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A simple monatomic system in two dimensions with a double-well interaction potential is investigated in a wide range of temperature by molecular dynamics simulation. The system is melted and equilibrated well above the melting temperature,…

Disordered Systems and Neural Networks · Physics 2015-05-13 Tomoko Mizuguchi , Takashi Odagaki

Supercooled liquids give rise, by homogeneous nucleation, to solid superclusters acting as building blocks of glass, ultrastable glass, and glacial glass phases before being crystallized. Liquid-to-liquid phase transitions begin to be…

Disordered Systems and Neural Networks · Physics 2019-06-26 Robert F. Tournier

At temperatures well below their glass transition, the deformation properties of bulk metallic glasses are characterised by a sharp transition from elasticity to plasticity, a reproducible yield stress, and an approximately linear decrease…

Soft Condensed Matter · Physics 2013-11-18 P. M. Derlet , R. Maaß

Isotopically layered amorphous solid water films were used to measure the diffusivity of deeply supercooled liquid water near the glass transition. The films, composed of separate layers of oxygen 16 and oxygen 18 labeled water, were grown…

Soft Condensed Matter · Physics 2025-02-06 R. Scott Smith , Wyatt A. Thornley , Greg A. Kimmel , Bruce D. Kay

We give a simple demonstration of the formula relating the glass transition temperature, $T_g$, to the molar concentration $x$ of a modifier in two types of glasses: binary glasses, whose composition can be denoted by $X_nY_m+xM_pY_q$, with…

Disordered Systems and Neural Networks · Physics 2015-06-25 R. Kerner , M. Micoulaut

Thermodynamic multi-component solution solidification approach to liquid-to-glass transition is proposed and actual mechanisms underlying vitrification, other than viscous slowdown, are identified. Due to polydisperse aggregation in liquid…

Materials Science · Physics 2022-09-14 Vladimir Belostotsky

The lack of thermal stability, originating from their metastable nature, has been one of the paramount obstacles that hinder the wide range of applications of metallic glasses. We report that the stability of a metallic glass can be…

We propose a method to study quantitatively the glass transition in a system of interacting particles. In spite of the absence of any quenched disorder, we introduce a replicated version of the hypernetted chain equations. The solution of…

Condensed Matter · Physics 2009-10-28 Marc Mezard , Giorgio Parisi

We propose a new simple way to evaluate the effect of anharmonicity on a system's thermodynamic functions such as heat capacity. In this approach, the contribution of all potentially complicated anharmonic effects to constant-volume heat…

Statistical Mechanics · Physics 2015-06-15 E. I. Andritsos , E. Zarkadoula , A. E. Phillips , M. T. Dove , C. J. Walker , V. V. Brazhkin , K. Trachenko

We study a recently introduced model of one-component glass-forming liquids whose constituents interact with anisotropic potential. This system is interesting per-se and as a model of liquids like glycerol (interacting via hydrogen bonds)…

Materials Science · Physics 2009-11-13 Valery Ilyin , Edan Lerner , Ting-Shek Lo , Itamar Procaccia

A universal dynamical crossover temperature, Tcr, in glassy liquids, associated with the {\alpha}-\b{eta} bifurcation temperature, TB, has been observed in dielectric spectroscopy and other experiments. Tcr lies significantly above the…

Soft Condensed Matter · Physics 2024-03-29 Shubham Kumar , Sarmistha Sarkar , Biman Bagchi

We address the interesting temperature range of a glass forming system where the mechanical properties are intermediate between those of a liquid and a solid. We employ an efficient Monte-Carlo method to calculate the elastic moduli, and…

Statistical Mechanics · Physics 2009-11-13 Valery Ilyin , Nataliya Makedonska , Itamar Procaccia , Nurith Schupper

We consider experimental data on the dynamics of water (1) in glass-forming aqueous mixtures with glass transition temperature Tg approaching the putative Tg=136 K of water from above and below, (2) in confined spaces of nanometer in size…

Statistical Mechanics · Physics 2015-05-28 S. Capaccioli , K. L. Ngai

The Kovacs effect is a remarkable feature of the ageing dynamics of glass forming liquids near the glass transition temperature. It consists in a non-monotonous evolution of the volume/enthalpy after a succession of two abrupt temperature…

Soft Condensed Matter · Physics 2021-10-20 Matteo Lulli , Chun-Shing Lee , Ling-Han Zhang , Hai-Yao Deng , Chi-Hang Lam

Low frequency dielectric spectroscopy and thermally stimulated discharge measurements of charge density wave (CDW) system K$_{0.3}$MoO$_{3}$ are presented. Below 80 K two distinct relaxational processes are observed, which freeze at finite…

Condensed Matter · Physics 2016-08-16 D. Starešinić , K. Hosseini , W. Brütting , K. Biljaković , E. Riedel , S. van Smaalen

We present results of the coefficient of thermal expansion for the frustrated quasi-two-dimensional molecular conductor $\theta$-(BEDT-TTF)$_2$RbZn(SCN)$_4$ for temperatures 1.5 K $\leq T \leq$ 290 K. A pronounced first-order phase…

Strongly Correlated Electrons · Physics 2024-05-08 Yohei Saito , Owen Ganter , Chao Shang , Kenichiro Hashimoto , Takahiko Sasaki , Stephen M. Winter , Jens Müller , Michael Lang

We have calculated heat capacity of TiO2 nanoparticles in three stable polymorphs by applying size and surface effects on heat capacity of the bulk structure. The size and surface corrections were imposed on the acoustic and optical bulk…

Materials Science · Physics 2013-07-30 M. Saeedian , M. Mahjour-Shafiei , E. Shojaee , M. R. Mohammadizadeh

A model of low-temperature polar liquids is constructed that accounts for configurational heat capacity, entropy, and the effect of a strong electric field on the glass transition. The model is based on Pad{\'e}-truncated perturbation…

Soft Condensed Matter · Physics 2016-08-03 D. V. Matyushov

The thermal conductivity of glasses is well-known to be significantly harder to theoretically describe compared to crystalline materials. Because of this fact, the fundamental understanding of thermal conductivity in glasses remain…

Disordered Systems and Neural Networks · Physics 2024-08-05 Philip Rasmussen , Søren Strandskov Sørensen

The thermal conductivity, heat capacity and heat release of NbTi, NbTi-H and NbTi-D were measured at low temperatures. All three systems reveal low temperature anomalies typical for structural glasses. It is shown that above a concentration…

Disordered Systems and Neural Networks · Physics 2016-10-17 S. Sahling , S. Abens , V. L. Katkov , V. A. Osipov