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Related papers: Tuning the spin dynamics of kagome systems

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We report an electron spin resonance investigation of the geometrically frustrated spin-1/2 kagome antiferromagnet vesignieite, BaCu$_3$V$_2$O$_8$(OH)$_2$. Analysis of the line widths and line shifts indicates the dominance of in-plane…

Strongly Correlated Electrons · Physics 2013-10-29 A. Zorko , F. Bert , A. Ozarowski , J. van Tol , D. Boldrin , A. S. Wills , P. Mendels

We report thermodynamic measurements of the S=1/2 kagome lattice antiferromagnet ZnCu$_{3}$(OH)$_{6}$Cl$_{2}$, a promising candidate system with a spin-liquid ground state. Using single crystal samples, the magnetic susceptibility both…

Strongly Correlated Electrons · Physics 2012-04-16 Tianheng Han , Shaoyan Chu , Young S. Lee

Motivated by the recent experiments on the new spin half Kagome compound ZnCu3(OH)6Cl2, we study a phenomenological model of a frustrated quantum magnet. The model has a spin liquid groundstate and is constructed so as to mimic the…

Strongly Correlated Electrons · Physics 2009-11-13 R. Chitra , M. J. Rozenberg

We report magnetization, electron spin resonance (ESR), and muon spin relaxation ($\mu $SR) measurements on single crystals of the $S=1/2$ (Cu$% ^{+2}$) kagom\'{e} compound Cu(1,3-benzendicarboxylate). The $\mu $SR is carried to…

Strongly Correlated Electrons · Physics 2015-06-18 Oren Ofer , Lital Marcipar , V. Ravi Chandra , Snir Gazit , Daniel Podolsky , Daniel P. Arovas , Amit Keren

The spin-$\frac{1}{2}$ kagome antiferromagnet is an archetypal frustrated system predicted to host a variety of exotic magnetic states. We show using neutron scattering measurements that deuterated vesignieite…

Strongly Correlated Electrons · Physics 2018-09-12 D. Boldrin , B. Fåk , E. Canévet , J. Ollivier , H. C. Walker , P. Manuel , D. Khalyavin , A. S. Wills

The magnetization of two spin-1/2 kagome antiferromagnets, volborthite and vesignieite, has been measured in pulsed magnetic fields up to 68 T. A magnetization plateau is observed for each compound near the highest magnetic field.…

Strongly Correlated Electrons · Physics 2015-05-27 Yoshihiko Okamoto , Masashi Tokunaga , Hiroyuki Yoshida , Akira Matsuo , Koichi Kindo , Zenji Hiroi

Two kagome compounds, volborthite Cu3V2O7(OH)2-2H2O and herbertsmithite ZnCu3(OH)6Cl2, are compared in order to derive information about the intrinsic properties of the spin-1/2 kagome antiferromagnet. Volborthite shows a broad maximum at T…

Strongly Correlated Electrons · Physics 2009-11-13 Z Hiroi , H Yoshida , Y Okamoto , M Takigawa

New physics can emerge in magnetic materials where quantum fluctuations are enhanced due to reduced dimensionality and strong frustration. One long sought example is the resonating-valence-bond (RVB) state, where atomic magnetic moments are…

Strongly Correlated Electrons · Physics 2013-07-19 Tian-Heng Han , Joel S. Helton , Shaoyan Chu , Daniel G. Nocera , Jose A. Rodriguez-Rivera , Collin Broholm , Young S. Lee

We have performed thermodynamic and neutron scattering measurements on the S=1/2 kagome lattice antiferromagnet Zn Cu_3 (OH)_6 Cl_2. The susceptibility indicates a Curie-Weiss temperature of ~ -300 K; however, no magnetic order is observed…

Strongly Correlated Electrons · Physics 2007-05-23 J. S. Helton , K. Matan , M. P. Shores , E. A. Nytko , B. M. Bartlett , Y. Yoshida , Y. Takano , A. Suslov , Y. Qiu , J. -H. Chung , D. G. Nocera , Y. S. Lee

We use Raman scattering to study spin, charge, and lattice dynamics in various phases of Ca_{2-x}Sr_{x}RuO_{4}. With increasing substitution of Ca by Sr in the range 0 =< x < 0.2, we observe (1) evidence for an increase of the…

Strongly Correlated Electrons · Physics 2009-11-10 H. Rho , S. L. Cooper , S. Nakatsuji , H. Fukazawa , Y. Maeno

Special arrangements of atoms with more than one atom per unit cell, including honeycomb or kagome (woven bamboo mat) lattices, can host propagating excitations with non-trivial topology as defined by their evolution along closed paths in…

We have used Raman scattering to investigate the magnetic excitations and lattice dynamics in the prototypical spin-orbit Mott insulators Sr2IrO4 and Sr3Ir2O7. Both compounds exhibit pronounced two-magnon Raman scattering features with…

Strongly Correlated Electrons · Physics 2016-04-06 H. Gretarsson , N. H. Sung , M. Hoeppner , B. J. Kim , B. Keimer , M. Le Tacon

Recent neutron scattering experiments on the spin-1/2 kagome lattice antiferromagnet ZnCu3(OH)6Cl2 (Herbertsmithite) provide the first evidence of fractionalized excitations in a quantum spin liquid state in two spatial dimensions. In…

Strongly Correlated Electrons · Physics 2014-04-03 Matthias Punk , Debanjan Chowdhury , Subir Sachdev

Thermodynamic investigations on volborthite (Cu3V2O7(OH)2 2H2O), which possesses a two-dimensional kagome structure of S-1/2 spins, are presented. The low-temperature heat capacities of volborthite and its Zn analogue compound were measured…

Strongly Correlated Electrons · Physics 2010-08-12 Satoshi Yamashita , Tomoya Moriura , Yasuhiro Nakazawa , Hiroyuki Yoshida , Yoshihiko Okamoto , Zenji Hiroi

Motivated by recent experiments on the vanadium oxyfluoride material DQVOF, we examine possible spin liquid phases on a breathing kagome lattice of S=1/2 spins. By performing a projective symmetry group analysis, we determine the possible…

Strongly Correlated Electrons · Physics 2017-02-15 Robert Schaffer , Yejin Huh , Kyusung Hwang , Yong Baek Kim

Raman scattering is an excellent method for simultaneously determining the dynamics of lattice, spin, and charge degrees of freedom. Furthermore, polarization selection rules in Raman scattering enable momentum-resolved quasiparticle…

Strongly Correlated Electrons · Physics 2024-09-04 Reshma Kumawat , Shubham Farswan , Simranjeet Kaur , Smriti Bhatia , Kaushik Sen

Volborthite compound is one of the very few realizations of S=1/2 quantum spins on a highly frustrated kagome-like lattice. Low-T SQUID measurements reveal a broad magnetic transition below 2K which is further confirmed by a peak in the 51V…

Strongly Correlated Electrons · Physics 2009-11-11 F. Bert , D. Bono , P. Mendels , F. Ladieu , F. Duc , J. -C Trombe , P. Millet

In two-dimensional (2D) metallic kagome lattice materials, destructive interference of electronic hopping pathways around the kagome bracket can produce nearly localized electrons, and thus electronic bands that are flat in momentum space.…

We report results of 51V NMR in the field-induced phase of volborthite Cu3V2O7(OH)dot2H2O, a spin-1/2 antiferromagnet on a distorted kagome lattice. In magnetic fields above 4.5 T, two types of V sites with different spin-echo decay rates…

Strongly Correlated Electrons · Physics 2017-12-01 M. Yoshida , M. Takigawa , H. Yoshida , Y. Okamoto , Z. Hiroi

The properties of the groundstate and first excitations of 2dimensionnal quantum antiferromagnets are rapidly sketched. A special emphasis is put on the gapped phases: Valence Bond Crystals and the two types of Spin Liquids. New results on…

Strongly Correlated Electrons · Physics 2007-05-23 C. Lhuillier , P. Sindzingre