English
Related papers

Related papers: Multiphoton Dissociation of HeH+ below the He+(1s)…

200 papers

The laser-induced fragmentation dynamics of this most fundamental polar molecule HeH$^+$ are measured using an ion beam of helium hydride and an isotopologue at various wavelengths and intensities. In contrast to the prevailing…

Chemical Physics · Physics 2018-08-21 P. Wustelt , F. Oppermann , Lun Yue , M. Möller , T. Stöhlker , S. Gräfe , M. Lein , G. G. Paulus , A. M. Sayler

We present a study of multiphoton dissociative ionization from molecules. By solving the time-dependent Schr\"{o}dinger equation for H$_2^+$ and projecting the solution onto double continuum scattering states, we observe the correlated…

Atomic Physics · Physics 2012-07-03 C B Madsen , F Anis , L B Madsen , B D Esry

Multiphoton ionization of helium is investigated in the superintense field regime, with particular emphasis on the role of the electron-electron interaction in the ionization and stabilization dynamics. To accomplish this, we solve ab…

Quantum Physics · Physics 2015-05-27 S. A. Sørngård , S. Askeland , R. Nepstad , M. Førre

The electron localization in the dissociation of the asymmetric charged molecular ion HeH$^{2+}$ exposed to an intense few-cycle laser pulse is studied by solving numerically the 3D time-dependent Schr\"odinger equation. By varying the…

Atomic Physics · Physics 2011-10-05 Kunlong Liu , Weiyi Hong , Peixiang Lu

We investigate dissociative single and double ionization of HeH+ induced by intense femtosecond laser pulses. By employing a semi-classical model with nuclear trajectories moving on field-dressed surfaces and ionization events treated as…

Atomic Physics · Physics 2018-10-24 Lun Yue , Philipp Wustelt , A. Max Sayler , Gerhard G. Paulus , Stefanie Gräfe

When a chemical bond is broken, the molecular structure undergoes a transformation. An ideal experiment should probe the change in the electronic and nuclear structure simultaneously. Here, we present a method for the simultaneous…

Atomic Physics · Physics 2024-10-11 Saurabh Mhatre , Zack Dube , André Staudte , Stefanie Gräfe , Matthias Kübel

The photodissociation of the HD+ molecular ion in intense short- pulsed linearly polarized laser fields is studied using a time- dependent wave-packet approach where molecular rotation is fully included. We show that applying a coherent…

chem-ph · Physics 2019-04-04 Eric Charron , Annick Giusti-Suzor , Frederick Mies

We study the breakup of $\text{H}_2^+$ exposed to super-intense, femtosecond laser pulses with frequencies greater than that corresponding to the ionization potential. By solving the time-dependent Schr\"odinger equation in an extensive…

Atomic Physics · Physics 2016-04-12 Lun Yue , Lars Bojer Madsen

Fully numerical mesh solutions of 2D and 3D quantum equations of Schroedinger and Hartree-Fock type allow us to work with wavefunctions which possess a very flexible geometry. This flexibility is especially important for calculations of…

Atomic Physics · Physics 2007-05-23 Mikhail V. Ivanov

The full-dimensional time-dependent Schrodinger equation for the electronic dynamics of single-electron systems in intense external fields is solved directly using a discrete method. Our approach combines the finite-difference and Lagrange…

Atomic Physics · Physics 2009-11-10 Liang-You Peng , J F McCann , Daniel Dundas , K T Taylor , I D Williams

We study the dissociation of H$_2$$^+$ in uv laser pulses by solving the non-Born-Oppenheimer time-dependent Schr\"{o}dinger equation as a function of the photon energy $\omega$ of the pulse. Significant enhancements of the dissociation…

Atomic and Molecular Clusters · Physics 2014-07-22 Kunlong Liu , Qianguang Li , Pengfei Lan , Peixiang Lu

We study double ionization (DI) dynamics of vibrating HeH$^+$ versus its isotopic variant HeT$^+$ in strong laser fields numerically. Our simulations show that for both cases, these two electrons in DI prefer to release together along the…

Atomic Physics · Physics 2020-03-18 S. Wang , R. H. Xu , W. Y. Li , X. Liu , W. Li , G. G. Xin , Y. J. Chen

The dissociation spectrum of the hydrogen molecular ion by short intense pulses of infrared light is calculated. The time-dependent Schr\"odinger equation is discretized and integrated in position and momentum space. For few-cycle pulses…

Atomic Physics · Physics 2009-11-10 Liang-You Peng , I D Williams , J F McCann

A clear understanding of the mechanisms that control the electron dynamics in strong laser field is still a challenge that requires to be interpreted by advanced theory. Development of accurate theoretical and computational methods, able to…

Based on a combined quantum-classical treatment, a complete study of the strong field dynamics of H2+, i.e. including all nuclear and electronic DOF as well as dissociation and ionization, is presented. We find that the ro-vibrational…

Atomic and Molecular Clusters · Physics 2011-08-09 J. Handt , S. M. Krause , J. M. Rost , M. Fischer , F. Grossmann , R. Schmidt

The dissociative ionization of H2+ interacting with intense, femtosecond extreme-ultraviolet laser pulses is investigated theoretically. This is done by numerical propagation of the time-dependent Schr\"{o}dinger equation for a colinear…

Atomic Physics · Physics 2015-02-25 Lun Yue , Lars Bojer Madsen

A simple analytical solution for the problem of multiphoton detachment from negative ions by a linearly polarized laser field is found. It is valid in the wide range of intensities and frequencies of the field, from the perturbation theory…

Atomic Physics · Physics 2009-10-30 G. F. Gribakin , M. Yu. Kuchiev

We report the observation of above-threshold dissociation of a multielectron molecular system, Na$_2^+$. The process is due to continuum-continuum transitions in a field-dressed molecular continuum. Three well resolved fragmentation…

Chemical Physics · Physics 2008-08-24 Qun Zhang , John W. Hepburn , Moshe Shapiro

The temporal dynamics of double ionization of H2 has been investigated both experimentally and theoretically with few-cycle laser pulses. The main observables are the proton spectra associated to the H^+ + H^+ fragmentation channel. The…

Quantum Physics · Physics 2008-09-23 Sébastien Saugout , Eric Charron , Christian Cornaggia

We investigated the high-order harmonic generation (HHG) process of diatomic molecular ion $\mathrm{H}_2^+$ in non-Born-Oppenheimer approximations. The corresponding three-dimensional time-dependent Schr\"odinger equation is solved with…

Atomic Physics · Physics 2017-02-28 Mu-Zi Li , Guang-Rui Jia , Xue-Bin Bian
‹ Prev 1 2 3 10 Next ›