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We report on the muon spin rotation/relaxation study of a pyrochlore oxide, Cd2Os2O7, which exhibits a metal-insulator (MI) transition at T_{MI}~225 K without structural phase transition. It reveals strong spin fluctuation (>10^8/s) below…

Strongly Correlated Electrons · Physics 2009-11-13 A. Koda , R. Kadono , K. Ohishi , S. R. Saha , W. Higemoto , S. Yonezawa , Y. Muraoka , Z. Hiroi

Sr$_2$IrO$_4$ is a weak ferromagnet where the spin arrangement is canted anti-ferromagnetic (AF). Moreover, the spin-structure coupling plays and important role in magnetic behavior of Sr$_2$IrO$_4$. In this concern the magnetization under…

Strongly Correlated Electrons · Physics 2019-04-19 Imtiaz Noor Bhatti , A. K. Pramanik

Neutron powder diffraction and inelastic measurements were performed examining the 5d pyrochlore Y$_2$Ir$_2$O$_7$. Temperature dependent measurements were performed between 3.4 K and 290 K, spanning the magnetic transition at 155 K. No sign…

Strongly Correlated Electrons · Physics 2014-05-30 M. C. Shapiro , S. C. Riggs , M. B. Stone , C. R. de la Cruz , S. Chi , A. A. Podlesnyak , I. R. Fisher

The bilayered rhodium oxide Sr3Rh2O7 was synthesized by high-pressure and high-temperature heating techniques. The single-phase polycrystalline sample of Sr3Rh2O7 was characterized by measurements of magnetic susceptibility, electrical…

Superconductivity · Physics 2009-11-07 K. Yamaura , Q. Huang , D. P. Young , Y. Noguchi , E. Takayama-Muromachi

Pyrochlore iridates have recently attracted growing interest in condensed matter physics because of their potential for realizing new topological states. In order to achieve such quantum states, it is essential to understand themagnetic…

Strongly Correlated Electrons · Physics 2015-01-06 W. K. Zhu , M. Wang , B. Seradjeh , Fengyuan Yang , S. X. Zhang

The lanthanide pyrochlore oxides Ln$_2$B$_2$O$_7$ are one of the most intensely studied classes of materials within condensed matter physics, firmly centered as one of the pillars of frustrated magnetism. The extensive chemical diversity of…

Strongly Correlated Electrons · Physics 2022-11-02 Brenden R. Ortiz , Paul M. Sarte , Ganesh Pokharel , Michael Garcia , Marcos Marmolejo , Stephen D. Wilson

Iridium-based 5d transition-metal oxides are attractive candidates for the study of correlated electronic states due to the interplay of enhanced crystal-field, Coulomb and spin-orbit interaction energies. At ambient pressure, these…

Strongly Correlated Electrons · Physics 2014-06-05 D. A. Zocco , J. J. Hamlin , B. D. White , B. J. Kim , J. R. Jeffries , S. T. Weir , Y. K. Vohra , J. W. Allen , M. B. Maple

Magnetic pyrochlores with non-Kramers rare-earth ions provide a platform for exploring emergent gauge physics and quantum spin-ice behavior, yet the influence of structural disorder on their ground states remains insufficiently understood.…

A new series of cubic double perovskites Ba$_2R_{2/3}$TeO$_6$ ($R$ = Y, La, Pr, Nd, Sm-Lu) was synthesized via solid state reaction. The $R^{3+}$ and Te$^{6+}$ ions are ordered on alternating octahedral sites, with the rare earth sites 2/3…

Materials Science · Physics 2019-03-14 Tai Kong , Robert J. Cava

We report Resonant Inelastic X-ray Scattering (RIXS) study of the magnetic excitation spectrum in a highly insulating Eu$_{2}$Ir$_{2}$O$_{7}$ single crystal that exhibits a metal-insulator transition at $T_{MI}$ = 111(7) K. A propagating…

Strongly Correlated Electrons · Physics 2018-06-13 Sae Hwan Chun , Bo Yuan , Diego Casa , Jungho Kim , Chang-Yong Kim , Zhaoming Tian , Yang Qiu , Satoru Nakatsuji , Young-June Kim

Over the past two decades, the magnetic ground states of all rare earth titanate pyrochlores have been extensively studied, with the exception of Sm$_2$Ti$_2$O$_7$. This is, in large part, due to the very high absorption cross-section of…

The recently synthesized first 4d transition-metal oxide-hydride LaSr3NiRuO4H4 with the unusual high H:O ratio surprisingly displays no magnetic order down to 1.8 K. This is in sharp contrast to the similar unusual low-valent Ni+ - Ru2+…

Strongly Correlated Electrons · Physics 2019-06-21 Xuan Wen , Ke Yang , Hua Wu

The Tb$_2$Ti$_2$O$_7$ pyrochlore magnetic material is attracting much attention for its {\em spin liquid} state, failing to develop long range order down to 50 mK despite a Curie-Weiss temperature $\theta_{\rm CW} \sim -14$ K. In this paper…

Statistical Mechanics · Physics 2007-05-23 Hamid R. Molavian , Michel J. P. Gingras , Benjamin Canals

We investigate the bilayer Ruddlesden-Popper iridate Sr$_3$Ir$_2$O$_7$ by temperature-dependent angle-resolved photoemission. We find a narrow-gap correlated insulator, with spectral features indicative of a polaronic ground state,…

Strongly Correlated Electrons · Physics 2013-07-01 P. D. C. King , T. Takayama , A. Tamai , E. Rozbicki , S. McKeown Walker , M. Shi , L. Patthey , R. G. Moore , D. Lu , K. M. Shen , H. Takagi , F. Baumberger

Contrary to the well known spin qubits, rare-earth qubits are characterized by a strong influence of crystal field due to large spin-orbit coupling. At low temperature and in the presence of resonance microwaves, it is the magnetic moment…

Strongly Correlated Electrons · Physics 2009-11-26 Sylvain Bertaina , J. H. Shim , S. Gambarelli , B. Z. Malkin , B. Barbara

Single crystals of a novel ruthenate, Ca2Ru2O7, were obtained. An X-ray diffraction study on a single crystal revealed that this material crystallizes in a pyrochlore structure with a lattice parameter, a = 10.197 Angstroms. The magnetic…

Materials Science · Physics 2009-11-11 Taiya Munenaka , Hirohiko Sato

Polycrystalline and single crystal samples of the insulating Shastry-Sutherland compound Er$_2$Be$_2$SiO$_7$ were synthesized via a solid-state reaction and the floating zone method respectively. The crystal structure, Er single ion…

Strongly Correlated Electrons · Physics 2024-05-15 A. Brassington , 1 Q. Ma , G. Sala , A. I. Kolesnikov , K. M. Taddei , Y. Wu , E. S Choi , H. Wang , W. Xie , J. Ma , H. D. Zhou , A. A. Aczel

The 6H-perovskite Ba3RRu2O9 (R = rare-earth), composed of Ru2O9 dimers connected through RO6 octahedra, exhibits an intriguing variety of magnetic ground states, ranging from non-magnetic to ferromagnetic and antiferromagnetic, depending on…

Materials Science · Physics 2025-06-13 E. Kushwaha , G. Roy , A. M. dos Santos , M. Kumar , S. Ghosh , T. Heitmann , T. Basu

Effects of spin-orbit interactions in condensed matter are an important and rapidly evolving topic. Strong competition between spin-orbit, on-site Coulomb and crystalline electric field interactions in iridates drives exotic quantum states…

Strongly Correlated Electrons · Physics 2018-02-27 Gang Cao , Pedro Schlottmann

Insulating magnetic rare-earth pyrochlores related to spin ice host emergent bosonic monopolar spinons, which obey a magnetic analogue of quantum electrodynamics and may open a route to a magnetic analogue of electronics. However, the…

Materials Science · Physics 2019-02-20 Shigeki Onoda , Fumiyuki Ishii