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We present a density functional theory analysis of the negatively charged nitrogen-vacancy (NV$^-$) defect complex in diamond located in the vicinity of (111)- or (100)-oriented surfaces with mixed (N,H)-terminations. We assess the…

Materials Science · Physics 2022-02-21 Wolfgang Körner , Reyhaneh Ghassemizadeh , Daniel F. Urban , Christian Elsässer

Pulsed ESR experiments are reported for ensembles of negatively-charged nitrogen-vacancy centers (NV$^-$) in diamonds at X-band magnetic fields (280-400 mT) and low temperatures (2-70 K). The NV$^-$ centers in synthetic type IIb diamonds…

Quantum Physics · Physics 2016-12-22 B. C. Rose , C. D. Weis , A. M. Tyryshkin , T. Schenkel , S. A. Lyon

The nitrogen-vacancy (NV) color center in diamond is an atom-like system in the solid-state which specific spin properties can be efficiently used as a sensitive magnetic sensor. An external magnetic field induces Zeeman shifts of the NV…

Mesoscale and Nanoscale Physics · Physics 2015-07-17 M. Chipaux , A. Tallaire , J. Achard , S. Pezzagna , J. Meijer , V. Jacques , J. -F. Roch , T. Debuisschert

We report a magnetic field dependence of fluorescence of diamond single crystals containing NV$^-$ centers. In such spectra, numerous sharp lines are found, which correspond to Level Anti-Crossings (LACs) in coupled spins systems comprising…

Mesoscale and Nanoscale Physics · Physics 2016-09-28 S. V. Anishchik , V. G. Vins , K. L. Ivanov

The nitrogen-vacancy (N-V) center in diamond is a promising atomic-scale system for solid-state quantum information processing. Its spin-dependent photoluminescence has enabled sensitive measurements on single N-V centers, such as: electron…

Other Condensed Matter · Physics 2015-06-25 R. J. Epstein , F. M. Mendoza , Y. K. Kato , D. D. Awschalom

Precise readout of spin states is crucial for any approach towards physical realization of a spin-based quantum computer and for magnetometry with single spins. Here, we report a new method to strongly improve the optical readout fidelity…

Quantum Physics · Physics 2010-03-01 M. Steiner , P. Neumann , J. Beck , F. Jelezko , J. Wrachtrup

Nuclear magnetic resonance (NMR) imaging with shallow nitrogen-vacancy (NV) centers in diamond offers an exciting route toward sensitive and localized chemical characterization at the nanoscale. Remarkable progress has been made to combat…

We describe a scanning device where a single spin is used as an ultrasensitive, nanoscale magnetic field sensor. As this "probe spin" we consider a single nitrogen-vacancy defect center in a diamond nanocrystal, attached to the tip of the…

Mesoscale and Nanoscale Physics · Physics 2008-09-23 C. L. Degen

Nitrogen-vacancy centres (NVs) in diamond are attractive for research straddling quantum information science and nanoscale magnetometry and thermometry. While ultrapure bulk diamond NVs sustain the longest spin coherence times among…

Mesoscale and Nanoscale Physics · Physics 2015-06-17 Helena S. Knowles , Dhiren M. Kara , Mete Atature

The interaction of solid-state electronic spins with deformations of their host crystal is an important ingredient in many experiments realizing quantum information processing schemes. Here, we theoretically characterize that interaction…

Mesoscale and Nanoscale Physics · Physics 2018-08-08 Péter Udvarhelyi , Vladyslav O. Shkolnikov , Adam Gali , Guido Burkard , András Pályi

We investigate the spin-coherence decay of NV$^-$-spins interacting with the strongly-coupled bath of nitrogen defects in diamond layers. For thin diamond layers, we demonstrate that the spin-coherence times exceed those of bulk diamond,…

Quantum-mechanical ab initio calculations are performed to elucidate the vibrational spectroscopic features of a common irradiation-induced defect in diamond, i.e. the neutral vacancy. Raman spectra are computed analytically through a…

Materials Science · Physics 2016-08-31 J. Baima , A. Zelferino , P. Olivero , A. Erba , R. Dovesi

Nuclear spins in solids exhibit long coherence times due to the small nuclear gyromagnetic ratio. This weak environmental coupling comes at the expense of slow quantum gate operations, which should be as fast as possible for many…

Quantum Physics · Physics 2022-11-11 R. M. Goldblatt , A. M. Martin , A. A. Wood

The negatively charged nitrogen-vacancy (NV) center in diamond is a leading solid-state quantum emitter, offering spin-photon interfaces over a wide temperature range with applications from electromagnetic sensing to bioimaging. While NV…

Magnetic Resonance Imaging (MRI) can characterize and discriminate among tissues using their diverse physical and biochemical properties. Unfortunately, submicrometer screening of biological specimens is presently not possible, mainly due…

Mesoscale and Nanoscale Physics · Physics 2010-11-03 C. A. Meriles , L. Jiang , G. Goldstein , J. S. Hodges , J. R. Maze , M. D. Lukin , P. Cappellaro

The negatively-charged nitrogen-vacancy (NV) center in diamond has been shown recently as an excellent sensor for external spins. Nevertheless, their optimum engineering in the near-surface region still requires quantitative knowledge in…

Mesoscale and Nanoscale Physics · Physics 2016-03-08 F. Favaro de Oliveira , S. A. Momenzadeh , D. Antonov , J. Scharpf , C. Osterkamp , B. Naydenov , F. Jelezko , A. Denisenko , J. Wrachtrup

The ground state spin of the negatively charged nitrogen-vacancy center in diamond has been the platform for the recent rapid expansion of new frontiers in quantum metrology and solid state quantum information processing. In ambient…

Materials Science · Physics 2012-06-05 M. W. Doherty , F. Dolde , H. Fedder , F. Jelezko , J. Wrachtrup , N. B. Manson , L. C. L. Hollenberg

The detection of a nuclear spin in an individual molecule represents a key challenge in physics and biology whose solution has been pursued for many years. The small magnetic moment of a single nucleus and the unavoidable environmental…

Quantum Physics · Physics 2015-03-19 Jianming Cai , Fedor Jelezko , Martin B. Plenio , Alex Retzker

Magnetic resonance techniques provide a powerful tool for controlling spin systems, with applications ranging from quantum information processing to medical imaging. Nevertheless, the behavior of a spin system under strong excitation…

Quantum Physics · Physics 2015-05-19 Lilian Childress , Jean McIntyre

High-spin defect centers in crystal matrices are used in quantum computing technologies, highly sensitive sensors, and single-photon sources. In this work, optically active nitrogen-vacancy color centers NV in a 28Si-enriched (nuclear spin…

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