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We investigate the polarization properties of high harmonics generated with the bichromatic counterrotating circularly polarized (BCCP) laser fields by numerically solving time-dependent Schr\"odinger equation (TDSE). It is found that, the…

Atomic Physics · Physics 2016-12-21 Xiaofan Zhang , Liang Li , Xiaosong Zhu , Xi Liu , Qingbin Zhang , Pengfei Lan , Peixiang Lu

We theoretically investigate correlated electron dynamics in high-harmonic generation (HHG), using all-electron \emph{ab initio} simulations for three-dimensional real alkali-metal atoms. The resulting harmonic spectra exhibit a plateau…

Atomic Physics · Physics 2019-04-10 Yang Li , Takeshi Sato , Kenichi L. Ishikawa

High-harmonic generation from solids can be utilized as probe of ultrafast dynamics, but thus far only over extended sample areas, since its spatial resolution is diffraction-limited. Here we propose spatial polarization gating, that is…

High-order harmonic generation in polyatomic molecules generally involves multiple channels, each associated with a different orbital. Their unambiguous assignment remains a major challenge for high-harmonic spectroscopy. Here we present a…

The harmonic generation has always been of fundamental interest in studying the nonlinear nature of any physical system. In the present study, Particle - In - Cell (PIC) simulations have been carried out to explore the harmonic generation…

Plasma Physics · Physics 2023-07-12 Trishul Dhalia , Rohit Juneja , Laxman Prasad Goswami , Srimanta Maity , Amita Das

We observe the generation of high harmonics in the plane perpendicular to the driving laser polarization and show that these are driven by the spin-orbit interaction. Using R-Matrix with time-dependence theory, we demonstrate that for…

We investigate the orientation dependence of high-order harmonic generation (HHG) from H$_2^+$ with different internuclear distances irradiated by intense laser fields both numerically and analytically. The calculated molecular HHG spectra…

Atomic Physics · Physics 2009-11-13 Yanjun Chen , Jie Liu , Bambi Hu

We present a theoretical model of high-harmonic generation from diatomic molecules. The theory includes effects of alignment as well as nuclear motion and is used to predict results for N$_2$, O$_2$, H$_2$ and D$_2$. The results show that…

Atomic Physics · Physics 2007-05-23 Christian Bruun Madsen , Lars Bojer Madsen

An accurate analytic model describing high-harmonic generation (HHG) in solids is derived. Extensive first-principles simulations within a time-dependent density-functional framework corroborate the conclusions of the model. Our results…

We carried out a joint theoretical and experimental study of the polarization of high-order harmonics generated from ZnO by intense infrared laser pulses. Experimentally we found that the dependence of parallel and perpendicular…

The generation of high-order harmonics in finite, hexagonal nanoribbons is simulated. Ribbons with armchair and zig-zag edges are investigated by using a tight-binding approach with only nearest neighbor hopping. By turning an alternating…

Mesoscale and Nanoscale Physics · Physics 2024-03-12 Hannah Jürß , Dieter Bauer

We theoretically investigate high-harmonic generation in hexagonal boron nitride with linearly polarized laser pulses. We show that imperfect recollisions between electron-hole pairs in the crystal give rise to an electron-hole-pair…

Atomic Physics · Physics 2020-04-22 Lun Yue , Mette Gaarde

High-harmonic generation in two-colour ($\omega-2\omega$) counter-rotating circularly polarised laser fields opens the path to generate isolated attosecond pulses and attosecond pulse trains with controlled ellipticity. The generated…

High-order frequency mixing in graphene using a two-color radiation field consisting of the fundamental and the second harmonic fields of an ultrashort linearly polarized laser pulse is studied. It is shown that the harmonics originated…

Mesoscale and Nanoscale Physics · Physics 2022-05-25 Hamlet K. Avetissian , Garnik F. Mkrtchian , Andreas Knorr

The underlying physics behind the molecular harmonic emission in relatively long sin$^2$-like laser pulses is investigated. We numerically solved the full-dimensional electronic time-dependent Schr\"{o}dinger equation beyond the…

Atomic Physics · Physics 2016-09-21 H. Ahmadi , M. Vafaee , A. Maghari

High-order harmonic generation with bicircular fields - the combination of counter-rotating circularly polarized pulses at different frequencies - results in a series of short-wavelength XUV harmonics with alternating circular…

Quantum Physics · Physics 2019-07-25 Emilio Pisanty , Álvaro Jiménez-Galán

High harmonic generation (HHG) is an extreme nonlinear process where intense pulses of light drive matter to emit high harmonics of the driving frequency, reaching the extreme ultraviolet (XUV) and x-ray spectral ranges. So far, the HHG…

We study high-order harmonic generation (HHG) resulting from the illumination of plasmonic nanostructures with a short laser pulse. We show that both the inhomogeneities of the local electric field and the confinement of the electron motion…

Atomic Physics · Physics 2012-04-27 M. F. Ciappina , Srdjan S. Acimovic , T. Shaaran , J. Biegert , R. Quidant , M. Lewenstein

Asymmetric molecules look different when viewed from one side or the other. This difference influences the electronic structure of the valence electrons, thereby giving stereo sensitivity to chemistry and biology. We show that attosecond…

An interesting property of high harmonic generation in solids is its laser polarization dependent nature which in turn provides information about the crystal and band structure of the generation medium. Here we report on the linear…