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We report about the dephasing of the spins states in a Garnet film excited by femtosecond laser pulses. It is shown that magneto-optical four-wave-mixing signals are efficiently generated and controlled with an external static magnetic…

Mesoscale and Nanoscale Physics · Physics 2013-11-05 M. Barthelemy , M. Vomir , M. Sanches Piaia , H. Vonesch , P. Molho , B. Barbara , J. -Y. Bigot

Laser radiation incident on a ferromagnetic sample produces excited electrons and currents whose spin polarization must not be aligned with the magnetization -- an effect due to spin-orbit coupling that is ubiquitous in spin- and…

Materials Science · Physics 2023-11-03 Oliver Busch , Franziska Ziolkowski , Ingrid Mertig , Jürgen Henk

Femtosecond magneto-optical pump-probe measurements of ultrafast demagnetization show an intriguing difference in the first 100 fs of the magneto-optical Kerr response depending on whether the polarization of the pump and probe beams are in…

Materials Science · Physics 2018-04-06 Ritwik Mondal , Marco Berritta , Peter M. Oppeneer

Understanding spin dynamics on femto- and picosecond timescales offers new opportunities for faster and more efficient spintronic devices. Here, we experimentally investigate the coherent spin dynamics after ultrashort laser excitation by…

Mesoscale and Nanoscale Physics · Physics 2024-01-26 Anulekha De , Akira Lentfert , Laura Scheuer , Benjamin Stadtmüller , Georg von Freymann , Martin Aeschlimann , Philipp Pirro

Since the beginning of femtomagnetism, it has been hotly debated how an ultrafast laser pulse can demagnetize a sample and switch its spins within a few hundred femtoseconds, but no consensus has been reached. In this paper, we propose that…

Materials Science · Physics 2015-06-22 G. P. Zhang , Mingqiang Gu , X. S. Wu

A new approach to all-optical detection and control of the coupling between electric and magnetic order on ultrafast timescales is achieved using time-resolved second harmonic generation (SHG) to study a ferroelectric (FE)/ferromagnet (FM)…

Materials Science · Physics 2015-01-12 Y. M. Sheu , S. A. Trugman , L. Yan , Q. X. Jia , A. J. Taylor , R. P. Prasankumar

Femtosecond laser excitation of materials that exhibit magnetic spin textures promises advanced magnetic control via the generation of ultrafast and non-equilibrium spin dynamics. We explore such possibilities in ferrimagnetic [Fe(0.35…

Exchange interactions determine the correlations between microscopic spins in magnetic materials. Probing the dynamics of these spin correlations on ultrashort length and time scales is, however rather challenging, since it requires…

Strongly Correlated Electrons · Physics 2023-05-02 Anatolii E. Fedianin , Alexandra M. Kalashnikova , Johan H. Mentink

Nonlinear spin motion in ferromagnets is considered with nonlinearity due to three factors: (i) the sample is prepared in a strongly nonequilibrium state, so that evolution equations cannot be linearized as would be admissible for spin…

Condensed Matter · Physics 2009-10-31 V. I. Yukalov , M. G. Cottam , M. R. Singh

We report on coherent control of excitation processes of translationally ultracold rubidium dimers in a magneto-optical trap by using shaped femtosecond laser pulses. Evolution strategies are applied in a feedback loop in order to optimize…

Coherent interactions between spins in quantum dots are a key requirement for quantum gates. We have performed pump-probe experiments in which pulsed lasers emitting at different photon energies manipulate two distinct subsets of electron…

Mesoscale and Nanoscale Physics · Physics 2011-10-03 S. Spatzek , A. Greilich , Sophia E. Economou , A. Schwan , S. Varwig , D. R. Yakovlev , D. Reuter , A. D. Wieck , T. L. Reinecke , M. Bayer

The dynamics of single laser-driven electrons and many particle systems with spin are investigated on the basis of a classical theory. We demonstrate that the spin forces can alter the electron dynamics in an ultra-relativistic laser field…

Plasma Physics · Physics 2014-06-17 Meng Wen , Heiko Bauke , Christoph H. Keitel

The ultrafast response to an optical pulse excitation of the spin-spin exchange interaction in transition metal anti-ferromagnets is studied within the framework of the time-dependent spin-density functional theory. We propose a formulation…

Mesoscale and Nanoscale Physics · Physics 2017-08-16 Jacopo Simoni , Maria Stamenova , Stefano Sanvito

We consider strongly interacting systems of effective spins, subject to dissipative spin-flip processes associated with optical pumping. We predict the existence of novel magnetic phases in the steady-state of this system, which emerge due…

Quantum Gases · Physics 2013-06-21 Tony E. Lee , Sarang Gopalakrishnan , Mikhail D. Lukin

Ultrafast laser pulses provide unique tools to manipulate magnetization dynamics at femtosecond timescales, where the interaction of the electric field -- such as excitation of spin carriers to non-equilibrium states, generation of…

In past decades, ultrafast spin dynamics in magnetic systems have been associated with heat deposition from high energy laser pulses, limiting the selective access to spin order. Here we use a long wavelength terahertz pump optical probe…

Materials Science · Physics 2021-06-04 Hovan Lee , Cedric Weber , Manfred Fähnle , Mostafa Shalaby

The spin dynamics in Ni is studied by an exact diagonalization method on the ultrafast time scale. It is shown that the femtosecond relaxation of the magneto-optical response results from exchange interaction and spin-orbit coupling. Each…

Materials Science · Physics 2009-10-30 W. Hubner , G. P. Zhang

In the field of femtomagnetism magnetic matter is controlled by ultrafast laser pulses; here we show that coupling phonon excitations of the nuclei to spin and charge leads to femto-phono-magnetism, a powerful route to control magnetic…

Materials Science · Physics 2022-03-29 S. Sharma , S. Shallcross , P. Elliott , J. K. Dewhurst

The impulsive generation of two-magnon modes in antiferromagnets by femtosecond optical pulses, so-called femto-nanomagnons, leads to coherent longitudinal oscillations of the antiferromagnetic order parameter that cannot be described by a…

Mesoscale and Nanoscale Physics · Physics 2019-07-31 D. Bossini , S. Dal Conte , O. Gomonay , R. V. Pisarev , M. Borovsak , D. Mihailovic , J. Sinova , G. Cerullo , J. H. Mentink , Th. Rasing , A. V. Kimel

Electron spins in quantum dots under coherent control exhibit a number of novel feedback processes. Here, we present experimental and theoretical evidence of a feedback process between nuclear spins and a single electron spin in a single…

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