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The assessed phase diagram of the boron-carbon system contains a single non-stoichiometric boron-carbide phase of rhombohedral symmetry with a broad, thermodynamically improbable, low temperature composition range. We combine first…

Materials Science · Physics 2014-02-10 William P. Huhn , Michael Widom

Boron carbide exhibits intrinsic substitutional disorder over a broad composition range. The structure consists of 12-atom icosahedra placed at the vertices of a rhombohedral lattice, together with a 3-atom chain along the 3-fold axis. In…

Materials Science · Physics 2017-02-08 Sanxi Yao , Qin Gao , Michael Widom

Boron Carbide exhibits a broad composition range, implying a degree of intrinsic substitutional disorder. While the observed phase has rhombohedral symmetry (space group R3(bar)m), the enthalpy minimizing structure has lower, monoclinic,…

Materials Science · Physics 2017-07-04 Sanxi Yao , W. P. Huhn , M. Widom

Configurationally disordered crystalline boron carbide, B$_{4}$C, is studied using first-principles calculations. We investigate both dilute and high concentrations of carbon-boron substitutional defects. For the latter purpose, we suggest…

Materials Science · Physics 2015-09-01 A. Ektarawong , S. I. Simak , L. Hultman , J. Birch , B. Alling

Raman spectra of PbZr1-xTixO3 ceramics with titanium concentration varying between 0.40 and 0.60 were measured at 7 K. By observing the concentration-frequency dependence of vibrational modes, we identified the boundaries among…

Recently a new monoclinic phase in the PbZr(1-x)TixO3 ceramic system has been reported by Noheda et al. for the composition x= 0.48. In the present work, samples with Ti contents of x= 0.47 and 0.50, which are both tetragonal below their…

Materials Science · Physics 2007-05-23 B. Noheda , J. A. Gonzalo , A. Caballero , C. Moure , D. E. Cox , G. Shirane

Noting the structural relationships between phases of carbon and boron carbide with phases of boron nitride and boron subnitride, we investigate their mutual solubilities using a combination of first principles total energies supplemented…

Materials Science · Physics 2016-04-13 Hantao Zhang , Sanxi Yao , Michael Widom

Boron carbide, a lightweight, high temperature material, has various applications as a structural material and as a neutron absorber. The large solubility range of carbon in boron, between $\approx$ 9% and 20%, stems from the…

Materials Science · Physics 2021-06-09 Guido Roma , Kevin Gillet , Antoine Jay , Nathalie Vast , Gaëlle Gutierrez

Boron carbide is a ceramic material with unique properties widely used in numerous, including armor, applications. Its mechanical properties, mechanism of compression, and limits of stability are of both scientific and practical value.…

A previously unreported ferroelectric phase has been revealed on a highly homogeneous sample of Pb(Zr0.52Ti0.48)O3 by high-resolution synchrotron x-ray powder diffraction measurements. At ambient temperature the sample has tetragonal…

Materials Science · Physics 2009-10-31 B. Noheda , D. E. Cox , G. Shirane , J. A. Gonzalo , L. E. Cross , S-E. Park , .

Two novel room-temperature phase transitions are observed, via synchrotron x-ray diffraction and Raman spectroscopy, in the Pb(Zr0.52Ti0.48)O3 alloy under hydrostatic pressures up to 16 GPa. A monoclinic (M)-to-rhombohedral (R1) phase…

Condensed Matter · Physics 2009-11-10 A. Sani , B. Noheda , I. A. Kornev , L. Bellaiche , P. Bouvier , J. Kreisel

The formation of boron carbide under high pressures and from elemental reactants has been studied and optimum parameters have been determined by varying the (P, T, reactants) conditions. To this end, stoichiometric mixtures of commercial…

Materials Science · Physics 2021-07-23 Amrita Chakraborti , Nicolas Guignot , Nathalie Vast , Yann Le Godec

Density Functional Theory calculations using the quasi-harmonic approximation have been used to calculate the solid Hugoniot of two polytypes of boron carbide up to 100 GPa. Under the assumption that segregation into the elemental phases…

Materials Science · Physics 2017-06-28 Andrew Shamp , Eva Zurek , Tadashi Ogitsu , Dayne E. Fratanduono , Sebastien Hamel

We present an ab-initio study of boron nitride as well as carbon allotropes. Their relative thermodynamic stabilities and structural phase transitions from low- to high-density phases are investigated. Pressure-temperature phase diagrams…

Materials Science · Physics 2019-02-22 Thomas Gruber , Andreas Grüneis

Heteroepitaxial boron carbide (BxC) can be grown on Si face 4H-SiC(0001) using a two-step process involving substrate boridation at 1200$^\circ$C under BCl3 + H2 followed by a chemical vapor deposition (CVD) growth step at 1600$^\circ$C by…

Group theoretical aspects of the three temperature-dependent and temperature-reversible experimentally observed phase transitions in the KNbO3 crystal (cubic-tetragonal, tetragonal-orthorhombic, orthorhombic-rhombohedral) in the framework…

Materials Science · Physics 2024-11-05 R. A. Evarestov , Yu. E. Kitaev , S. S. Novikov

We present theoretical studies of morphology, stability, and electronic structure of monolayer hexagonal CBN alloys with rich content of h-BN and carbon concentration not exceeding 50 %. Our studies are based on the bond order type of the…

Materials Science · Physics 2019-06-26 Agnieszka Jamróz , Jacek A. Majewski

In this work, the successful heteroepitaxial growth of boron carbide (B x C) on 4HSiC(0001) 4{\textdegree} off substrate using chemical vapor deposition (CVD) is reported. Towards this end, a two-step procedure was developed, involving the…

The local structure of V$_{2}$O$_{3}$, an archetypal strongly correlated electron system that displays a metal-insulator transition around 160 K, has been investigated via pair distribution function (PDF) analysis of neutron and x-ray total…

Strongly Correlated Electrons · Physics 2021-11-30 Ethan R. A. Fletcher , Kentaro Higashi , Yoav Kalcheim , Hiroshi Kageyama , Benjamin A. Frandsen

A first-principles-derived approach is used to study structural, piezoelectric and dielectric properties of Pb(Zr_{1-x}Ti_{x})O_{3} (PZT) solid solutions near the morphotropic phase boundary at low temperature. Three ferroelectric phases…

Materials Science · Physics 2007-05-23 L. Bellaiche , A. Garcia , David Vanderbilt
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