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To investigate the magnetic properties of SmFe$_{12}$, we construct an effective spin model, where magnetic moments, crystal field (CF) parameters, and exchange fields at 0 K are determined by first principles. Finite temperature magnetic…

Materials Science · Physics 2020-12-02 Takuya Yoshioka , Hiroki Tsuchiura , Pavel Novák

On the basis of a first-principles, relativistic electronic structure theory of finite temperature metallic magnetism, we investigate the variation of magnetic anisotropy, K, with magnetisation, M, in metallic ferromagnets. We apply the…

Materials Science · Physics 2009-11-10 J. B. Staunton , S. Ostanin , S. S. A. Razee , B. L. Gyorffy , L. Szunyogh , B. Ginatempo , Ezio Bruno

ZrMnP and HfMnP single crystals are grown by a self-flux growth technique and structural as well as temperature dependent magnetic and transport properties are studied. Both compounds have an orthorhombic crystal structure. ZrMnP and HfMnP…

We present a study of high-quality BaCo$_2$(PO$_4$)$_2$ single crystals via magnetization, heat-capacity, thermal-expansion and magnetostriction measurements. Sharp anomalies in the thermodynamic properties at $T_N=3.4\,$K reveal a…

Strongly Correlated Electrons · Physics 2023-02-08 Xiao Wang , Rohit Sharma , Petra Becker , Ladislav Bohatý , Thomas Lorenz

The origins of the anomalous temperature dependence of magnetocrystalline anisotropy in (Fe$_{1-x}$Co$_{x}$)$_{2}$B alloys are elucidated using first-principles calculations within the disordered local moment model. Excellent agreement with…

Materials Science · Physics 2015-11-17 Ivan A. Zhuravlev , Vladimir P. Antropov , Kirill D. Belashchenko

Recent work [1] demonstrated high coercivity and magnetic moment in cobalt carbide nanoparticle assemblies and explained the high coercivity from first principles in terms of the high magnetocrystalline anisotropy of the cobalt carbide…

Mesoscale and Nanoscale Physics · Physics 2018-09-26 Pallabi Sutradhar , Shiv N. Khanna , Jayasimha Atulasimha

Here we report an unconventional magnetic and transport phenomenon in a layered cobalt oxide, NaxCoO2. Only for x = 0.75, a magnetic transition of the second order was clearly detected at Tm ~ 22 K where an apparent specific-heat jump, an…

Strongly Correlated Electrons · Physics 2009-11-07 T. Motohashi , R. Ueda , E. Naujalis , T. Tojo , I. Terasaki , T. Atake , M. Karppinen , H. Yamauchi

Magnetism of Cu$_2$(OH)$_3$Br single crystals based on a triangular lattice is studied by means of magnetic susceptibility, pulsed-field magnetization, and specific heat measurements. There are two inequivalent Cu$^{2+}$ sites in an…

Strongly Correlated Electrons · Physics 2019-09-04 Z Y Zhao , H L Che , R Chen , J F Wang , X F Sun , Z Z He

We investigate the interplay of quantum fluctuations and magnetic anisotropies in metallic ferromagnets. Our central result is that fluctuations close to a quantum critical point can drive the moments to point along a magnetic hard axis. As…

Strongly Correlated Electrons · Physics 2014-10-07 F. Krüger , C. J. Pedder , A. G. Green

Precise magnetic hysteresis measurements of small single crystals of Mn$_{12}$ acetate of spin 10 have been conducted down to 0.4 K using a high sensitivity Hall magnetometer. At higher temperature (>1.6K) step-like changes in magnetization…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 Andrew D. Kent , Yicheng Zhong , Louisa Bokacheva , Daniel Ruiz , David N. Hendrickson , M. P. Sarachik

We present magnetization and dilatometry measurements on the honeycomb cobaltate Na$_3$Co$_2$SbO$_6$ and map out its detailed field-temperature phase diagram down to sub-Kelvin temperatures. Our data for in-plane magnetic fields show a…

We report the crystal growth and structural, magnetic, conductivity, and specific heat investigations of Rb(1-x)Fe(2-y)Se2 single crystals with varying stoichiometry prepared by self-flux and Bridgman methods. The system exhibits a strongly…

Superconductivity · Physics 2011-11-01 V. Tsurkan , J. Deisenhofer , A. Günther , H. -A. Krug von Nidda , S. Widmann , A. Loidl

We report on a 59Co NMR investigation of the trigonal cobaltate Ca3Co2O6 carried out on a single crystal, providing precise determinations of the electric field gradient and chemical shift tensors, and of the internal magnetic fields at the…

Strongly Correlated Electrons · Physics 2015-05-20 G. Allodi , R. De Renzi , S. Agrestini , C. Mazzoli , M. R. Lees

Magnetic behavior of BaMoP$_2$O$_8$ with the spatially anisotropic triangular arrangement of the $S=1$ Mo$^{4+}$ ions is explored using thermodynamic measurements, neutron diffraction, and density-functional band-structure calculations. A…

We present a thorough study on the magnetoanisotropic properties and magnetocaloric effect in the layered ferromagnetic Cr$_4$Te$_5$ single crystals by performing the critical behaviour analysis of magnetization isotherms. The critical…

Materials Science · Physics 2022-09-20 Shubham Purwar , Susmita Changdar , Susanta Ghosh , S. Thirupathaiah

The anisotropic magnetic properties of the antiferromagnetic compound CePd$_2$Ge$_2$, crystallizing in the tetragonal crystal structure have been investigated in detail on a single crystal grown by Czochralski method. From the electrical…

Strongly Correlated Electrons · Physics 2015-06-16 Arvind Maurya , R. Kulkarni , S. K. Dhar , A. Thamizhavel

Large magnetic anisotropy and coercivity are key properties of functional magnetic materials and are generally associated with rare earth elements. Here we show an extreme, uniaxial magnetic anisotropy and the emergence of magnetic…

Strongly Correlated Electrons · Physics 2014-02-27 A. Jesche , R. W. McCallum , S. Thimmaiah , J. L. Jacobs , V. Taufour , A. Kreyssig , R. S. Houk , S. L. Bud'ko , P. C. Canfield

We present here high resolution magnetization measurements on high-quality BaFe$_{2(1-x)}$Co$_{2x}$As$_{2}$, 0$\leq$x$\leq$0.046 as-grown single crystals. The results confirm the existence of a magnetic tricritical point in the ($x$,$T$)…

Superconductivity · Physics 2015-05-28 C. R. Rotundu , R. J. Birgeneau

We report the discovery of a giant out-of-plane coercivity in the Fe-doped Mn3Sn single crystals. The compound of Mn2.42Fe0.58Sn exhibits a series of magnetic transitions accompanying with large magnetic anisotropy and electric transport…

Applied Physics · Physics 2023-10-31 Weihao Shen , Yalei Huang , Xinyu Yao , Fangyi Qi , Guixin Cao

We report a study of anisotropy in transport and magnetic properties of K0.64Fe1.44Se2.00 single crystals. The anisotropy in resistivity is up to one order of magnitude between 1.8 K and 300 K. Magnetic susceptibility exhibits weak…

Superconductivity · Physics 2011-05-19 Hechang Lei , C. Petrovic