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We have investigated the magnetic properties of CuNCN, the first nitrogen-based analogue of cupric oxide, CuO. Our muon spin relaxation, nuclear magnetic resonance and electron spin resonance studies reveal that classical magnetic ordering…

Strongly Correlated Electrons · Physics 2011-07-26 A. Zorko , P. Jeglič , A. Potočnik , D. Arčon , A. Balčytis , Z. Jagličić , X. Liu , A. L. Tchougréeff , R. Dronskowski

Copper carbodiimide, CuNCN, is a geometrically frustrated nitrogen-based analogue of cupric oxide, whose magnetism remains ambiguous. Here, we employ a combination of local-probe techniques, including $^{63,\, 65}$Cu nuclear quadrupole…

Strongly Correlated Electrons · Physics 2018-07-03 A. Zorko , P. Jeglič , M. Pregelj , D. Arčon , H. Luetkens , A. L. Tchougréeff , R. Dronskowski

We show that short-range resonating-valence-bond correlations and long-range order can coexist in the ground state (GS) of a frustrated spin system. Our study comprises a comprehensive investigation of the quantum magnetism on the…

Strongly Correlated Electrons · Physics 2022-08-16 Long Yuan , Yuqian Zhao , Boqiang Li , Yiru Song , Yuanhua Xia , Benqiong Liu , Junfeng Wang , Yuesheng Li

New physics can emerge in magnetic materials where quantum fluctuations are enhanced due to reduced dimensionality and strong frustration. One long sought example is the resonating-valence-bond (RVB) state, where atomic magnetic moments are…

Strongly Correlated Electrons · Physics 2013-07-19 Tian-Heng Han , Joel S. Helton , Shaoyan Chu , Daniel G. Nocera , Jose A. Rodriguez-Rivera , Collin Broholm , Young S. Lee

The prospect of merging the paradigms of geometric frustration on a triangular lattice and bond anisotropies in the strong spin-orbit coupling limit holds tremendous promise in the ongoing hunt for exotic quantum materials. Here we identify…

We propose a new form of the frustrated Heisenberg antiferromagnetic Hamiltonian with spatially anisotropic exchange parameters Jc, Ja, and Jac extended along the c, a, and a +/- c lattice directions and apply it to describe fascinating…

Strongly Correlated Electrons · Physics 2013-04-10 A. L. Tchougréeff , R. Dronskowski

Inelastic neutron scattering provides a powerful probe of the magnetic excitations of quantum magnets. Altermagnets have recently emerged as a new class of magnets with vanishing net magnetization characteristic of antiferromagnets and with…

Strongly Correlated Electrons · Physics 2023-09-29 Thomas A. Maier , Satoshi Okamoto

The topology of the magnetic interactions of the copper spins in the nitrosonium nitratocuprate (NO)[Cu(NO3)3] suggests that it could be a realization of the Nersesyan-Tsvelik model, whose ground state was argued to be either a resonating…

Strongly Correlated Electrons · Physics 2015-05-18 O. Volkova , I. Morozov , V. Shutov , E. Lapsheva , P. Sindzingre , O. Cepas , M. Yehia , V. Kataev , R. Klingeler , B. Büchner , A. Vasiliev

We have investigated magnetic properties of Rb$_2$Cu$_2$Mo$_3$O$_{12}$ powder. Temperature dependence of magnetic susceptibility and magnetic-field dependence of magnetization have shown that this cuprate is a model compound of a…

Other Condensed Matter · Physics 2009-11-10 Masashi Hase , Haruhiko Kuroe , Kiyoshi Ozawa , Osamu Suzuki , Hideaki Kitazawa , Giyuu Kido , Tomoyuki Sekine

We use Schwinger boson mean field theory to study the antiferromagnetic spin-1/2 Heisenberg model on an anisotropic triangular lattice in the presence of a uniform external magnetic field. We calculate the field dependence of the spin…

Strongly Correlated Electrons · Physics 2009-11-07 S. Q. Shen , F. C. Zhang

In this work, a long-range resonating valence bond state is proposed as a variational wave function for the ground state of the $S=1/2$ antiferromagnetic Heisenberg model on the honeycomb lattice. Employing Variational Monte Carlo (VMC)…

Strongly Correlated Electrons · Physics 2009-05-06 Zahra Nourbakhsh , Farhad Shahbazi , S. A. Jafari , G. Baskaran

We report magnetization, nuclear magnetic resonance (NMR), nuclear quadrupole resonance (NQR), and transmission electron microscopy (TEM) studies on the quasi-two-dimensional spin-gap system (CuCl)LaNb2O7, a possible candidate for the J1-J2…

Strongly Correlated Electrons · Physics 2017-12-01 M. Yoshida , N. Ogata , M. Takigawa , J. Yamaura , M. Ichihara , T. Kitano , H. Kageyama , Y. Ajiro , K. Yoshimura

The frustrated magnet clinoatacamite, $\gamma$-Cu$_2$(OH)$_3$Cl, is attracting a lot of interest after suggestions that at low temperature it forms an exotic quantum state termed a Valence Bond Solid (VBS) made from dimerised Cu$^{2+}$…

Strongly Correlated Electrons · Physics 2009-07-08 A. S. Wills , T. G. Perring , S. Raymond , B. Fak , J. -Y. Henry , M. Telling

Rare-earth triangular-lattice magnets serve as an excellent platform for investigating exotic quantum magnetic phenomena. Recently, the hexaaluminate \cmao\ has been proposed to host a $U(1)$ Dirac quantum spin liquid state with dominant…

Strongly Correlated Electrons · Physics 2025-07-16 Yantao Cao , Huanpeng Bu , Toni Shiroka , Helen C. Walker , Zhendong Fu , Zhaoming Tian , Jinkui Zhao , Hanjie Guo

The spin-1/2 Heisenberg model on the pyrochlore lattice is an iconic frustrated three-dimensional spin system with a rich phase diagram. Besides hosting several ordered phases, the model is debated to possess a spin-liquid ground state when…

Strongly Correlated Electrons · Physics 2021-11-16 Nikita Astrakhantsev , Tom Westerhout , Apoorv Tiwari , Kenny Choo , Ao Chen , Mark H. Fischer , Giuseppe Carleo , Titus Neupert

Inhomogeneity in the ground state is an intriguing, emergent phenomenon in magnetism. Recently, it has been observed in the magnetostructural channel of the geometrically frustrated $\alpha$-NaMnO$_2$, for the first time in the absence of…

Strongly Correlated Electrons · Physics 2015-03-20 A. Zorko , J. Kokalj , M. Komelj , O. Adamopoulos , H. Luetkens , D. Arčon , A. Lappas

The ground state of an S=1/2 antiferromagnetic Heisenberg model on a spatially anisotropic triangular lattice, which is an effective model of Mott insulators on a triangular layer of organic charge transfer salts or Cs2CuCl4, is numerically…

Strongly Correlated Electrons · Physics 2012-11-19 Kenji Harada

We consider the exchange couplings present in an effective Hamiltonian of $\alpha$-RuCl$_3$, known as the K-$\Gamma$ model. This material has a honeycomb lattice, and is expected to be a representative of the Kitaev materials (which can…

Strongly Correlated Electrons · Physics 2022-04-19 Ipsita Mandal

A three-dimensional system of interacting spins typically develops static long-range order when it is cooled. If the spins are quantum (S = 1/2), however, novel quantum paramagnetic states may appear. The most highly sought state among them…

Strongly Correlated Electrons · Physics 2015-05-13 S. -H. Lee , H. Kikuchi , Y. Qiu , B. Lake , Q. Huang , K. Habicht , K. Kiefer

We report the magnetic properties in the Co- and Zn-doped spin-1/2 honeycomb-lattice compound In$_3$Cu$_2$VO$_9$. The magnetic susceptibility and specific heat experiments show no long-range ordering down to 2 K in In$_3$Cu$_2$VO$_9$. In…

Strongly Correlated Electrons · Physics 2012-06-05 Y. J. Yan , Z. Y. Li , T. Zhang , X. G. Luo , G. J. Ye , Z. J. Xiang , P. Cheng , Liang-Jian Zou , X. H. Chen
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