density functional (vdW-DF) method. The adsorption energies of two competing adsorption structures, butterfly (BF) and…

Materials Science · Physics 2016-08-03 Yuji Hamamoto , Ikutaro Hamada , Kouji Inagaki , Yoshitada Morikawa

Extensive density-functional calculations are performed for chemisorption of atoms in the three first periods (H, B, C, N, O, F, Al, Si, P, S, and Cl) on the polar TiC(111) surface. Calculations are also performed for O on TiC(001), for…

Materials Science · Physics 2007-05-23 Carlo Ruberto , Bengt I. Lundqvist

Using scanning tunneling microscopy at low temperatures we investigated the adsorbate system Cu(111)-Cs for various cesium coverages. At low coverages we observe a hexagonally ordered Cs adsorption layer with a mutual adsorbate distance of…

Materials Science · Physics 2009-11-11 Th. von Hofe , J. Kroeger , R. Berndt

The first principles density functional theory (DFT) is applied to study effects of molecular adsorption on optical losses of silver (111) surface. The ground states of the systems including water, methanol, and ethanol molecules adsorbed…

Materials Science · Physics 2015-05-14 Alexander V. Gavrilenko , Carla S. McKinney , Vladimir I. Gavrilenko

Hydrogen segregation to vacancies in the surface and subsurface layers of (111) and (100) surfaces of Pd is studied in the density functional theory (DFT) approach. Adsorption energies and configurations of various clusters of H atoms at…

Materials Science · Physics 2020-06-24 A. V. Subashiev , H. H. Nee

We report scanning tunneling microscopy observations of Ge deposited on the Si(111)-7x7 surface for a sequence of sub-monolayer coverages. We demonstrate that Ge atoms replace so-called Si adatoms. Initially, the replacements are random,…

Materials Science · Physics 2007-05-23 Y. L. Wang , H. -J. Gao , H. M. Guo , Sanwu Wang , Sokrates T. Pantelides

We investigate the adsorption of a single tetracyanoethylene (TCNE) molecule on the silver (001) surface. Adsorption structures, electronic properties, and scanning tunneling microscopy (STM) images are calculated within density-functional…

Mesoscale and Nanoscale Physics · Physics 2016-06-22 Thorsten Deilmann , Peter Krüger , Michael Rohlfing , Daniel Wegner

Using density-functional theory and a tight-binding approach we investigate the physical origin of distinct favourable geometries of adsorbed hydrogen atoms in various graphyne structures, and the relation with electronic properties. In…

Materials Science · Physics 2014-02-07 Hunpyo Lee , Jahyun Koo , Massimo Capone , Yongkyung Kwon , Hoonkyung Lee

We present a density functional study of the structural and electronic properties of small Cu_n (n=1,4) aggregates on defect-free MgO(100). The calculations employ a slab geometry with periodic boundary conditions, supercells with up to 76…

Materials Science · Physics 2009-10-30 V. Musolino , A. Selloni , R. Car

The variation of the work function upon carbon adsorption on the reconstructed Au(110) surface is measured experimentally and compared to density functional calculations. The adsorption dynamics is simulated with ab-initio molecular…

Atomic Physics · Physics 2018-08-08 H. Z. Jooya , K. S. McKay , E. Kim , P. F. Weck , D. P. Pappas , D. A. Hite , H. R. Sadeghpour

The structures and energetics of organic molecules adsorbed onto clean and H-passivated Si(001)-(2$\times$1) surfaces have been calculated using density functional theory. For benzene adsorbed on the clean Si surface the tight-bridge…

Materials Science · Physics 2009-11-13 Karen Johnston , Risto M. Nieminen

During the design of fixed bed adsorbers, it is vital to understand the dynamic adsorption properties of the system. Because temperature is one of the most important factors affecting adsorbent performance, such that the dynamic adsorption…

We report a first-principles calculation that models the effect of iron (Fe) atoms on the adsorption of a tungsten (W) atom on W(100) surfaces. The adsorption of a W atom on a clean W(100) surface is compared with that of a W atom on a…

Materials Science · Physics 2009-11-13 J. Houze , Sungho Kim , Seong-Jin Park , Randall M. German , M. F. Horstemeyer , Seong-Gon Kim