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We present a time-dependent density-functional method able to describe the photoelectron spectrum of atoms and molecules when excited by laser pulses. This computationally feasible scheme is based on a geometrical partitioning that…

Atomic Physics · Physics 2012-06-28 U. De Giovannini , D. Varsano , M. A. L. Marques , H. Appel , E. K. U. Gross , A. Rubio

Molecular absorption and photo-electron spectra can be efficiently predicted with real-time time-dependent density-functional theory (TDDFT). We show here how these techniques can be easily extended to study time-resolved pump-probe…

Atomic and Molecular Clusters · Physics 2013-01-10 Umberto De Giovannini , Gustavo Brunetto , Alberto Castro , Jessica Walkenhorst , Angel Rubio

Ultracold neutral plasmas exhibit a density-dependent resonant response to applied radio-frequency (RF) fields in the frequency range of several MHz to hundreds of MHz for achievable densities. We have conducted measurements where short…

Plasma Physics · Physics 2015-06-04 Truman Wilson , Wei-Ting Chen , Jacob Roberts

A laser-boosted relativistic solid-density paraboloidal foil is known to efficiently reflect and focus a counterpropagating laser pulse. Here we show that in the case of an ultrarelativistic counterpropagating pulse, a high-energy and…

Plasma Physics · Physics 2014-07-14 M. Tamburini , A. Di Piazza , T. V. Liseykina , C. H. Keitel

Based on the time-dependent density-functional theory, we have derived a rigorous formula for the stopping power of an {\it interacting} electron gas for ions in the limit of low projectile velocities. If dynamical correlation between…

Materials Science · Physics 2009-11-11 V. U. Nazarov , J. M. Pitarke , C. S. Kim , Y. Takada

It has been shown that the non-sinusoidal character oscillations appear in the transmitted, reflected and absorbed light fluxes when light pulses irradiate a semiconductor quantum well (QW), containing a set of a large number of the…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 I. G. Lang L. I. Korovin , D. A. Contreras-Solorio , S. T. Pavlov

The subject of this paper is the scattering of a very intense laser pulse (intensity $I\sim10^{21}\;{\mathrm{W/cm^2}}$) on relativistic electrons with Lorentz factor between 10 and 45. The laser pulse is modeled by a plane wave with finite…

Quantum Physics · Physics 2011-10-18 Madalina Boca , Andreea Oprea

We study the temperature-dependent optical properties of gold over a broad energy spectrum covering photon energies below and above the interband threshold. We apply a semi-analytical Drude-Lorentz model with temperature-dependent…

Materials Science · Physics 2024-04-26 P. D. Ndione , S. T. Weber , D. O. Gericke , B. Rethfeld

This dissertation explores the interaction between high-intensity lasers and plasmas to accelerate electrons and produce radiation via experimental and computational efforts. The laser pulses used in this dissertation have ultrashort…

Plasma Physics · Physics 2022-10-19 Jinpu Lin

A novel deflection effect of an intense laser beam with spin angular momentum is revealed theoretically by an analytical modeling using radiation pressure and momentum balance of laser plasma interaction in the relativistic regime, as a…

Plasma Physics · Physics 2019-12-16 Y. H. Tang , Z. Gong , J. Q. Yu , Y. R. Shou , X. Q. Yan

We investigate the two-pulse photon echo response of excitons in the mixed lead halide perovskite crystal \sample in dependence on the excitation intensity and polarization of the incident laser pulses. Using spectrally narrow picosecond…

The electric dipole (E1) strength functions have been systematically calculated based on the time-dependent density functional theory (TDDFT), using the finite amplitude method and the real-time approach to the TDDFT with pairing…

Nuclear Theory · Physics 2017-08-23 Shuichiro Ebata , Tsunenori Inakura , Takashi Nakatsukasa

We derive upper and lower bounds on the absorption of ultraintense laser light by solids as a function of fundamental laser and plasma parameters. These limits emerge naturally from constrained optimization techniques applied to a…

Plasma Physics · Physics 2013-11-19 M. C. Levy , S. C. Wilks , M. Tabak , S. B. Libby , M. G. Baring

The creation of well-thermalized, hot and dense plasmas is attractive for warm dense matter studies. We investigate collisionally induced energy absorption of an ultraintense and ultrashort laser pulse in a solid copper target using…

Plasma Physics · Physics 2020-04-29 Andréas Sundström , Laurent Gremillet , Evangelos Siminos , István Pusztai

The reflection and transmission of a few-cycle laser pulse impinging on two parallel thin metal layers have been analyzed. The two layers, with a thickness much smaller than the skin depth of the incoming radiation field, are represented by…

Classical Physics · Physics 2019-05-16 M. Polner , S. Varró , A. Vörös-Kiss

The particle-hole interaction problem is longstanding within time-dependent density functional theory (TDDFT) and leads to extreme errors in the prediction of K-edge X-ray absorption spectra (XAS). We derive a linear-response formalism that…

Chemical Physics · Physics 2022-10-18 Kevin Carter-Fenk , Leonardo A. Cunha , Juan E. Arias-Martinez , Martin Head-Gordon

By introducing the self-energy density functionals for the dissipative interactions between the reduced system and its environment, we develop a time-dependent density-functional theory formalism based on an equation of motion for the…

Quantum Physics · Physics 2009-11-13 Xiao Zheng , Fan Wang , Chi Yung Yam , Yan Mo , GuanHua Chen

The nonlinear optical dynamics of nano-materials comprised of plasmons interacting with quantum emitters is investigated by a self-consistent model based on the coupled Maxwell-Liouville-von Neumann equations. It is shown that ultra-short…

Mesoscale and Nanoscale Physics · Physics 2013-12-04 Maxim Sukharev , Tamar Seideman , Robert J. Gordon , Adi Salomon , Yehiam Prior

It was recently shown [Y. Suzuki, L. Lacombe, K. Watanabe, and N. T. Maitra, Phys. Rev. Lett. 119, 263401 (2017)] that peak and valley structures in the exact exchange-correlation potential of time-dependent density functional theory are…

Chemical Physics · Physics 2018-07-04 Lionel Lacombe , Yasumitsu Suzuki , Kazuyuki Watanabe , Neepa T. Maitra