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In simulating charged systems, it is often useful to treat some ionic components of the system at the mean-field level and solve the Poisson-Boltzmann (PB) equation to get their respective density profiles. The numerically intensive task of…

Soft Condensed Matter · Physics 2013-09-30 Vikram Jadhao , Francisco J. Solis , Monica Olvera de la Cruz

The optimized effective potential method is formulated as a convex minimization problem. This formulation does not require assumptions about $v$-representability nor functional differentiability. The formulation provides a natural framework…

Chemical Physics · Physics 2022-02-01 Erik I. Tellgren , Andre Laestadius , Markus Penz

We study finite-difference approximations of both Poisson and Poisson-Boltzmann (PB) electrostatic energy functionals for periodic structures constrained by Gauss' law and a class of local algorithms for minimizing the finite-difference…

Numerical Analysis · Mathematics 2024-09-25 Bo Li , Qian Yin , Shenggao Zhou

A variational approach is used to develop a robust numerical procedure for solving the nonlinear Poisson-Boltzmann equation. Following Maggs et al., we construct an appropriate constrained free energy functional, such that its…

Soft Condensed Matter · Physics 2020-04-29 M. Baptista , R. Schmitz , B. Duenweg

We consider the nonlinear Poisson-Boltzmann equation in the context of electrostatic models for a biological macromolecule, embedded in a bounded domain containing a solution of an arbitrary number of ionic species which is not necessarily…

Analysis of PDEs · Mathematics 2022-04-26 José A. Iglesias , Svetoslav Nakov

We introduce a new minimisation principle for Poisson equation using two variables: the solution and the gradient of the solution. This principle allows us to use any conforming finite element spaces for both variables, where the finite…

Numerical Analysis · Mathematics 2015-09-07 Bishnu P. Lamichhane

Poisson-Boltzmann (PB) theory is the classic approach to soft matter electrostatics which has been applied to numerous problems of physical chemistry and biophysics. Its essential limitations are the neglect of correlation effects and of…

Soft Condensed Matter · Physics 2016-08-03 Sahin Buyukdagli , Ralf Blossey

Starting from the microscopic reduced Hartree-Fock equation, we derive the nanoscopic linearized Poisson-Boltzmann equation for the electrostatic potential associated with the electron density.

Mathematical Physics · Physics 2020-12-07 Ilias , Chenn , Israel Michael Sigal

Mobile charge in an electrolytic solution can in principle be represented as the divergence of ionic polarization. After adding explicit solvent polarization a finite volume of electrolyte can then be treated as a composite non-uniform…

Soft Condensed Matter · Physics 2021-03-03 Michiel Sprik

We present a continuation of our theoretical research into the influence of co-solvent polarizability on a differential capacitance of the electric double layer [EPL 111, 28002 (2015)]. We formulate a modified Poisson-Boltzmann theory,…

Soft Condensed Matter · Physics 2016-05-11 Yu. A. Budkov , A. L. Kolesnikov , M. G. Kiselev

The basic aim is to extend some results and concepts of non-autonomous second order differential systems with convex potentials to the new context of multi-time Poisson-gradient PDE systems with convex potential. In this sense, we prove…

Dynamical Systems · Mathematics 2007-05-23 Iulian Duca , Ana-Maria Teleman , Constantin Udriste

A widely used electrostatics model in the biomolecular modeling community, the nonlinear Poisson-Boltzmann equation, along with its finite element approximation, are analyzed in this paper. A regularized Poisson-Boltzmann equation is…

Numerical Analysis · Mathematics 2010-01-12 Long Chen , Michael Holst , Jinchao Xu

The description of a conducting medium in thermal equilibrium, such as an electrolyte solution or a plasma, involves nonlinear electrostatics, a subject rarely discussed in the standard electricity and magnetism textbooks. We consider in…

Chemical Physics · Physics 2018-08-01 C. G. Gray , P. J. Stiles

We consider a class of nonlinear elliptic problems associated with models in biophysics, which are described by the Poisson-Boltzmann equation (PBE). We prove mathematical correctness of the problem, study a suitable class of…

Numerical Analysis · Mathematics 2020-12-15 Johannes Kraus , Svetoslav Nakov , Sergey Repin

The computational study of chemical reactions in complex, wet environments is critical for applications in many fields. It is often essential to study chemical reactions in the presence of applied electrochemical potentials, taking into…

Materials Science · Physics 2016-01-20 G. Fisicaro , L. Genovese , O. Andreussi , N. Marzari , S. Goedecker

The Poisson-Boltzmann equation offers an efficient way to study electrostatics in molecular settings. Its numerical solution with the boundary element method is widely used, as the complicated molecular surface is accurately represented by…

Numerical Analysis · Mathematics 2021-08-25 Stefan D. Search , Christopher D. Cooper , Elwin van't Wout

Electrostatic correlations and fluctuations in ionic systems can be described within an extended Poisson-Boltzmann theory using a Gaussian variational form. The resulting equations are challenging to solve because they require the solution…

Computational Physics · Physics 2015-06-17 Zhenli Xu , A. C. Maggs

An approximate analytical solution to the fluctuation potential problem in the modified Poisson-Boltzmann theory of electrolyte solutions in the restricted primitive model is presented. The solution is valid for all inter-ionic distances,…

Statistical Mechanics · Physics 2017-12-15 E. O. Ulloa-Dávila , L. B. Bhuiyan

Non-locality is being intensively studied in various PDE-contexts and in variational problems. The numerical approximation also looks challenging, as well as the application of these models to Continuum Mechanics and Image Analysis, among…

Analysis of PDEs · Mathematics 2021-06-07 Pablo Pedregal

We prove existence of variational solutions for a class of nonlocal evolution equations whose prototype is the double phase equation \begin{align*} \partial_t u &+ \text{P.V.}\int_{\mathbb{R}^N}…

Analysis of PDEs · Mathematics 2022-01-06 Harsh Prasad , Vivek Tewary
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