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We report electron spin resonance (ESR) spectroscopy results on the double perovskite Ba$_2$YIrO$_6$. On general grounds, this material is expected to be nonmagnetic due to the strong coupling of the spin and orbital momenta of Ir$^{5+}$…

Strongly Correlated Electrons · Physics 2018-06-12 S. Fuchs , T. Dey , G. Aslan-Cansever , A. Maljuk , S. Wurmehl , B. Büchner , V. Kataev

The electrical resistivity, magnetic susceptibility, and heat capacity of sintered samples of Ca2Ir2O7, in which pentavalent Ir atoms with 5d4 electron configuration form a pyrochlore structure, have been studied. The obtained experimental…

Strongly Correlated Electrons · Physics 2022-11-18 Yuki Nakayama , Yoshihiko Okamoto , Daigorou Hirai , Koshi Takenaka

The very nature of the ground state of the pyrochlore compound Yb$_2$Ti$_2$O$_7$ is much debated, as experimental results demonstrate evidence for both a disordered or a long-range ordered ground state. Indeed, the delicate balance of…

Strongly Correlated Electrons · Physics 2014-05-13 E. Lhotel , S. R. Giblin , M. R. Lees , G. Balakrishnan , L. J. Chang , Y. Yasui

We perform a comparative magnetic study on two series of rare-earth (RE) based double perovskite iridates RE2BIrO6 (RE=Pr,Nd,Sm-Gd;B=Zn,Mg), which show Mott insulating state with tunable charge energy gap from ~330 meV to ~560 meV by…

Strongly Correlated Electrons · Physics 2020-06-19 Yuxia Gao , Zhaoming Tian , Longmeng Xu , Malik Ashtar , Zongtang Wan , Zhengcai Xia , Feng Yang , Songliu Yuan , Yuyan Han , Wei Tong

We report the synthesis of single crystals of a novel layered iridate Ba$_{21}$Ir$_9$O$_{43}$, and present the crystallographic, transport and magnetic properties of this material. The compound has a hexagonal structure with two iridium…

We report detailed measurements of the low temperature magnetic phase diagram of Er$_2$Ti$_2$O$_7$. Heat capacity and time-of-flight neutron scattering studies of single crystals, subject to magnetic fields applied along the…

Strongly Correlated Electrons · Physics 2012-07-16 J. P. C. Ruff , J. P. Clancy , A. Bourque , M. A. White , M. Ramazanoglu , J. S. Gardner , Y. Qiu , J. R. D. Copley , H. A. Dabkowska , B. D. Gaulin

Physical properties of a pyrohafnate compound Pr2Hf2O7 have been investigated by ac magnetic susceptibility \chi_ ac(T), dc magnetic susceptibility \chi(T), isothermal magnetization M(H) and heat capacity C_p(T) measurements on…

The nature of the low temperature ground state of the pyrochlore compound Tb2Ti2O7 remains a puzzling issue. Dynamic fluctuations and short-range correlations persist down to 50 mK, as evidenced by microscopic probes. In parallel,…

Strongly Correlated Electrons · Physics 2012-08-02 E. Lhotel , C. Paulsen , P. Dalmas de Réotier , A. Yaouanc , C. Marin , S. Vanishri

Sr2IrO4 is a magnetic insulator driven by spin-orbit interaction (SOI) whereas the isoelectronic and isostructural Sr2RhO4 is a paramagnetic metal. The contrasting ground states have been shown to result from the critical role of the strong…

Strongly Correlated Electrons · Physics 2012-09-07 T. F. Qi , O. B. Korneta , L. Li , K. Butrouna , V. S. Cao , Xiangang Wan , P. Schlottmann , R. K. Kaul , G. Cao

Transition metal oxides of the $4d$ and $5d$ block have recently become the targets of materials discovery, largely due to their strong spin-orbit coupling that can generate exotic magnetic and electronic states. Here we report the high…

We report an analysis of neutron diffraction from single crystals of the spin-liquid pyrochlore Tb2Ti2O7 under the application of magnetic fields along the crystallographic $[110]$ direction. Such a perturbation has been shown to destroy…

Strongly Correlated Electrons · Physics 2009-11-17 J. P. C. Ruff , B. D. Gaulin , K. C. Rule , J. S. Gardner

The Hall resistivity and magnetization have been investigated in the ferromagnetic state of the bilayered manganite La(2-2x)Sr(1+2x)Mn2O7 (x=0.36). The Hall resistivity shows an increase in both the ordinary and anomalous Hall coefficients…

Strongly Correlated Electrons · Physics 2009-11-11 Y. Hirobe , Y. Ashikawa , R. Kawasaki , K. Noda , D. Akahoshi , H. Kuwahara

We present here magnetization, specific heat and Raman studies on single-crystalline specimens of the first pyrochlore member $Sm_2Ti_2O_7$ of the rare-earth titanate series. Its analogous compound $Sm_2Zr_2O_7$ in the rare-earth zirconate…

Materials Science · Physics 2009-11-13 Surjeet Singh , Surajit Saha , S. K. Dhar , R. Suryanarayanan , A. K. Sood , A. Revcolevschi

The thermodynamic properties of the pyrochlore Yb2Ti2O7 material are calculated using the numericallinked-cluster (NLC) calculation method for an effective anisotropic-exchange spin-1/2 Hamiltonian with parameters recently determined by…

Strongly Correlated Electrons · Physics 2014-04-11 N. R. Hayre , K. A. Ross , R. Applegate , T. Lin , R. R. P. Singh B. D. Gaulin , M. J. P. Gingras

In the search for topological phases in correlated electron systems, iridium-based pyrochlores A2Ir2O7 -- materials with 5d transition-metal ions -- provide fertile grounds. Several novel topological states have been predicted but the…

Strongly Correlated Electrons · Physics 2015-10-21 Liviu Hozoi , H. Gretarsson , J. P. Clancy , B. -G. Jeon , B. Lee , K. H. Kim , V. Yushankhai , Peter Fulde , Young-June Kim , Jeroen van den Brink

We report structural and magnetic properties studies of large high quality single-crystals of the frustrated magnet, Nd$_2$Zr$_2$O$_7$. Powder x-ray diffraction analysis confirms that Nd$_2$Zr$_2$O$_7$ adopts the pyrochlore structure.…

Strongly Correlated Electrons · Physics 2015-05-18 M. Ciomaga Hatnean , M. R. Lees , O. A. Petrenko , D. S. Keeble , G. Balakrishnan , M. J. Gutmann , V. V. Klekovkina , B. Z. Malkin

The intrinsic noncollinear spin patterns in rare-earth pyrochlore are physically interesting, hosting many emergent properties, e.g. spin ice and monopole-type excitation. Recently, the magnetic monopole excitation of spin ice systems was…

Materials Science · Physics 2015-12-18 Lin Lin , Y. L. Xie , J. -J. Wen , Shuai Dong , Z. B. Yan , J. -M. Liu

The pyrochlore Ho2Ge2O7 is a new highly correlated spin ice material. Physical property measurements including x-ray diffraction, dc susceptibility and ac susceptibility, confirm that it shares the distinctive characteristics of other known…

Quantum magnets with significant bond-directional Ising interactions, so-called Kitaev materials, have attracted tremendous attention recently in the search for exotic spin liquid states. Here we present a comprehensive set of measurements…

We report measurements and analysis of magnetization, resistivity and thermopower of polycrystalline samples of the perovskite-type Co/Rh oxide La$_{0.8}$Sr$_{0.2}$Co$_{1-x}$Rh$_x$O$_{3-\delta}$. This system constitutes a solid solution for…

Strongly Correlated Electrons · Physics 2015-05-19 S. Shibasaki , I. Terasaki , E. Nishibori , H. Sawa , J. Lybeck , H. Yamauchi , M. Karppinen
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