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We present a neutron diffraction study of FeV2O4, which is rare in exhibiting spin and orbital degrees of freedom on both cation sublattices of the spinel structure. Our data confirm the existence of three structural phase transitions…

Strongly Correlated Electrons · Physics 2012-09-03 G. J. MacDougall , V. O. Garlea , A. A. Aczel , H. D. Zhou , S. E. Nagler

We report a ferroelectric order at ~ 98 K for NiFe2O4, which carries an inverse spinel structure with a centrosymmetric Fd3m structure at room temperature. The value of spontaneous electric polarization is considerably high as ~ 0.29…

Materials Science · Physics 2019-05-10 J. K. Dey , A. Chatterjee , S. Majumdar , A. -C. Dippel , O. Gutowski , M. v. Zimmermann , S. Giri

The lacunar spinel GeV4S8 undergoes orbital and ferroelectric ordering at the Jahn-Teller transition around 30 K and exhibits antiferromagnetic order below about 14 K. In addition to this orbitally driven ferroelectricity, lacunar spinels…

Strongly Correlated Electrons · Physics 2017-01-23 S. Widmann , A. Günther , E. Ruff , V. Tsurkan , H. -A. Krug von Nidda , P. Lunkenheimer , A. Loidl

Neutron and X-ray diffraction, magnetic susceptibility, and specific heat measurements have been used to investigate the magnetic and structural phase transitions of the spinel system Fe1+xCr2-xO4(0.0<=x<=1.0). The temperature versus Fe…

Spinel compounds AB$_{2}$X$_{4}$ consist of both tetrahedral (AX$_{4}$) and octahedral (BX$_{6}$) environments with the former forming a diamond lattice and the latter a geometrically frustrated pyrochlore lattice. Exploring the fascinating…

Chemical Physics · Physics 2023-03-29 Qiang Zhang , Wei Tian , Roshan K. Nepal , Ashfia Huq , Stephen Nagler , J. F. DiTusa , Rongying Jin

Neutron inelastic scattering and diffraction techniques have been used to study the MnV2O4 spinel system. Our measurements show the existence of two transitions to long-range ordered ferrimagnetic states; the first collinear and the second…

Strongly Correlated Electrons · Physics 2009-11-13 V. O. Garlea , R. Jin , D. Mandrus , B. Roessli , Q. Huang , M. Miller , A. J. Schultz , S. E. Nagler

A ferroelectric transition occurring simultaneously with helical spin order has been found in both the polycrystalline and single crystal samples of LiCuVO4. The system has Cu2+ spins (s=1/2) of the CuO2 chains formed of edge-sharing CuO4…

Strongly Correlated Electrons · Physics 2015-06-25 Yutaka Naito , Kenji Sato , Yukio Yasui , Yusuke Kobayashi , Yoshiaki Kobayashi , Masatoshi Sato

The compound Ba3HoRu2O9 magnetically orders at 50 K (TN1) followed by another complex magnetic ordering at 10.2 K (TN2). The 2nd magnetic phase transition was characterized by the co-existence of two competing magnetic ground states…

Strongly Correlated Electrons · Physics 2024-06-18 E. Kushwaha , G. Roy , M. Kumar , A. M. dos Santos , S. Ghosh , D. T. Adroja , V. Caignaert , O. Perez , A. Pautrat , T. Basu

We report a systematic study of the structure, electric and magnetic properties of Ca$_3$Co$_{2-x}$Mn$_x$O$_6$ single crystals with $x =$ 0.72 and 0.26. The DC and AC magnetic susceptibilities display anomalies with characteristic of the…

Materials Science · Physics 2017-09-08 J. Shi , J. D. Song , J. C. Wu , X. Rao , H. L. Che , Z. Y. Zhao , H. D. Zhou , J. Ma , R. R. Zhang , L. Zhang , X. G. Liu , X. Zhao , X. F. Sun

We present neutron scattering measurements on powder samples of the spinel FeSc2S4 that reveal a previously unobserved magnetic ordering transition occurring at 11.8(2)~K. Magnetic ordering occurs subsequent to a subtle cubic-to-tetragonal…

Strongly Correlated Electrons · Physics 2016-12-21 K. W. Plumb , Jennifer Morey , J. A. Rodriguez-Rivera , Hui Wu , A. A. Podlesnyak , T. M. McQueen , C. L. Broholm

The tetragonal copper oxide Bi$_2$CuO$_4$ has an unusual crystal structure with a three-dimensional network of well separated CuO$_4$ plaquettes. This material was recently predicted to host electronic excitations with an unconventional…

Strongly Correlated Electrons · Physics 2017-08-23 L. Zhao , H. Guo , W. Schmidt , K. Nemkovski , M. Mostovoy , A. C. Komarek

Magnetic and ferroelectric properties of layered geometrically frustrated cluster compound FeTe$_2$O$_5$Br were investigated with single-crystal neutron diffraction and dielectric measurements. Incommensurate amplitude modulated magnetic…

Materials Science · Physics 2009-10-01 M. Pregelj , O. Zaharko , A. Zorko , Z. Kutnjak , P. Jeglic , P. J. Brown , M. Jagodic , Z. Jaglicic , H. Berger , D. Arcon

The spinel MnV_2O_4 is a two-sublattice ferrimagnet, with site A occupied by the Mn^{2+} ion and site B by the V^{3+} ion. The magnon of the system, the transversal fluctuation of the total magnetization, is a complicated mixture of the…

Strongly Correlated Electrons · Physics 2009-11-13 Naoum Karchev

The spin ordering and spin-charge coupling in LuFe2O4 were investigated on the basis of density functional calculations and Monte Carlo simulations. The 2:1 ferrimagnetism arises from the strong antiferromagnetic intra-sheet Fe3+-Fe3+ and…

Materials Science · Physics 2009-12-22 H. J. Xiang , E. J. Kan , Su-Huai Wei , M. -H. Whangbo , Jinlong Yang

Ferrimagnetic spinel materials of formula AB2X4, where A and B are transition metals and X is oxygen or sulphur, hold promise for the realization of multiferroic characteristics. In this work, we report synthesis of spinel CoMn2O4 and…

Materials Science · Physics 2026-04-07 P. Kumar , P. Das , B. K. Kuanr , S. Patnaik

By studying the dielectric properties of the geometrically frustrated spinel CdV2O4, we observe ferroelectricity developing at the transition into the collinear antiferromagnetic ground state. In this multiferroic spinel, ferroelectricity…

A detailed study of poly- and single crystalline samples of the normal spinel HgCr2S4 is reported. The structural refinement reveals enhanced values of the atomic displacements suggesting closeness to a structural instability.…

Materials Science · Physics 2009-11-11 V. Tsurkan , J. Hemberger , A. Krimmel , H. -A. Krug von Nidda , P. Lunkenheimer , S. Weber , V. Zestrea , A. Loidl

Spinel oxides demonstrate significant technological promise due to the vast array of interrelated physical properties that their unique structure supports. Specifically, the Fe1+xV2-xO4 spinel system garners extensive interest due to the…

Vanadium spinels (ZnV_2O_4, MgV_2O_4, and CdV_2O_4) exhibit a sequence of structural and magnetic phase transitions, reflecting the interplay of lattice, orbital, and spin degrees of freedom. We offer a theoretical model taking into account…

Strongly Correlated Electrons · Physics 2007-05-23 O. Tchernyshyov

Multiferroic materials, which reveal magnetic and electric order, are in the focus of recent solid state research. Especially the simultaneous occurrence of ferroelectricity and ferromagnetism, combined with an intimate coupling of…

Strongly Correlated Electrons · Physics 2009-11-11 J. Hemberger , P. Lunkenheimer , R. Fichtl , H. -A. Krug von Nidda , V. Tsurkan , A. Loidl
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