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Using density functional theory, we study the influence of hydrostatic pressure on the crystal structure of lanthanide monoxides, focusing on the monoxides formed by the fifteen elements of the lanthanide series, from La to Lu. Calculations…

Materials Science · Physics 2026-04-14 Sergio Ferrari , Daniel Errandonea

Applying pressure around megabar is indispensable in the synthesis of high-temperature superconducting hydrides, such as SH$_3$ and LaH$_{10}$. Stabilizing the high-pressure phase of hydride around ambient condition is a severe challenge.…

Superconductivity · Physics 2023-05-17 Miao Gao , Peng-Jie Guo , Huan-Cheng Yang , Xun-Wang Yan , Fengjie Ma , Zhong-Yi Lu , Tao Xiang , Hai-Qing Lin

High-temperature and high-pressure experiments were conducted on columbite-type ZnNb2O6, reaching temperatures up to 873 K at ambient pressure and pressures up to 30 GPa at ambient temperature, respectively. Through systematic analysis…

Two novel room-temperature phase transitions are observed, via synchrotron x-ray diffraction and Raman spectroscopy, in the Pb(Zr0.52Ti0.48)O3 alloy under hydrostatic pressures up to 16 GPa. A monoclinic (M)-to-rhombohedral (R1) phase…

Condensed Matter · Physics 2009-11-10 A. Sani , B. Noheda , I. A. Kornev , L. Bellaiche , P. Bouvier , J. Kreisel

The high-pressure and high-temperature thermodynamic properties of iridium are studied using density functional theory in combination with the quasi-harmonic approximation, where both the contributions to the free energy of phonons and of…

Materials Science · Physics 2024-01-24 Balaram Thakur , Xuejun Gong , Andrea Dal Corso

In comparison with the accurate data on the on-top electron density n(0) in the proton-embedded electron gas with the density parameter r_s in the range 1-12 obtained by diffusion Monte Carlo (DMC) simulations, we have successfully…

Materials Science · Physics 2018-07-18 Yasutami Takada

We report experimental evidence for pressure instabilities in the model multiferroic BiFeO3 and namely reveal two structural phase transitions around 3 GPa and 10 GPa by using diffraction and far-infrared spectroscopy at a synchrotron…

Materials Science · Physics 2011-07-26 R. Haumont , P. Bouvier , A. Pashkin , K. Rabia , S. Frank , B. Dkhil , W. A. Crichton , C. A. Kuntscher , J. Kreisel

A first-principles density-functional-theory method has been used to reinvestigate the mechanical and dynamical stability of the metallic phase of AlH3 between 65-110 GPa. The electronic properties and phonon dynamics as a function of…

Superconductivity · Physics 2015-05-18 A. K. M. A. Islam , M. M. Ali , M. L. Ali

We study the effects of hydrostatic pressure in the range 0.0--2.0 GPa on anion mobility in the orthorhombic $Pnma$ phase of CsPbBr$_{3}$. Using density functional theory and the climbing nudged elastic band method, we calculate the…

Materials Science · Physics 2021-07-14 Thijs J. A. M. Smolders , Alison B. Walker , Matthew J. Wolf

Neutron powder diffraction studies of the crystal and magnetic structures of the magnetocaloric compound Mn1.1Fe0.9(P0.8Ge0.2) have been carried out as a function of temperature, applied magnetic field, and pressure. The data reveal that…

Materials Science · Physics 2009-11-30 D. M. Liu , Q. Huang , M. Yue , J. W. Lynn , L. J. Liu , Y. Chen , Z. H. Wu , J. X. Zhang

Without the use of any empirical fitting to experimental or high-level ab initio data, we present a double-hybrid density functional approximation for the exchange-correlation energy, combining the exact Hartree-Fock exchange and…

Chemical Physics · Physics 2015-06-04 Jeng-Da Chai , Shan-Ping Mao

We study the temperature and pressure dependence of the structural and electronic properties of the iron pnictide superconductor BaFe2As2. We use density functional theory based Born-Oppenheimer molecular dynamics simulations to investigate…

Strongly Correlated Electrons · Physics 2013-08-06 Steffen Backes , Harald O. Jeschke

It has been well established that nitrogen coordinated transition metal, TM-N$_{4}$-C (TM$=$Fe and Co) moieties, are responsible for the higher catalytic activity for the electrochemical oxygen reduction reaction. However, the results…

Materials Science · Physics 2022-09-20 Azim Fitri Zainul Abidin , Ikutaro Hamada

Proton transport property is studied by modelling the intermolecular pair correlation functions of the proton ion with the electrode and the electrolyte of a polymer electrolyte fuel cell (PEMFC) by using Materials-Studio and then applying…

Materials Science · Physics 2023-05-05 S. S. Awulachew , K. N. Nigussa

The combination of spin transitions and magnetic ordering provides an interesting structure of phase transitions in Prussian blue analogues (PBAs). To understand the structure of stable and metastable states of Co-Fe PBA, it is necessary to…

Materials Science · Physics 2009-11-11 Y. Konishi , H. Tokoro , M. Nishino , S. Miyashita

First-principles calculations based on density functional theory have been widely used in studies of the structural, thermoelastic, rheological, and electronic properties of earth-forming materials. The exchange-correlation term, however,…

Computational Physics · Physics 2009-11-13 S. H. Lee , Jones T. K. Wan

Within the framework of a realistic multi-band p-d-model, we derived an effective Hamiltonian to describe the exchange interaction effects near the spin crossover in magnetic Mott-Hubbard insulators under pressure. It is shown that…

Strongly Correlated Electrons · Physics 2017-10-18 Alexander I. Nesterov , Yuri S. Orlov , Sergey G. Ovchinnikov , Sergey V. Nikolaev

High pressure behaviour of superhydrous phase B(HT) of Mg10Si3O14(OH)4 (Shy B) is investigated with the help of density functional theory based first principles calculations. In addition to the lattice parameters and equation of state, we…

Other Condensed Matter · Physics 2015-05-14 H. K. Poswal , Surinder M Sharma , S. K. Sikka

Density functional perturbation theory calculations of alpha-quartz using extended norm conserving pseudopotentials have been used to study the elastic properties and phonon dispersion relations along various high symmetry directions as a…

Materials Science · Physics 2007-05-23 N. Choudhury , S. L. Chaplot

Simultaneous high pressure x-ray diffraction and electrical resistance measurements have been carried out on a PbO type {\alpha}-FeSe0.92 compound to a pressure of 44 GPa and temperatures down to 4 K using designer diamond anvils at…