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An overview of computational methods to describe high-dimensional potential energy surfaces suitable for atomistic simulations is given. Particular emphasis is put on accuracy, computability, transferability and extensibility of the methods…

Chemical Physics · Physics 2020-07-08 Oliver T. Unke , Debasish Koner , Sarbani Patra , Silvan Käser , Markus Meuwly

Particle suspensions are ubiquitous in our daily life, but are not well understood due to their complexity. During the last twenty years, various simulation methods have been developed in order to model these systems. Due to varying…

Soft Condensed Matter · Physics 2011-03-16 Jens Harting , Martin Hecht , Hans J. Herrmann , Sean McNamara

We describe the thermodynamic state of a single-phase fluid confined to a porous medium with Hill's thermodynamics of small systems, also known as nanothermodynamics. This way of defining small system thermodynamics, with a separate set of…

Chemical Physics · Physics 2022-02-01 Olav Galteland , Michael T. Rauter , Kevin K. Varughese , Dick Bedeaux , Signe Kjelstrup

In this work, we provide a solution to the problem of computing collision stress in particle-tracking simulations. First, a formulation for the collision stress between particles is derived as an extension of the virial stress formula to…

Fluid Dynamics · Physics 2019-02-18 Wen Yan , Huan Zhang , Michael J. Shelley

Modeling electronic systems is an important application for quantum computers. In the context of materials science, an important open problem is the computational description of chemical reactions on surfaces. In this work, we outline a…

Stress, or pressure, is a central quantity in engineering and remains vital in molecular modelling. However, the commonly used virial stress tensor is invalid for an inhomogeneous fluid, which is essential in fluid dynamics and…

Chemical Physics · Physics 2026-01-13 E. R. Smith

Molecular dynamics refers to the computer simulation of a material at the atomic level. An open problem in numerical analysis is to explain the apparent reliability of molecular dynamics simulations. The difficulty is that individual…

Numerical Analysis · Mathematics 2015-05-13 P. F. Tupper

Classical molecular dynamics simulations of hydrogen plasmas have been performed with emphasis on the analysis of equilibration process. Theoretical basis of simulation model as well as numerically relevant aspects -- such as the proper…

Plasma Physics · Physics 2024-02-07 M. A. Gigosos , D. Gonzalez-Herrero , R. Florido , A. Calisti , S. Ferri , B. Talin

The identification of local pressure in active matter systems remains a subject of considerable debate. Through theoretical calculations and extensive simulations of various active systems, we demonstrate that intrinsic pressure (defined in…

Soft Condensed Matter · Physics 2025-07-22 Zihao Sun , Longfei Li , Chuyun Wang , Jing Wang , Huaicheng Chen , Gao Wang , Liyu Liu , Fangfu Ye , Mingcheng Yang

We discuss different definitions of pressure for a system of active spherical particles driven by a non-thermal coloured noise. We show that mechanical, kinetic and free-energy based approaches lead to the same result up to first order in…

Statistical Mechanics · Physics 2016-03-18 Umberto Marini Bettolo Marconi , Claudio Maggi , Simone Melchionna

Motivated by existing models used for soft body simulation which are rather complex to implement, we present a novel technique which is based on simple laws of physics and gives high quality results in real-time. We base the implementation…

Computational Physics · Physics 2007-05-23 Matyka Maciej , Ollila Mark

We present a multiscale hybrid particle-field scheme for the simulation of relaxation and diffusion behavior of soft condensed matter systems. It combines particle-based Brownian dynamics and field-based local dynamics in an adaptive sense…

Soft Condensed Matter · Physics 2017-09-06 Shuanhu Qi , Friederike Schmid

In order to provide a formally correct thermodynamical description of inhomogeneous fluids valid on all length scales down to the classical limit we postulate that all extensive quantities have locally extensive analogues. We derive local…

Statistical Mechanics · Physics 2016-08-14 Aljaž Godec , Janko Jamnik , Franci Merzel

A robust method to handle vacuum and near vacuum regions in hybrid simulations for space and astrophysical plasmas is presented. The conventional hybrid simulation model dealing with kinetic ions and a massless charge-neutralizing electron…

Plasma Physics · Physics 2015-06-22 Takanobu Amano , Katsuaki Higashimori , Keisuke Shirakawa

We introduce and test via molecular simulation a simple model for predicting the manner in which interparticle interactions and thermodynamic conditions impact the single-particle free-volume distributions of equilibrium fluids. The model…

Soft Condensed Matter · Physics 2007-05-23 William P. Krekelberg , Venkat Ganesan , Thomas M. Truskett

For simulation studies of (macro) molecular liquids it would be of significant interest to be able to adjust or increase the level of resolution within one region of space, while allowing for the free exchange of molecules between open…

Consider briefly the equations of fluid dynamics-they describe the enormous wealth of detail in all the interacting physical elements of a fluid flow-whereas in applications we want to deal with a description of just that which is…

chao-dyn · Physics 2016-08-31 A. J. Roberts

Colloidal dispersions are widely found in systems ranging from natural environments to industrial materials. Their macroscopic properties such as viscosity and light scattering depend on their dispersibility, which is characterized by…

Soft Condensed Matter · Physics 2026-05-22 Keita Saito , Fumito Araoka

It is often difficult to quantitatively determine if a new molecular simulation algorithm or software properly implements sampling of the desired thermodynamic ensemble. We present some simple statistical analysis procedures to allow…

Statistical Mechanics · Physics 2013-03-04 Michael R. Shirts

Mutual information between local stress and local non-affine deformation is proposed as a collective field variable quantifying the {\em local softness} of soft materials. The liquid-solid transition in a simple liquid is considered as a…

Soft Condensed Matter · Physics 2025-02-18 Tamoghna Das