Related papers: Electronic coherence dynamics in trans-polyacetyle…
An optoelectronic oscillator exhibiting a large delay in its feedback loop is studied both experimentally and theoretically. We show that multiple square-wave oscillations may coexist for the same values of the parameters…
We report on the application of a dynamic decoherence control pulse sequence on a nuclear quadrupole transition in $Pr^{3+}:Y_2SiO_5$ . Process tomography is used to analyse the effect of the pulse sequence. The pulse sequence was found to…
A wide variety of experimental results and theoretical investigations in recent years have convincingly demonstrated that several transition metal oxides and other materials, have dominant states that are not spatially homogeneous. This…
A direct classical analog of the quantum dynamics of intrinsic decoherence in Hamiltonian systems, characterized by the time dependence of the linear entropy of the reduced density operator, is introduced. The similarities and differences…
The notion that decoherence rapidly reduces a superposition state to an incoherent mixture implicitly adopts a special representation, namely, the representation of preferred (pointer) states (PS). For weak or strong system-environment…
We present a perturbation approach rooted in time-dependent density-functional theory to calculate electron hole (eh)-pair excitation spectra during the non-adiabatic vibrational damping of adsorbates on metal surfaces. Our analysis for the…
Emergent strongly-correlated electronic phenomena in atomically-thin transition metal dichalcogenides are an exciting frontier in condensed matter physics, with examples ranging from bilayer superconductivity~\cite{zhao2023evidence} and…
The decoherence of a test particle interacting with an ideal gas is studied by the help of the effective Lagrangian, derived in the leading order of the perturbation expansion and in order $\ord{\partial^2_t}$. The stationary decoherence…
For the prototypical example of the Ising chain in a transverse field, we study the impact of decoherence on the sweep through a second-order quantum phase transition. Apart from the advance in the general understanding of the dynamics of…
We have studied the quantum oscillations of the conductance for arrays of connected mesoscopic metallic rings, in the presence of an external magnetic field. Several geometries have been considered: a linear array of rings connected with…
We analyze the entanglement between electronic and nuclear motions in molecular wave functions, by using different widely used ansatzes in molecular Hamiltonian models (H$^+_2$ in 1D and the Shin-Metiu model); namely, i) Born-Oppenheimer…
In this Thesis we study the quantum to classical transition process in the context of quantum mechanics and quantum field theory. We shall analyze the effects that general environments, namely ohmic and non-ohmic, at zero and high…
Quantum sensors and qubits are usually two-level systems (TLS), the quantum analogs of classical bits which assume binary values '0' or '1'. They are useful to the extent to which they can persist in quantum superpositions of '0' and '1' in…
In quantum systems, coherent superpositions of electronic states evolve on ultrafast timescales (few femtosecond to attosecond, 1 as = 0.001 fs = 10^{-18} s), leading to a time dependent charge density. Here we exploit the first attosecond…
Coherence and de-coherence are the most fundamental steps that follow the initial photo-excitation occurring in typical Pump&Probe experiments. Indeed, the initial external laser pulse transfers coherence to the system in terms of creation…
Quantum states inevitably decay with time into a probabilistic mixture of classical states, due to their interaction with the environment and measurement instrumentation. We present the first measurement of the decoherence dynamics of…
Microscopic models of electronic subsystems with orbital degeneracy of energy states and non-diagonal matrix elements of electron interactions (correlated hopping) are considered within the configuration-operator approach. Equations for…
We investigate the time evolution of a superposition of macroscopically distinct quantum states in a system of two-level atoms interacting with a thermal environment of photon modes. We show that the atomic coherent states are robust…
Conjugated polymers are soft, one-dimensional conductors that admit complex interactions between their polymeric, conformational degrees of freedom and their electronic ones. The presence of extended electronic states along their backbone…
Organic semiconductors have the remarkable property that their optical excitation not only generates charge-neutral electron-hole pairs (excitons) but also charge-separated polaron pairs with high yield. The microscopic mechanisms…