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We describe a pump-probe scheme with which the spatial asymmetry of dissociating molecular fragments --- as controlled by the carrier-envelope phase of an intense few-cycle laser pulse --- can be enhanced by an order of magnitude or more.…

Quantum Physics · Physics 2013-07-03 Fatima Anis , B. D. Esry

A theory is developed for the evolution of the non-equilibrium distribution of quasiparticles when the scattering rate decreases due to particle collisions. We propose a "modified one-collision approximation" which is most effective for…

Disordered Systems and Neural Networks · Physics 2009-11-10 R. N. Gurzhi , A. I. Kopeliovich , A. N. Kalinenko , A. V. Yanovsky , E. N. Bogachek , Uzi Landman , H. Buhmann , L. W. Molenkamp

Shaping electron beams with the cycles of light provides femtosecond and attosecond time resolution in electron microscopy and enables fundamental quantum-coherent measurements. However, efficient light-electron control requires a prolonged…

We analyze a model problem representing a multi-electronic molecule sitting on a metal surface. Working with a reduced configuration interaction Hamiltonian, we show that one can extract very accurate ground state wavefunctions as compared…

Chemical Physics · Physics 2020-09-24 Junhan Chen , Zuxin Jin , Wenjie Dou , Joseph Subotnik

Different electron acceleration regimes in the evanescent field of a surface plasma wave are studied by considering the interaction of a test electron with the high-frequency electromagnetic field of a surface wave. The non-relativistic and…

Plasma Physics · Physics 2015-06-30 C. Riconda , M. Raynaud , T. Vialis , M. Grech

In this work we present a new method of approximating the continuum wavefunctions with a discrete basis set. This method aims to be at least compatible with other well known methods of the electronic structure theory to describe processes…

Chemical Physics · Physics 2019-09-18 Mateusz S. Szczygieł , Michał Lesiuk , Robert Moszynski

The tunability and spatial precision of paramagnetic molecules makes them attractive for quantum sensing. However, usual microwave-based detection methods have poor temporal and spatial resolution, and optical methods compatible with…

Quantum Physics · Physics 2024-07-30 Erica Sutcliffe , Nathanael P. Kazmierczak , Ryan G. Hadt

Distributed linear control design is crucial for large-scale cyber-physical systems. It is generally desirable to both impose information exchange (communication) constraints on the distributed controller, and to limit the propagation of…

Systems and Control · Electrical Eng. & Systems 2021-03-31 Jing Yu , Yuh-Shyang Wang , James Anderson

Complex and correlated quantum systems with promise for new functionality often involve entwined electronic degrees of freedom. In such materials, highly unusual properties emerge and could be the result of electron localization. Here, a…

Strongly correlated solids are extremely complex and fascinating quantum systems, where new states continue to emerge, especially when interaction with light triggers interplay between them. In this interplay, sub-laser-cycle electron…

Strongly Correlated Electrons · Physics 2023-03-13 V. Valmispild , E. Gorelov , M. Eckstein , A. Lichtenstein , H. Aoki , M. Katsnelson , M. Ivanov , O. Smirnova

We propose a laser-based method for the preparation of high-energy polarized electrons, from the ionization of isolated spin-polarized hydrogen (SPH) atoms. The SPH atoms are prepared from the photodissociation of HCl, using two consecutive…

High-harmonic spectroscopy (HHS) is a nonlinear all-optical technique with inherent attosecond temporal resolution, which has been applied successfully to a broad variety of systems in the gas phase and solid state. Here, we extend HHS to…

Here, we investigate the physical mechanisms that may enable squeezing a complex electromagnetic field distribution through a narrow and/or partially obstructed region with little amplitude and phase distortions. Following our recent works,…

Materials Science · Physics 2015-06-03 Mario G. Silveirinha , Nader Engheta

Quantum hydrodynamic (QHD) model of charged spin-1/2 particles contains physical quantities defined for all particles of a species including particles with spin-up and with spin-down. Different population of states with different spin…

Plasma Physics · Physics 2015-04-01 Pavel A. Andreev

Plane-wave electrons undergo momentum transfer as they scatter off a target in overlapping spherical waves. The transferred momentum leads to target structural information to be encoded in angle and energy differential scattering. For…

Atomic and Molecular Clusters · Physics 2024-02-14 Aiswarya R. , Rasheed Shaik , Jobin Jose , Hari R. Varma , Himadri S. Chakraborty

A scheme to characterize the dynamics of the electron beam-electromagnetic power exchange along a traveling wave tube (TWT) is proposed. The method is based on defining a state vector at discrete periodic locations along the TWT and…

Plasma Physics · Physics 2021-03-05 Tarek Mealy , Filippo Capolino

A spin-wave (SW) approach for hard-core bosons is presented to treat the problem of two dimensional boson localization in a random potential. After a short review of the method to compute 1/S-corrected observables, the case of random…

Strongly Correlated Electrons · Physics 2014-12-04 Juan Pablo Álvarez Zúñiga , Gabriel Lemarié , Nicolas Laflorencie

We propose a novel probe technique capable of performing local low-temperature spectroscopy on a 2D electron system (2DES) in a semiconductor heterostructure. Motivated by predicted spatially-structured electron phases, the probe uses a…

Mesoscale and Nanoscale Physics · Physics 2011-01-06 Adam Sciambi , Matthew Pelliccione , Seth R. Bank , Arthur C. Gossard , David Goldhaber-Gordon

Electron energy loss spectroscopy is consolidating as a powerful tool to explore electronic (as well as vibrational) excitations of matter, including molecules. Performed in a scanning transmission electron microscope, this technique is…

Chemical Physics · Physics 2021-03-05 Ciro A. Guido , Enzo Rotunno , Matteo Zanfrognini , Stefano Corni , Vincenzo Grillo

A new simulation box setup is introduced for the precise description of the wavepacket evolution of two electronic systems in intense laser pulses. In this box, the regions of the hydrogen molecule H$_{2} $, and singly and doubly ionized…

Atomic Physics · Physics 2016-03-03 Mohsen Vafaee , Firoozeh Sami , Babak Shokri , Behnaz Buzari , Hassan Sabzyan